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FNG SiC EXPERIMENT
1. Name of Experiment: ------------------ FNG Benchmark Experiment on Silicon Carbide (SiC) (2001) 2. Purpose and Phenomena Tested: ---------------------------- The purpose is to validate the cross sections of Si and of C in the European Fusion File (EFF), as the SiC, in the form of ceramic matrix (SiC-fiber/SiC), is a candidate structural material for the fusion reactor and its development is pursued in the European Fusion Technology Program. The experiment [1] - [4] was performed at the 14 MeV Frascati Neutron Generator (FNG) on a monolithic, sintered SiC block. 3. Description of Source and Experimental Configuration: ---------------------------------------------------- The 14-MeV d-T Frascati Neutron Generator (FNG, [5]) was the neutron source. The angular dependence of the source intensity is presented in Table 1 and in Figure 1. The angular dependence of the source energy distribution is given in Table 2 and in Figure 2. The geometry of the mock-up is outlined in Figure 3. The experimental set-up consisted of a block of sintered SiC (45.72 cm x 45.72 cm, 71.12 cm in thickness), located in front of the FNG target, 5.3 cm from the neutron source. The SiC block was assembled with a total of 116 bricks. Inside the block, four experimental positions at different penetration depths were available to locate detectors of various types (activation foils, TLD holders, active spectrometers). The average weight density of the used SiC was 3.158 g/cm3, major impurities were boron (0.19 % in weight), aluminium (0.79 wt%) and iron (0.14 wt%). 4. Measurement System: ------------------ The following quantities are measured : a - Neutron reaction rates by activation foils b - Nuclear heating by thermo-luminescent detectors (GR-200A) Four different reactions: 197Au(n,g), 58Ni(n,p), 27Al(n,a) and 93Nb(n,2n) were used to derive the neutron flux, from thermal energy up to the fusion neutron peak. The reaction rates were measured at four experimental positions, 10.41 cm, 25.65 cm, 40.89 cm and 56.13 cm respectively from the block surface, using the radiometric techniques based upon the use of absolutely calibrated HPGe detectors. The overall contribution to the quoted uncertainty comes from the HPGe calibration (±2%), measured activity (<±3%) and total neutron yield (±3%). The neutron yield is measured using the associated alpha particle method. The experimental results are given in Table 3. Nuclear heating was measured at 14.99 cm, 30.23 cm, 45.47 cm and 60.71 cm depth from the block surface using high sensitivity GR-200 (LiF:Mg,Cu,P) thermoluminescent dosimeters (TLD). Since the TLD technique is a relative method, TLDs were calibrated against a Co-60 g-ray source. The calibration uncertainty was within ±5%. The calibration was performed using a secondary standard. Four TLDs were located in each experimental position and the averaged values of the measured TL light was used as experimental data. From this datum, after conversion via the calibration factor, the experimental total dose in TLDs was obtained. The total uncertainty is ±7%. This uncertainty includes the above mentioned calibration error, the error (standard deviation) on the averaged TL light value, the uncertainty on the FNG neutron yield (±3%), summed using the quadratic law. The experimental results are given in Table 4. 5. Description of Results and Analysis: ----------------------------------- The experimental results (E) were analysed by the Monte Carlo code MCNP-4C [6] using point-wise cross sections derived from FENDL-2.0 [7], EFF-2.4 and also with the new evaluation for 28Si included in EFF-3.0. The calculations are presented in [1] and [2]. Activation reaction rates where calculated using tally f4 of MCNP, the dosimetric reactions needed for the calculation were taken from IRDF-90.2 library [8] (mcnp.inp). The calculated reaction rates (C) are given in Table 5 together with the statistical uncertainty. The gamma dose Dg and the neutron dose Dn in TLDs was calculated with tally f6 of MCNP, using a very detailed model in MCNP of the dosimeters and of their plastic containers (mcnp_tld.inp). The dose in TLD was obtained from: DTLD = Kn*Dn + Dg where Kn is neutron sensitivity of the TL detector to neutrons and is usually depending upon the neutron energy. The Kn data were taken from [9] and were then weighted over the calculated neutron spectra at each experimental position. The resulting Kn values are reported in Table 7. Comparison between the measured dose in TLD and the same quantity calculated with EFF-2.4, EFF-3.0 and FENDL-2.0 nuclear data is also given in Tab. 7. The transport and cross section sensitivity/uncertainty analyses were also performed using the deterministic codes DORT, TWODANT and SUSD3D, and are presented in [3] and [4]. Analytic uncollided and first collision source approach was used in order to mitigate the ray effects. Input data for the following codes are included: - TRANSX (cross section preparation), - GRTUNCL and DORT (uncollided/first collision source and discrete ordinates (SN) transport calculation) - TWODANT (SN neutron transport using first collision approach). 6. Special Features: ---------------- None 7. Author/Organizer: ---------------- Experiment and analysis: P. Batistoni, M. Angelone, M. Pillon, L. Petrizzi ENEA Centro Ricerche Energie Frascati UTS Fusione Via E. Fermi 27 C.P. 65 I-00044 Frascati (Rome) Italy Compiler of data for Sinbad: P. Batistoni ENEA Centro Ricerche Energie Frascati UTS Fusione Via E. Fermi 27 C.P. 65 I-00044 Frascati (Rome) Italy E-mail: batiston at efr406.frascati.enea.it Reviewer of compiled data: I. Kodeli OECD/NEA, 12 bd des Iles, 92130 Issy les Moulineaux, France e-mail: ivo.kodeli at oecd.org Acknowledgement --------------- The experiment and the corresponding analysis was performed in the framework of the EFDA (European Fusion Development Agreement) Task (TTMN-002-2001). 8. Availability: ------------ Unrestricted 9. References: ---------- [1] P. Batistoni, M. Angelone, L. Petrizzi, M. Pillon, Measurements and Analysis of Reaction Rates and of Nuclear Heating in SiC, Dec. 2001 [2] M. Angelone, P. Batistoni, I. Kodeli, L. Petrizzi, M. Pillon, “Benchmark analysis of neutronics performances of a SiC block irradiated with 14 Mev neutrons”, Fus. Eng. Design 63-64 (2002) 475 [3] Y. Chen, U. Fischer, I. Kodeli, R. L. Perel, M. Angelone, P. Batistoni, L. Petrizzi, K. Seidel, S. Unholzer, “Sensitivity and uncertainty analyses of 14 Mev neutron benchmark experiment on Silicon Carbide”, 22nd Symposium on Fusion Technology, Helsinki, Finland, 9-13 Sept 2002. [4] I. Kodeli, Deterministic Transport, Sensitivity and Uncertainty Analysis of SiC Benchmark Experiment Using EFF-3 and FENDL-2 Evaluations, EFFDOC-818, Dec. 2001. [5] M. Martone, M. Angelone, M. Pillon, The 14 MeV Frascati Neutron Generator, Journal of Nuclear Materials 212-215 (1994) 1661-1664; [6] Briesmeister, J. F. (Ed.), MCNP - A general Monte Carlo n-particle transport code, version 4C, Report LA12625, Los Alamos, September 1999. [7] M. Herman, A. B. Pashchenko, Extension and improvement of the FENDL library for fusion applications (FENDL-2), Report INDC(NDS)-373, IAEA Vienna, 1997. [8] N. P. Kocherov, P. K. McLaughlin, The International Reactor Dosimetry File (IRDF-90), Report IAEA-NDS-141, Rev. 2, Oct. 1993. [9] J.A. Gibson, The relative tissue-kerma sensitivity of thermoluminescent materials to neutrons, Report EUR 10105 EN (1985) 10. Data and Format: --------------- FILE NAME bytes Content ---- ------------ ------ ------- 1 fngsic-a.htm 12,207 This information file 2 fngsic-e.htm 30,979 Description of Experiment 3 source.for 45,178 FORTRAN subroutine for MCNP source description 4 mcnp.inp 47,410 3-D model for MCNP-4A calculations of neutron activation reaction rates 5 mcnp_tld.inp 53,655 3-D model for MCNP-4A calculations of nuclear heating 6 trx-sic.inp 522 Input data for TRANSX cross-section preparation 7 dort-sic.inp 8,085 Input data for GRTUNCL first collision source and DORT transport codes 8 2dant-si.inp 6,478 Input data for TWODANT transport code 9 fig1.gif 5,242 Fig. 1: Angular dependence of the source 10 fig2.gif 9,505 Fig. 2: Energy/angular dependence of the source 11 fig3.gif 64,368 Fig. 3: Geometry of the experimental mock-up 12 fig4.gif 9,633 Fig. 4: Geometry of the source 13 fig5.gif 5,165 Fig. 5: Geometry of TLD detector 14 enea-sic.pdf 904,911 Reference 1 15 fed2002.pdf 282,929 Reference 2 16 soft-22.pdf 236,191 Reference 3 17 eff-818.pdf 605,072 Reference 4 File fngsic-e.htm contains the following tables: Tab. 1: Angular dependence of the source Tab. 2: Angular/energy dependence of the source energy distribution Tab. 3: Measured neutron reaction rates Tab. 4: Measured absorbed dose in TLD Tab. 5: Calculated reaction rates Tab. 6: Comparison between calculated (C) and measured (E) reaction rates - C/E ratios Tab. 7: Calculated absorbed dose in TLD - C/E ratios The figures are included in gif format. SINBAD Benchmark Generation Date: 4/2003 SINBAD Benchmark Last Update: 4/2003