SINBAD ABSTRACT NEA-1517/83
Baikal-1 Skyshine Benchmark Experiment
1. Name of Experiment: ------------------ Measurements of spatial energy distributions of neutrons and photons scattered in the air near the ground-air interface (skyshine-experiment) (1996-1998). 2. Purpose and Phenomena Tested: ---------------------------- Detailed studying of the spatial energy distributions of neutrons and photons scattered in the air near the ground-air interface for generation of a database (of experimental and analytical nature) to verify the computer codes that are used for justification of the radiation and ecological safety of population residing in direct proximity to nuclear power plants. 3. Description of the Source and Experimental Configuration: -------------------------------------------------------- The experimental studies were carried out at the research RA reactor incorporated in the "Baikal-1" unique complex of research reactors near Semipalatinsk, belonging to Kurchatov Institute of Atomic Energy in the Kazakhstan National Nuclear Centre (IAE NNC RK), being constructed in thinly populated steppe area. The altitude differences in the region of measurements (0.0 - 1500 m from the source) never exceed ±5 m. The distance from the nearest residential settlements was at least 60 km. The vegetative cover is purely grass; its height doesn't exceed 20-30 cm above the soil layer. The core of the RA research reactor was the source of neutron and photon radiation; the core was 700 mm high and 297 mm in diameter comprising 37 air-cooled fuel assemblies with highly enriched fuel made of uranium carbide. A zirconium hydride cylinder 339 mm in diameter was used as a moderator. There were 372 holes (3 mm in diameter) bored in it for cooling. Lateral reactor side shielding consisted of the beryllium reflector 102 mm thick, the 16 mm steel vessel and additional graphite reflector 180 mm thick. Biological shielding made of heavy serpentinite concrete, 1100-1400 mm thick, was arranged around the core and reflectors; from outside the shielding was surrounded with a steel bell-shaped structure, about 350 mm thick. In the upper direction the shielding consisted of a steel plate (reactor cover) ~ 120 mm thick, and a concrete block (shielding plug) – its thickness was about 850 mm immediately above the reactor. This block was removed during the experiments to ensure release of highly intensive fluxes of neutron and photon radiation to the air. The measurements which were made close to the reactor on the outer surface of biological shielding at the levels of ground surface and 1-2 m above it showed that reactor radiation is completely released to the air uprightly, and there was no reactor-caused radiation that directly reached the detectors as line-of-sight beams. During the experiment the spatial detection points were located at the height of 1.0 m above the ground at a distance from 50 to 1500 m from the reactor axis. Reactor power during measurements was 300 kW. 4. Measurement System and Uncertainties: ------------------------------------ Measurements of neutron energy spectra were conducted within the wide range of energy (30 keV - 10 MeV) applying the following sets of spectrometric instruments: • 1H-spectrometer with a cylindrical counter (Ø32×150 mm), its energy range is 30 - 400 keV; the measurement error is ±(20 - 30)%. • 3He-spectrometer with a cylindrical counter (Ø32×150 mm), its energy range is 0.05 - 2.5 MeV; the measurement error within the range of energy higher 1 MeV is ±(15 - 20)%, and it doesn't exceed ±(10-15)% for the range of 0.1 - 1 MeV; • scintillation spectrometer of fast neutrons with a stilbene crystal (Ø40×40 mm) and the energy range of measurements is 0.8 - 10 MeV; the measurement error is ±(10 - 15)% for the range of 1-3 MeV, and ±(15 - 20)% - if the energy is higher that 3 MeV; • multisphere spectrometer with a set of 6 spheres, their diameters varying from 51 to 305 mm. The spectrometer features a high sensitivity and ability to measure in the energy range of 1 eV - 10 MeV. The photons energy spectra were measured by: • scintillation gamma-spectrometer with a stilbene crystal (Ø40×40 mm) in 0.1 - 10 MeV energy range; the measurement error within the range of energy of 0.1 - 2.0 MeV is ±(15 - 20)%, and it increases up to ±(30 - 40)% for the energy higher than 2.0 MeV. The neutron fluxes were measured by: • MKS-01R radiometer-dosimeter with the BDKN-03R detection unit and two polyethylene spheres have 240 and 150 mm in diameter; the measurement error doesn't exceed ±20%. • scintillation fast neutron counter with pellet of ZnS(Ag) + organic glass detector (Ø80×6 mm); the measurement error for fast neutron flux is ±(15-20)%; • scintillation thermal neutron counter with ZnS(Ag) + boron detector (Ø40×200 mm); the measurement error is ±(20-30)%. For the photon dose rates the following instruments were used: • MKS-01R radiometer-dosimeter with the BDKG-02R detection unit and tissue-equivalent scintillator (Ø25×25 mm) and DBG-01-N, DRG-01T dosimeters; the measurement error doesn't exceed ±(20 - 30)%. • a set of the IKS-A type thermoluminescent dosimeters based on the aluminophosphate glass, the energy range is 0.5 - 1000 rad. The measurement error within the photon energy range of 30 keV to 6.1 MeV does not exceed ±20%. Sets of threshold and resonance detectors were used to measure the reaction rates and unfolding of neutron spectra near the core; the energy range is 0.1 eV - 10 MeV, and total error of measurements does not exceed ±30%. 5. Description of Results and Analysis: ----------------------------------- Basic parameters of neutron and photon radiation released to the atmosphere were measured during 1996-1997 in several series of experimental studies at the RA reactor: • Fast and thermal neutron fluxes, dose rates of neutron and photon radiation at various altitudes from the reactor cover; • Spatial differential energy distributions of neutrons at various distances from the reactor axis (100, 200, 400, 500, 600, 800, 1000 m); • Spatial distribution of neutron radiation dose rate at 50 from 1500 m; • Energy distribution of photon radiation fluxes and photon dose rates at various distances off the reactor. In addition • Influence of weather conditions and soil composition on radiation field characteristics has been studied; • It has been demonstrated that neutron radiation makes the major input to the total dose rate in the vicinity of the reactor; • It has been showed that for the case of long distances from the reactor the photons emerging as a result of thermal neutrons radiation capture in the soil, give a major contribution into photon dose rate in comparison to the photons emerging as a result of inelastic scattering of neutrons in the air. 6. Special Features: ---------------- 1. The work was accomplished during the years of 1996-1998 within the project # 517 of the International Scientific and Technical Centre under the contract with Japan Ministry of Foreign Affairs; 2. As the result of work the set of experimental and computed data which provided detailed description of radiation situation both around the reactor and the regularities in radiation fields formation stipulated by scattering of reactor-caused radiation in the air, ground reflection and emerging of photons due to neutrons radiation capture in the soil under different weather conditions has been received; 3. At all stages of work analytical estimation of data using the codes and methods of high accuracy (Monte-Carlo method, method of discrete ordinates) was carried out. 7. Author/Organizer ---------------- Experiment: Yu.V.Orlov, V.N.Avaev, G.A.Vasiljev, N.N.Soukharev, A.I.Yashnikov (FSUE RDIPE, P.O. Box 788, Moscow, 101000, Russia) Analysis: M.E.Netecha, O.F.Dikareva, V.P.Zharkov, I.A.Kartashev (FSUE RDIPE, P.O. Box 788, Moscow, 101000, Russia) Compiler of data for SINBAD: M.E.Netecha, O.F.Dikareva, V.P.Zharkov, I.A.Kartashev (FSUE RDIPE, P.O. Box 788, Moscow, 101000, Russia) Evaluators for ICSBEP: O. F. Dikareva, I. A. Kartashev, M. E. Netecha, V. P. Zharkov Research Development Institute of Power Engineering Reviewer of SINBAD compiled data: I. Kodeli OECD/NEA, 12 bd des Iles, 92130 Issy les Moulineaux, France ICSBEP Internal Reviewer: A. P. Vasiliev ICSBEP Independent Reviewers Dale Hankins, USA Virginia Dean, USA International Criticality Safety Benchmark Evaluation Project (ICSBEP) 8. Availability: ------------ Unrestricted 9. References: ---------- [1] I.I. Deryavko, V.S. Zhdanov, I.G. Perepelkin, Yu.S. Cherepnin, Radiating stability of carbide materials at an irradiation in the reactor with low neutron fluxes. VANT, ser. Physics of radiating damages and radiating materiology. Kharkov, v. 1, ð.48, 1992 [2] Zh.R. Zhotabaev, D.I. Zelensky, Î.S. Pivovarov, V.P. Smetannikov, Yu.S. Cherepnin. Possibilities of the experimental base of Kazakhstan for tests of elements of space nuclear reactors. Bulletin NNC RK, "Nuclear engineering and safety of the nuclear power station", v.1, ð.7, 2000 [3] Sc.T. Tuhvatulin, I.L. Tazhibaeva, V.P. Smetannikov, V.P. Pavshuk, N.N. Ponomarev-Stepnoj, I.I. Fedik, Yu.S. Cherepnin. Reactor complexes of the National nuclear center of Republic Kazakhstan. Proc. of the International conference "Experience of Designing of nuclear reactors", Moscow, 2002 [4] MCNP - A General Monte-Carlo N-Particle Transport Code, Version 4B, LA-12625-M (March 1997) [5] S. Berg. Modification of SAND-2. BNWL-855, 1968 [6] I.A. Bochvar, T.I. Imadova et al. Method of IKS Dosimetry, M., Atomizdat, 1977 [7] MKS-01R Radiometer-Dosimeter. Certificate Zh1P.289.201PS [8] V.N. Avaev, G.A. Vasiliev et al. Experimental Studies of Gamma and Neutron Radiation Fields. Edited by Yu.A. Egorov, M., Atomizdat, 1974 [9] R.L. Bramlett, R.I. Ewing, T.W. Bonner. A New Type of Neutron Spectrometer. Nucl. Instr. and Meth., 1960, v. 9, n.1, p. 1 [10] R.H. Johnson, B.W. Wehring, J.J. Dorning. Nucl. Sci.Eng., v.73, 1980, p.93 [11] R.V. Hemming, Numerical Methods. Nauka, M., 1968 [12] L.Z. Rumshinsky. Mathematical Processing of Experimental Results, M., Nauka, 1971 [13] R.D. Vasiliev et al. Method of Reaction Rate Calculation and Its Errors. In collection: Metrology of Neutron Measurements at Nuclear-Physical Facilities. M., Atominform, 1976 [14] A.A. Gui, J.K. Shultis, R.E. Fow. Response Functions for Neutron Skyshine Analysis. Nucl. Sci. Eng., 1997, v. 125, No. 2, p.111-127 [15] W.A. Rhoades, R.L. Childs. The DORT Two-dimensional Discrete Ordinates Transport Code. Nucl.Sci.Eng. 99, 1, 88-89 (May 1988) [16] RSIC library DLC-23/CASK. 40-Group coupled neutron and gamma-ray cross-section data, 1973 [17] Zharkov V.P., Dikareva O.F., Kartashev I.A., Kiselev A.N., Netecha M.E., Sakamoto H., Nomura Y., Naito Y., Analytical Study of Reactor Radiation Scattering in the Atmosphere, Proc. of ANS conference "Technologies for the New Century", Tennessee, Nashville, USA, April 1998 [18] Yu.V. Orlov, M.E. Netecha, V.N. Avaev, G.A. Vasiljev, Yu.L. Istomin, D.I. Zelensky, Yu.S. Cherepnin, H. Sakamoto, Y. Nomura, Y. Naito, Neutron and Gamma-Radiation Skyshine Experiment at Nuclear Reactor, Proc. of ANS conference "Technologies for the New Century", Tennessee, Nashville, USA, April 1998 [19] M.E. Netecha, O.F. Dikareva, V.P. Zharkov, I.A. Kartashev, Compilation of the series of measurements of spatial energy distributions of neutrons and photons scattered in the air near the ground-air interface in standard SINBAD Database format, Final Report, Federal Agency for Atomic Energy, Federal State Unitary Enterprise, Research and Development Institute of Power Engineering, Moscow 2005. [20] Final Report on ISTC Project No. 517-96: Experimental study of reactor radiation scattering in the atmosphere (for a period of 24 months from September 1, 1996 to August 31, 1998), Mikhail E. Netecha, (Project Manager), Research and Development Institute of Power Engineering, September, 1998 [21] "BAIKAL-1 SKYSHINE EXPERIMENT" ICSBEP evaluated version September 2009 (NEA/NSC/DOC/(95)03/VIII Volume VIII) 10. Data and Format: --------------- DETAILED FILE DESCRIPTIONS -------------------------- Filename Size[bytes] Content --------------- ----------- ------------- 1 sks_a.htm 22.140 This information file 2 sks_e.htm 64.742 Description of Experiment 3 sks-f1.gif 61.675 Fig. 1: Schematic diagram of the RA reactor 4 sks_f2.gif 72.122 Fig. 2: Detailed diagram of the RA reactor core 1) Radial cross section of the fuel assembly; 2) Radial cross section of the some part of RA core with the steel vessel and reflector; 3) RA core and its vicinity. Material zone numbers are taken in the Tables 1-2. 5 sks_f3.gif 68.093 Fig. 3: Detailed model of the experiment 6 sks_f4.gif 9.055 Fig. 4: "Simplified" model of the experiment 7 table1.htm 7.494 Table 1: Material composition of zones. 8 table2.htm 2.421 Table 2: Meteorological data and nuclear concentrations of atmospheric air elements at the period of on-site measurements 9 table3.htm 2.678 Table 3: Characteristics of threshold detectors 10 table4.htm 3.121 Table 4: Characteristics of resonance detectors 11 table5.htm 4.636 Table 5: Characteristics of detectors used for on-site measurements 12 table6.htm 12.001 Table 6: Radial distribution of 115In(n,n') reaction rates, thermal neutron fluxes and photons dose rates at various altitudes from the reactor cover 13 table7.htm 31.555 Table 7: Neutron spectrum measured by foils activation for the RA reactor 14 table8.htm 5.647 Table 8: Neutron dose rates measured at the RA reactor 15 table9.htm 5.706 Table 9: Photon radiation dose rate measured at the RA reactor 16 table10.htm 5.708 Table 10: Thermal neutron fluxes measured at the RA reactor 17 table11.htm 5.739 Table 11: Intermediate and fast neutrons fluxes measured at the RA reactor 18 table12.htm 7.542 Table 12: Relative count rates of spherical moderators at various distances from the RA reactor 19 table13.htm 71.785 Table 13: Differential neutron spectra, measured by scintillation spectrometer with a stilbene crystal at different distances from the RA reactor 20 table14.htm 70.286 Table 14: Differential photons spectra measured by scintillation spectrometer with a stilbene crystal at different distances from the RA reactor 21 table15.htm 16.636 Table 15: Comparison of computed (MCNP) and experiment-determined (Exp.) functionals of the radiation fields near the RA reactor core 22 table16.htm 6.566 Table 16: Normalized neutron and photon energy distributions for "effective" sources 23 table17.htm 6.114 Table 17: Spatial distribution of neutron and photon dose rates, total neutron flux and thermal neutron flux for the cases with and without ground presence 24 table18.htm 6.427 Table 18: Comparison of computed and experiment-determined values of neutron dose rate measured at the RA reactor 25 table19.htm 5.089 Table 19: Comparison of computed and experiment-determined values of photon radiation dose rate measured at the RA 26 table20.htm 6.424 Table 20: Comparison of computed and experiment-determined values of thermal neutron fluxes measured at the RA reactor 27 table21.htm 5.127 Table 21: Comparison of computed and experiment-determined values of intermediate and fast neutron fluxes, measured at the RA reactor 28 table22.htm 8.130 Table 22: Relative counting rate of spherical moderators at various distances from the RA reactor 29 table23.htm 9.904 Table 23: Energy dependence of sphere effectiveness for multisphere spectrometer 30 table24.htm 2.232 Table 24: Counting rates of multisphere moderators for 252Cf source 31 table25.htm 9.955 Table 25: Comparison of neutron differential spectra calculated by the MCNP code, with experimental data 32 table26.htm 9.551 Table 26: Comparison of photon differential spectra calculated by the MCNP code, with the experimental data 33 sk_eranp.mcnp 26.848 Input file for MCNP, neutron + secondary photon transport 34 sk_erapp.mcnp 17.209 Input file for MCNP, primarily photon transport 35-48 im01.jpg - im15.jpg Corresponding formulae 49 skycal.pdf 149.262 Ref. [17]: Report on ANS conference, Tennessee, April 1998 50 skyexp.pdf 252.948 Ref. [18]: Report on ANS conference, Tennessee, April 1998 51 skyshine_rep.pdf 1,709,413 Ref. [19] by M.E. Netecha, et al., Compilation of the series of Measurements of spatial energy distributions of neutrons and photons scattered in the air near the ground-air interface in standard SINBAD Database format. 52 517_report.pdf 1,218,021 Ref. [20]: M.E. Netecha, Final Report on ISTC Project No. 517-96, (1998) 53 Rearsk01.pdf 1,743,437 Ref. [21]: Recommended evaluation of the benchmark (September 2009) Figures are stored in GIF format. SINBAD Benchmark Generation Date: 6/2006 SINBAD Benchmark Last Update: 9/2009