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90-Th-232 MINSK EVAL-JUN01 V.M. Maslov et al. DIST-JAN09 20090105 ----JEFF-311 MATERIAL 9040 -----INCIDENT NEUTRON DATA ------ENDF-6 FORMAT *************************** JEFF-3.1.1 ************************* ** ** ** Original data taken from: JEFF-3.1 ** ** ** ****************************************************************** ***************************** JEFF-3.1 ************************* Original data taken from: ENDF/B-VI.8 + New eval. New evaluation: Maslov, Minsk. MF=12-15 from ENDF/B-VI.8 MT=458(ENERGY RELEASE IN FISSION) evaluation from ENDF/B-VI.4 05-01 NEA/OECD (Rugama) 8 delayed neutron groups Jefdoc-976(Spriggs,Campbel and Piksaikin,Prg Nucl Eng 41,223(2002) ----B-404-ISTC MATERIAL 9040 -----INCIDENT NEUTRON DATA -----ENDF/B-VI FORMAT ***************************************************************** UNRESOLVED RESONANCE PARAMETERS FOR 4-150 KEV REGION, TOTAL, ELASTIC SCATTERING, INELASTIC SCATTERING, FISSION, CAPTURE,(N,2N), (N,3N) AND (N,4N) CROSS SECTIONS AS WELL AS ANGULAR AND ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS WERE EVALUATED BY V.M. MASLOV, Yu.V. PORODZINSKIJ, M. BABA, A. HASEGAWA, N.V. KORNILOV, A.B. KAGALENKO AND N.A. TETEREVA/1/. MF=1 GENERAL INFORMATION MT=451 DESCRIPTIVE DATA AND DIRECTORY RECORDS MT=452 NUMBER OF NEUTRONS PER FISSION SUM OF MT'S= 455 AND 456 MT=455 DELAYED NEUTRON DATA TAKEN FROM REF./2/. MT=456 NUMBER OF PROMPT NEUTRONS PER FISSION CALCULATED WITH THE EMISSIVE FISSION MODEL TO FIT MEASURED DATA /3-9/, BUT BASICALLY DATA BY FREHAUT ET AL./5/ AND HOWE /9/, IRREGULARITY AROUND(n,nf) REACTION THRESHOLD IS REPRODUCED. MF=2 RESONANCE PARAMETERS MT=151 RESOLVED AND UNRESOLVED RESONANCE PARAMETERS (RESOLVED RESONANCE REGION = 1.0E-5 EV TO 4 KEV), (UNRESOLVED RESONANCE REGION = 4 KEV TO 150 KEV) 1) RESOLVED RESONANCE PARAMETERS (Breit-Wigner)WERE ADOPT FROM ENDF/B-VI AS EVALUATED BY OLSEN /10/. 2) ENERGY-DEPENDENT UNRESOLVED RESONANCE PARAMETERS COVER ENERGY RANGE FROM 4.0 TO 150 KEV. PARAMETERS WERE OBTAINE TO REPRODUCE SMOOTH TOTAL AND CAPTURE CROSS SECTIONS, CALCULATED WITH STATISTICAL MODEL. ENDF/B PROCESSING CODES /11,12/ IGNORE DIRECT INELASTIC SCATTERING. TO COMPENSATE THAT DEFICIENCY WE INCREASED AVERAGE INELASTIC SCATTERING WIDTHS, CAPTURE WIDTHS ABOVE 50 KEV ALSO WAS SLIGHTLY INCREASED TO KEEP CAPTURE CROSS SECTION UNDISTORTED AS COMPARED WITH CALCULATED BY PHYSICALLY CORRECT CODES (PCC). CALCULATED WITH PCC CODES CROSS SECTIONS FIT MEASURED DATA ON TOTAL, CAPTURE AND INELASTI SCATTERING. AS A RESULT, TOTAL,ELASTIC SCATTERING AND CAPTURE CROSS SECTIONS, CALCULATED WITH THESE PCC CODES, ARE REPRODUCED WITH CONVENTIONAL ENDF PROCESSING CODES USING AVERAGE RESONANCE PARAMETERS GIVEN IN MF=2 MT=151. 2200-M/S CROSS SECTIONS AND CALCULATED RESONANCE INTEGRALS. 2200 M/S(B) RES. INTEG.(B) TOTAL 12.077 ELASTIC 9.360 FISSION 11.8E-06 1.72 CAPTURE 2.717 277 MF=3 NEUTRON CROSS SECTIONS BELOW 4 KEV, BACKGROUND CROSS SECTIONS WERE GIVEN FOR TOTAL CROSS SECTION ONLY. ABOVE 4 KEV UP TO 150 KEV EVALUATED CROSS SECTIONS WERE REPRESENTED WITH THE UNRESOLVED RESONANCE PARAMETERS. MT= 1, 2, 4, 51-81, 91 - TOTAL, ELASTIC AND INELASTIC SCATTERING CROSS SECTIONS. TOTAL, ELASTIC AND DIRECT INELASTIC FOR ROTATIONAL GROUND STATE BAND LEVELS MT=51,52,53,54 (COUPLED LEVELS) AS WELL AS OPTICAL TRANSMISSION COEFFICIENTS ARE OBTAINED IN A RIGID ROTATOR MODEL COUPLED CHANNELS CALCULATIONS. DIRECT EXCITATION OF VIBRATIONAL, OCTUPOLE AND K=2+ QUADRUPOL BAND LEVELS,MT=55,56,57,58,59,61,62,63,64,65,66,67,68,72,75, 78,79, ARE OBTAINED IN A SOFT ROTATOR MODEL COUPLED CHANNEL CALCULATIONS, FOR NORMALIZATION PURPOSES THESE DIRECT INELASTIC CROSS SECTIONS WERE SUBTRACTED FROM MT=2 ELASTIC SCATTERING CROSS SECTION. DIRECT INELASTIC CONTRIBUTIONS WERE ADDED INCOHERENTLY TO HAUSER-FESHBACH CALCULATIONS OF COMPOUND NUCLEUS INELASTIC SCATTERING CROSS SECTIONS. THE DEFORMED OPTICAL POTENTIAL USED: ENERGY DEPENDENCE OF VR AND WD VARIED TO FIT MEASURED TOTAL DATA /13-19/, ELASTIC SCATTERING DATA /20-22/ AND EVALUATED VALUE OF S0=(.94+-.02)x10-4(EV)-1/2 VR=(45.722-0.334xE) MEV; RR =1.2668 FM; AR =.6468 FM; WD=(3.145+0.455xE)MEV; E< 8 MEV RD =1.25 FM; WD= 6.785 MEV; E>= 8 MEV AD =.5246 FM; VSO= 6.2 MEV; RS0=1.12 FM; ASO=.47 FM; B2= .188; B4=.071; FISSION, CAPTURE AND COMPOUND INELASTIC SCATTERING CROSS SECTIONS WERE CALCULATED WITH HAUSER-FESHBACH-MOLDAUER/23/ APPROACH, AT INCIDENT NEUTRON ENERGIES HIGHER THAN 1.21 MEV (LEVEL OVERLAPPING ENERGY) TEPEL ET AL./24/ THEORY WAS EMPLOYED. MEASURED DATA ON DISCRETE LEVEL EXCITATION CROSS SECTIONS /25-31/, GROUPS OF LEVELS OF VIBRATIONAL, OCTUPOLE AND K=2+ BAND LEVELS /27/ AS WELL AS TOTAL INELASTIC CROSS SECTION /29-31/ WERE TAKEN INTO ACCOUNT. ADOPTED LEVEL SCHEME OF Th-232 FROM NUCLEAR DATA SHEETS /32/. LEVEL SCHEME: -------------------------------------------------------- NO. ENERGY(MEV) SPIN-PARITY K-PARITY -------------------------------------------------------- G.S. 0.0 0 + 0+ 0.4936900-01 2 + 0+ 0.1621200+00 4 + 0+ 0.3332000+00 6 + 0+ 0.5569000+00 8 + 0+ 0.7142500+00 1 - 0- 0.7303500+00 0 + 0+ 0.7741000+00 2 + 0+ 0.7744000+00 3 - 0- 0.7853000+00 2 + 2+ 0.8270000+00 10 + 0+ 0.8296000+00 3 + 2+ 0.8730000+00 4 + 2+ 0.8836000+00 5 - 0- 0.8901000+00 4 + 0+ 0.9604000+00 5 + 2+ 0.1023100+01 6 + 2+ 0.1042900+01 7 - 0- 0.1049900+01 6 + 0+ 0.1053600+01 2 + 0.1072900+01 2 + 0.1077500+01 1 - 0.1078700+01 0 + 0+ 0.1094400+01 3 + 0.1105700+01 3 - 0.1121800+01 2 + 0+ 0.1137100+01 12 + 0.1143300+01 4 - 0.1146000+01 7 + 0.1148300+01 4 + 0+ 0.1182500+01 3 - 0.1208900+01 5 - OVERLAPPING LEVELS ARE ASSUMED ABOVE 1.21 MEV MT=16,17,37. (N,2N), (N,3N) AND (N,4N) CROSS SECTION FROM STATISTICAL MODEL CALCULATIONS /1/ WITH THE ACCOUNT OF PRE-EQUILIBRIUM NEUTRON EMISSION (MODIFIED STAPRE CODE/33/ WAS USED). MEASURED (N,2N) DATA /34-46/ WERE CONSISTENTLY REPRODUCED, WHILE CALCULATED FISSION CROSS SECTION, WHICH DESCRIBES MEASURED DATA BASE, WAS USED AS MAJOR CONSTRAINT. MT=18, 19, 20, 21. FISSION CROSS SECTION IS CALCULATED WITHIN STATISTICAL MODEL /1/. FOR FISSION DATA ANALYSIS MEASURED DATA /47-51/ WERE USED. THE CONTRIBUTION OF EMISSIVE FISSION TO THE TOTAL FISSION CROSS SECTION IS FIXED ACCORDING TO CONSISTENT DESCRIPTION OF(N,F) AND (N,XN) REACTION DATA MT=102 CAPTURE CAPTURE CROSS SECTION DATA /52-55/ ARE DESCRIBED WITHIN A STATISTICAL MODEL. ABOVE NEUTRON ENERGY 5 MEV CAPTURE IS ASSUMED TO BE CONSTANT. COMPETITION OF (N,GF) AND (N,GN') REACTIONS IS TAKEN INTO ACCOUNT. RADIATIVE STRENGTH FUNCTION SGO = 0.XXX WAS ADJUSTED TO FIT CAPTURE CROSS SECTION DATA ABOVE 4 KEV. CAPTURE CROSS SECTION DATA AT HIGHER ENERGIES WERE DESCRIBED VARYING LEVEL DENSITY OF 233-Th COMPOUND NUCLIDE. MF=4 ANGULAR DISTRIBUTIONS OF SECONDARY NEUTRONS FOR MT=2,51,52,53 AND 54 FROM COUPLED CHANNEL CALCULATIONS (RIGID ROTATOR MODEL), FOR MT=55,56,57,58,59,61,62,63,64,65,66,67,68,72,75, 78,79, FROM COUPLED CHANNEL MODEL (SOFT ROTATOR MODEL) WITH ADDED ISOTROPIC STATISTICAL CONTRIBUTION. MT=16, 17, 18-21, 37,38, 60, 69-71,73,76,77,80,81 AND 91 ARE ISOTROPIC IN THE LAB SYSTEM. MF=5 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS ENERGY DISTRIBUTIONS FOR MT=16,17,38,91 WERE CALCULATED BY STATISTICAL MODEL OF CASCADE NEUTRON EMISSION TAKING INTO ACCOUNT THE HISTORY OF THE DECAY WITH THE ALLOWANCE OF PRE- EQUILIBRIUM EMISSION OF THE FIRST NEUTRON. MEASURED NEUTRON EMISSION SPECTRA DATA BY BABA ET AL./56,57/ ARE REPRODUCED. MT=18,19,20,21,37 PROMPT FISSION NEUTRON SPECTRA (PFNS)WERE CALCULATED WITH THE SEMI-EMPIRICAL MODEL/1/, PRE-FISSION NEUTRON EMISSION IN (N,XNF) REACTION, EITHER EQUILIBRIUM AND PRE-EQUILIBRIUM MODES ARE INCLUDED. BASICALLY PFNS FROM FISSION FRAGMENTS (FF) WERE CALCULATED AS A SUPERPOSITION OF TWO WATT DISTRIBUTIONS FOR LIGHT AND HEAVY FF WITH EQUAL CONTRIBUTIONS, BUT DIFFERENT TEMPERATURE PARAMETERS. FF KINETIC ENERGY, ONE MORE MODEL PARAMETER, MIGHT BE LOWER THAN TKE, WHICH REFLECTS IT'S DEPENDENS ON THE MOMENT OF NEUTRON EMISSION. THIS EFFECTIVELY REDUCES AVERAGE ENERGY OF PFNS FOR INCIDENT NEUTRON ENERGIES ABOVE EMISSIVE FISSION THRESHOLD. DATA ON PFNS OF /58-62/ ARE FITTED. ************************************************************** MF=12-15 is from ENDFB-VI.7 evaluation (OECD/NEA Data Bank, Rugama) ************************************************************** MF = 12 MT = 18 FOR ALL INCIDENT ENERGIES THE MULTIPLICITY OF PHOTONS FROM FISSION WAS DERIVED FROM THE DATA OF REF. 63 WHICH REPORTED THE PHOTON SPECTRUM AND TOTAL PHOTON ENERGY FOR THERMAL FISSION OF U-235. IT WAS ASSUMED THAT THE MULTIPLICITY IS INDEPENDENT OF INCIDENT NEUTRON ENERGY. MT = 102 FOR ALL INCIDENT NEUTRON ENERGIES PHOTON PRODUCTION FROM NEUTRON CAPTURE IS REPRESENTED BY AN ENERGY DEPENDENT MULTIPLI- CITY TO BE APPLIED TO THE (N,GAMMA) CROSS SECTION AND BY AN ENERGY INDEPENDENT SPECTRUM. THE SPECTRUM USED WAS BASED ON AN UNDOCUMENTED MEASURED SPECTRUM FOR U-238 WITH A MINOR ADJUSTMENT FOR SMALL Q-VALUE DIFFERENCE BETWEEN TH-232 AND U-238. THE AVERAGE ENERGY OF TE ASSUMED SPECTRUM WAS THEN DIVIDED INTO THE Q-VALUE TO OBTAIN A MULTIPLICITY AT ZERO NEUTRON ENERGY. THE MULTIPLICITY AT 20 MEV WAS OBTAINED (REF 64) BY USE OF THE FORMULA M(E) = M0(EN+Q)/Q WHERE M0 IS THE MULTIPLICITY AT ZERO NEUTRON ENERGY AS DESCRIBED ABOVE. MF = 13 MT = 3 EXPLICIT REPRESENTATION OF THREE PHOTONS (.04971, .1632 AND .3344 MEV) FROM INELASTIC SCATTERING WAS DERIVED FROM FILE 3 DATA AND KNOWN BRANCHING RATIOS. FOR INCIDENT NEUTRON ENERGIES GT .7251 MEV THE METHOD OF REF. 36 WAS USED TO CALCULATE PHOTON PRODUCTION CROSS SECTIONS AND SPECTRA FROM ALL REACTIONS EXCEPT PHOTONS FROM THE FIRST THREE INELASTIC GROUPS, NEUTRON CAPTURE AND NEUTRON-INDUCED FISSION. MF = 14 MT = 3,18,102 ALL PHOTONS WERE ASSUMED TO BE ISOTROPIC MF = 15 MT = 3 PHOTON SPECTRA WERE OBTAINED USING THE METHOD OF REF. 65. MT = 18 THE MEASURED PHOTON SPECTRUM OF REF. 63 WAS USED FOR ALL INCIDENT NEUTRON ENERGIES BECAUSE THERE ARE NO EXPERIMENTAL DATA FOR TH-232. MT = 102 THE SECTRUM USED WAS BASED ON AN UNDOCUMENTED MEASURED PHOTON SPECTRUM AT THERMAL NEUTRON ENERGY FOR U-238 WITH A MINOR ADJUSTMENT FOR THE SMALL Q-VALUE DIFFERENCE BETWEEN U-238 AND TH -232. IT WAS ASSUMED THAT THE SPECTRUM REMAINED UNCHANGED FOR ALL INCIDENT NEUTRON ENERGIES. REFERENCES 1) Maslov V., Porodzinskij Yu., Baba M.,Hasegawa A., Kornilov N.V., Kagalenko A.B. JAERI-Research 01-0XX, 2001. 2) M.C.Brady and T.R.England Nucl.Sci. Eng. 103,129(1989). 3) Glendenin L.E., Gindler J.E ., Ahmad I. et. al., Phys. Rev. C 152 (1980). 4) Conde H., Holmberg M., AF, 29, 4, 33 (1965). 5) Frehaut J., Bois R., Bertin A., Int. Conf. on Nuclear Data for Science and Technology, Antwerp., Belgium, 6-10 Sep. 1982, 78(1982). 6) Prokhorova L.I., Smirenkin G.N., Yad. Fizika, 7, 961 (1968). 7) Malinovskij V.V.,Vorob'jova V.G., Kuz'minov B.D. et al., Atomnaya Energ.,54, (3), 209 (1983). 8) Caruana J., Boldeman J.W.,Walsh R.L., Nuclear Physics A, 285, 217 (1977). 9) Howe R.E., Nucl. Sci. Eng., 86, 157 (1984). 10) Olsen K.D. ORNL/TM-8056 (1982), ENDF-319. 11) Cullen D. PREPRO2000: 2000 ENDF/B Pre-Processing Codes. 12) NJOY 94.10 Code System for Producing Pointwise and Multigroup Neutron and Photon Cross Sections from ENDF/B Data, RSIC Peripheral Shielding Routine Collection, ORNL, PSR-355, LANL, Los Alamos, New Mexico (1995). 13) Hibdon C.T., Langsdorf A. jr.,ANL-5175, 7 (1954). 14) Kobayashi K., Fujita Y., Oosaki T. et al., Nucl. Sci. Eng., 65, (2), 347 (1978). 15) Vertebnyj V.P., Kirilyuk A.L.,Gnidak N.L. et al., 3rd All-Uni Conf. on Neutron Physics, 9-13 Jun, Kiev, 3, 151 (1975). 16) Vertebnyj V.P., Murzin A.V.,. Pshenichnyj V.A. et al., IAEA-4 257 (1987). 17) Poenitz W.P., Whalen J.F., Smith A.B., Nucl. Sci. Eng., 78, 333 (1981). 18) Poenitz W.P., Whalen J.F., ANL-NDM-80 (1983). 19) Uttley C.A., Newstead C.M., Diment K.M., 66PARIS, 1, 165 (1966). 20) Haouat G., Lachkar J., Lagrange Ch. et al., Nucl. Sci. and Eng. 81, 491 (1982). 21) Haouat et al., NEANDC(E)-196 (1978). 22) Miura T., Baba M., Ibaraki M. et al. Proc. of the 1998 Symp. Nuclear Data, November 19-20, 1998, JAERI, Tokai, Japan, JAERI-Conf., 99-002, p. 101. 23) Moldauer P.A., Phys. Rev., C11, 426 (1975). 24) Tepel J.W., Hoffman H.M., Weidenmuller H.A. Phys. Lett. 49, 1 (1974). 25) Ciarcia C.A., Couchell G.P., Egan J.J. et al., Nucl. Sci. and Eng. 91, 428 (1985). 26) Dave J.H., Egan J.J., Couchell G.P. et al., Nucl. Sci. and Eng. 91, 187 (1985). 27) Sheldon E., Alliyar A., Beghian L.E., et al., Proc. Int. Conf Nucl. Data for Sci. and Technol., Julich, 1991,p.989. 28) Goswani G.C., Egan J.J., Kegel G.H.R. et al., Nucl. Sci. and Eng. 100,48 (1988). 29) Glazkov N.P., Atomnaya Energ. 14, (4), 400, (1963). 30) Smith W., Phys. Rev, 126, 718 (1962). 31) Fujita Y., Ohsawa T., Bugger R.M. et al.,J. of Nucl. Sci. and Tech., 20, 983 (1983). 32) Shurshikov E.N., Nucl. Data Sheets, 53, 601 (1988). 33) Uhl M., Strohmaier B., IRK-76/01, IRK, Vienna (1976). 34) Tewes H.A., Caretto A.A., Miller A.E., Nethaway D.R., UCRL-6028-T,1960. 35) Butler J.P., Santry D.C. Canadian Journal of Chemistry, 39, 89(1961). 36) Cochran D.R.F., Henkel R.L. Preprint WASH-1013, 34 (1958). 37) Raics P., Daroczy S., Csikai J., Kornilov N.V. et al.,Phys. Rev.C 32,87, (1985); Report INDC(HUN)-029/L, IAEA, 1990. 38) Prestwood R.J., Bayhurst B.P. Phys. Rev., 121, 1438 (1961). 39) Smith, B. Am.Phy.Soc.2, 196 (1957). 40) Karius H., Ackermann A., Scobel W. Journ. Physics part G , 5, 715 (1979). 41) Perkin J.L., Coleman R.F. Journal of Nuclear Energy, 14, 69 (1961). 42) Phillips J.A. Report of AERE-NP/R-2033, 1956. 43) Chatani H., Kimura I. Annals of Nuclear Energy, 19,477 (1992) 44) Zysin Yu.A., et al., Journal of Atomic Energy, 8, 360, (1960) 45) Filatenkov A.A. et al.,INDC(CCP)-402, (1997); RI- 252, (1999) 46) Batchelor R.,Gilboy W.B.,Towle J.H. Nuclear Physics, 65, 236 (1965). 47) Behrens J.W., Browne J.C., Ables E., Nucl. Sci. Eng., 81, 512 (1982). 48) Meadows J.W., Int.Conf. on Nuclear Cross Sections for Technology,Knoxville, Tennessee, 22-26 Oct 1979, 479 (1979). 49) Goverdovskij A.A. et al., Atomnaya Energ.60, (6), 416 (1986). 50) Goverdovskij A.A. et. al., Atomnaya Energ.61, 380 (1986). 51) Fursov B.I., Baranov E.Yu., Klemyshev M.P. et.al., Atomnaya Energ. 71,(4), 320 (1991). 52) Kobayashi K., Fujita Y., Yamamuro N. Nucl. Sci. Techn., 18, 823 (1981). 53) Wissak K., Voss F., Kaeppeler F.Nucl. Sci. Eng.,137, 183(2000 54) Grigor'ev Yu.V., Kitaev V.Ya. et al. ISINN-8, 68 Dubna, 2000. 55) Lindner M., Nagle R.J., Landrum J.H. Nucl. Sci. and Eng., 59, 381 (1976). 56) Baba M.,Wakabayashi H.,Ito N. et al.,INDC(NDS)-220,1989,R, INDC(JAP)-129/L,(1989). 57) Miura T., Baba M., Ibaraki M. et al. Ann. Nucl.Energy, 28, 937 (2001). 58) Sukhikh S.E., Lovchikova G.N.,Vinogradov V.A. et al., Yadernye Konstanty,(3),34 (1986). 59) Boykov G.S.,Dmitriev V.D.,Kudyaev G.A. et al., Yadernaya Fizika,53,(3),628 (1993). 60) Miura T.,T. Win, Baba M. et al., Proc. of the 1999 Symp. on Nuclear Data, November 18-19, 1999, JAERI, Tokai, Japan, JAERI-Conf., 2000-005, 137 (1999). 61) Lovchikova G.N. et al., Proc. of Meeting on PFNS properties, Mito, Japan,. 62) Lovchikova G.N., Trufanov A.M.,Svirin M.I. et al., Proc. Int. Workshop on Nuclear Fission Physics, Obninsk, 2000,72 (2000) 63) R.W.PEELE AND F.C.MAIENSCHEIN, NUCL.SCI.ENG. 40, 485 (1970) 64) R.J. HOWERTON, D.E. CULLEN, R.C. HAIGHT, M.H. MACGREGOR, S.T. PERKINS, AND E.F. PLECHARTY, "THE LLL EVALUATED NUCLEAR DATA LIBRARY (ENDL): EVALUATION TECHNIQUES, REACTION INDEX, AND DESCRIPTIONS OF INDIVIDUAL EVALUATIONS," UCRL-50400, VOL. 15, PART A, LAWERENCE LIVERMORE LABORATORY (1975). 65) S.T.PERKINS,R.C.HAIGHT AND R.J.HOWERTON,NUCL.SCI.ENG.57,1 (1975)Back |