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61-Pm-147 NEA EVAL-JUN06 NEA/WPEC Subgroup 23
DIST-JAN09 20090105
----JEFF-311 MATERIAL 6149
-----INCIDENT NEUTRON DATA
------ENDF-6 FORMAT
*************************** JEFF-3.1.1 *************************
** **
** Original data taken from: ENDFB-7 +New Eval **
** Modification: Int. FP Library NEA WPEC/SG23 **
******************************************************************
==============================================================
File produced by WPEC Subgroup 23 in 2004-2005
- WPEC: NEA Working Party on Evaluation Cooperation
- SG23: International Fission Product Library, IFPL
File obtained by merging: &&
- Resolved Resonances (MLBW) <300 eV : Ref.1 &&
- Unresolved Resonances 300 eV - 100 keV : JENDL-3.3 &&
- Fast neutron region >100 keV : JENDL-3.3 &&
&&
Calculated thermal cross sections & resonance integrals: &&
--------------------------------------------- &&
Reaction Cross section Res. integral &&
(barn) (barn) &&
Total 1.8931E+02 - &&
Elastic 2.0966E+01 - &&
Capture 1.6835E+02 2.1086E+03 &&
--------------------------------------------- &&
Corrected interpolation in MF=5.
Reference:
1) S.F.Mughabghab: Atlas of Neutron Resonances, to be
published by Elsevier, 2006 (5-th edition of BNL-325)
==============================================================
HISTORY
84-10 EVALUATION FOR JENDL-2 WAS MADE BY JNDC FPND W.G./1/
90-03 MODIFICATION FOR JENDL-3 WAS MADE/2/.
MF = 1 GENERAL INFORMATION
MT=451 COMMENTS AND DICTIONARY
MF = 2 RESONANCE PARAMETERS
MT=151 RESOLVED AND UNRESOLVED RESONANCE PARAMETERS
RESOLVED RESONANCE PARAMETERS FOR MLBW FORMULA (BELOW 102 EV)
FOR JENDL-3, THE EXISTING JENDL-2 DATA WERE ENTIRELY
REPLACED BY NEW EVALUATION MENTIONED BELOW. THE RADIATION
WIDTHS AND NEUTRON WIDTHS WERE ADOPTED FROM REF./3/. THE
ORBITAL ANGULAR MOMENTUM L WAS ASSIGNED BY TAKING INTO
ACCOUNT THE MAGNITUDE OF NEUTRON WIDTHS. TOTAL SPIN J OF
SOME RESONANCES WAS TENTATIVELY ESTIMATED WITH A RANDOM
NUMBER METHOD. SCATTERING RADIUS OF 8.21 FM WAS ESTIMETED
FROM THE MEASURED VALUES FOR ADJACENT NUCLIDES/3/. A
NEGATIVE RESONANCE WAS ADDED SO AS TO REPRODUCE THE THERMAL
CAPTURE AND ELASTIC SCATTERING CROSS SECTIONS GIVEN BY
MUGHABGHAB/3/.
UNRESOLVED RESONANCE REGION : 0.102 KEV - 100 KEV
THE NEUTRON STRENGTH FUNCTION S0 WAS BASED ON THE COMPILATION
OF MUGHABGHAB /3/, AND S1 AND S2 WERE CALCULATED WITH OPTICAL
MODEL CODE CASTHY/4/. THE OBSERVED LEVEL SPACING WAS
DETERMINED TO REPRODUCE THE CAPTURE CROSS SECTION CALCULATED
WITH CASTHY. THE EFFECTIVE SCATTERING RADIUS WAS OBTAINED
FROM FITTING TO THE CALCULATED TOTAL CROSS SECTION AT 100 KEV.
THE RADIATION WIDTH GG WAS BASED ON THE COMPILATION OF
MUGHABGHAB.
TYPICAL VALUES OF THE PARAMETERS AT 70 KEV:
S0 = 3.100E-4, S1 = 1.000E-4, S2 = 2.100E-4, SG = 145.E-4,
GG = 0.068 EV, R = 3.916 FM.
CALCULATED 2200-M/S CROSS SECTIONS AND RES. INTEGRALS (BARNS)
2200 M/S RES. INTEG.
TOTAL 188.6 -
ELASTIC 20.91 -
CAPTURE 167.7 2210
MF = 3 NEUTRON CROSS SECTIONS
BELOW 100 KEV, RESONANCE PARAMETERS WERE GIVEN.
ABOVE 100 KEV, THE SPHERICAL OPTICAL AND STATISTICAL MODEL
CALCULATION WAS PERFORMED WITH CASTHY, BY TAKING ACCOUNT OF
COMPETING REACTIONS, OF WHICH CROSS SECTIONS WERE CALCULATED
WITH PEGASUS/5/ STANDING ON A PREEQUILIBRIUM AND MULTI-STEP
EVAPORATION MODEL. THE OMP'S FOR NEUTRON GIVEN IN TABLE 1 WERE
ADOPTED FROM MOLDAUER/6/ BECAUSE THEY REPRODUCED WELL A THE
PM-147 TOTAL CROSS SECTION MEASURED BY FOSTER AND GLASGOW/7/.
THE OMP'S FOR CHARGED PARTICLES ARE AS FOLLOWS:
PROTON = PEREY/8/
ALPHA = HUIZENGA AND IGO/9/
DEUTERON = LOHR AND HAEBERLI/10/
HELIUM-3 AND TRITON = BECCHETTI AND GREENLEES/11/
PARAMETERS FOR THE COMPOSITE LEVEL DENSITY FORMULA OF GILBERT
AND CAMERON/12/ WERE EVALUATED BY IIJIMA ET AL./13/ MORE
EXTENSIVE DETERMINATION AND MODIFICATION WERE MADE IN THE
PRESENT WORK. TABLE 2 SHOWS THE LEVEL DENSITY PARAMETERS USED
IN THE PRESENT CALCULATION. ENERGY DEPENDENCE OF SPIN CUT-OFF
PARAMETER IN THE ENERGY RANGE BELOW E-JOINT IS DUE TO GRUPPELAAR
/14/.
MT = 1 TOTAL
BELOW 5 MEV, SPHERICAL OPTICAL MODEL CALCULATION WAS ADOPTED.
ABOVE 5 MEV, AN EYE-GUIDED CURVE WAS DETERMINED ON THE BASIS
OF EXPERIMENTAL DATA OF FOSTER AND GLASGOW/7/.
MT = 2 ELASTIC SCATTERING
CALCULATED AS (TOTAL - SUM OF PARTIAL CROSS SECTIONS).
MT = 4, 51 - 91 INELASTIC SCATTERING
SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WAS
ADOPTED. THE LEVEL SCHEME WAS TAKEN FROM REF./15/.
NO. ENERGY(MEV) SPIN-PARITY
GR. 0.0 7/2 +
1 0.0911 5/2 +
2 0.4105 3/2 +
3 0.4893 5/2 +
4 0.5310 5/2 +
5 0.6800 7/2 +
6 0.6858 5/2 +
LEVELS ABOVE 0.7 MEV WERE ASSUMED TO BE OVERLAPPING.
MT = 102 CAPTURE
SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WITH
CASTHY WAS ADOPTED. DIRECT AND SEMI-DIRECT CAPTURE CROSS
SECTIONS WERE ESTIMATED ACCORDING TO THE PROCEDURE OF BENZI
AND REFFO/16/ AND NORMALIZED TO 1 MILLI-BARN AT 14 MEV.
THE GAMMA-RAY STRENGTH FUNCTION (1.40E-02) WAS DETERMINED FROM
THE SYSTEMATICS OF RADIATION WIDTH (0.066 EV) AND AVERAGE
S-WAVE RESONANCE LEVEL SPACING (4.7 EV).
MT = 16 (N,2N) CROSS SECTION
MT = 17 (N,3N) CROSS SECTION
MT = 22 (N,N'A) CROSS SECTION
MT = 28 (N,N'P) CROSS SECTION
MT = 32 (N,N'D) CROSS SECTION
MT = 33 (N,N'T) CROSS SECTION
MT =103 (N,P) CROSS SECTION
MT =104 (N,D) CROSS SECTION
MT =105 (N,T) CROSS SECTION
MT =106 (N,HE3) CROSS SECTION
MT =107 (N,ALPHA) CROSS SECTION
THESE REACTION CROSS SECTIONS WERE CALCULATED WITH THE
PREEQUILIBRIUM AND MULTI-STEP EVAPORATION MODEL CODE PEGASUS.
THE KALBACH'S CONSTANT K (= 130.6) WAS ESTIMATED BY THE
FORMULA DERIVED FROM KIKUCHI-KAWAI'S FORMALISM/17/ AND LEVEL
DENSITY PARAMETERS.
FINALLY, THE (N,P) AND (N,ALPHA) CROSS SECTIONS WERE
NORMALIZED TO THE FOLLOWING VALUES AT 14.5 MEV:
(N,P) 7.06 MB (SYSTEMATICS OF FORREST/18/)
(N,ALPHA) 2.73 MB (SYSTEMATICS OF FORREST)
MT = 251 MU-BAR
CALCULATED WITH CASTHY.
MF = 4 ANGULAR DISTRIBUTIONS OF SECONDARY NEUTRONS
LEGENDRE POLYNOMIAL COEFFICIENTS FOR ANGULAR DISTRIBUTIONS ARE
GIVEN IN THE CENTER-OF-MASS SYSTEM FOR MT=2 AND DISCRETE INELAS-
TIC LEVELS, AND IN THE LABORATORY SYSTEM FOR MT=91. THEY WERE
CALCULATED WITH CASTHY. FOR OTHER REACTIONS, ISOTROPIC DISTRI-
BUTIONS IN THE LABORATORY SYSTEM WERE ASSUMED.
MF = 5 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS
ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS WERE CALCULATED WITH
PEGASUS FOR INELASTIC SCATTERING TO OVERLAPPING LEVELS AND FOR
OTHER NEUTRON EMITTING REACTIONS.
TABLE 1 NEUTRON OPTICAL POTENTIAL PARAMETERS
DEPTH (MEV) RADIUS(FM) DIFFUSENESS(FM)
---------------------- ------------ ---------------
V = 46.0 R0 = 6.722 A0 = 0.62
WS = 7.0 RS = 6.722 AS = 1.0
VSO= 7.0 RSO= 6.722 ASO= 0.62
THE FORM OF SURFACE ABSORPTION PART IS GAUSSIAN TYPE.
TABLE 2 LEVEL DENSITY PARAMETERS
NUCLIDE SYST A(1/MEV) T(MEV) C(1/MEV) EX(MEV) PAIRING
---------------------------------------------------------------
59-PR-143 1.500E+01 6.280E-01 2.607E+00 4.558E+00 7.600E-01
59-PR-144 1.600E+01 6.000E-01 1.045E+01 3.744E+00 0.0
59-PR-145 * 2.088E+01 5.411E-01 7.911E+00 5.258E+00 9.200E-01
59-PR-146 * 2.263E+01 5.387E-01 8.918E+01 4.815E+00 0.0
60-ND-144 1.771E+01 5.640E-01 4.792E-01 5.691E+00 1.940E+00
60-ND-145 2.054E+01 5.120E-01 2.465E+00 4.869E+00 1.180E+00
60-ND-146 2.019E+01 5.660E-01 1.121E+00 6.714E+00 2.100E+00
60-ND-147 2.398E+01 4.850E-01 5.510E+00 5.235E+00 1.180E+00
61-PM-145 * 1.769E+01 5.411E-01 2.780E+00 4.120E+00 7.600E-01
61-PM-146 * 1.942E+01 5.387E-01 2.241E+01 3.849E+00 0.0
61-PM-147 2.192E+01 4.913E-01 4.801E+00 4.589E+00 9.200E-01
61-PM-148 2.227E+01 4.300E-01 1.420E+01 2.672E+00 0.0
---------------------------------------------------------------
SYST: * = LDP'S WERE DETERMINED FROM SYSTEMATICS.
SPIN CUTOFF PARAMETERS WERE CALCULATED AS 0.146*SQRT(A)*A**(2/3).
IN THE CASTHY CALCULATION, SPIN CUTOFF FACTORS AT 0 MEV WERE
ASSUMED TO BE 4.666 FOR PM-147 AND 5.0 FOR PM-148.
REFERENCES
1) AOKI, T. ET AL.: PROC. INT. CONF. ON NUCLEAR DATA FOR BASIC
AND APPLIED SCIENCE, SANTA FE., VOL. 2, P.1627 (1985).
2) KAWAI, M. ET AL.: PROC. INT. CONF. ON NUCLEAR DATA FOR SCIENCE
AND TECHNOLOGY, MITO, P. 569 (1988).
3) MUGHABGHAB, S.F.: "NEUTRON CROSS SECTIONS, VOL. I, PART B",
ACADEMIC PRESS (1984).
4) IGARASI, S.: J. NUCL. SCI. TECHNOL., 12, 67 (1975).
5) IIJIMA, S. ET AL.: JAERI-M 87-025, P. 337 (1987).
6) MOLDAUER, P. A.: NUCL. PHYS., 47, 65 (1963).
7) FOSTER. D.G. JR. AND GLASGOW, D.W.: PHYS. REV., C3, 576
(1971).
8) PEREY, F.G: PHYS. REV. 131, 745 (1963).
9) HUIZENGA, J.R. AND IGO, G.: NUCL. PHYS. 29, 462 (1962).
10) LOHR, J.M. AND HAEBERLI, W.: NUCL. PHYS. A232, 381 (1974).
11) BECCHETTI, F.D., JR. AND GREENLEES, G.W.: POLARIZATION
PHENOMENA IN NUCLEAR REACTIONS ((EDS) H.H. BARSHALL AND
W. HAEBERLI), P. 682, THE UNIVERSITY OF WISCONSIN PRESS.
(1971).
12) GILBERT, A. AND CAMERON, A.G.W.: CAN. J. PHYS., 43, 1446
(1965).
13) IIJIMA, S., ET AL.: J. NUCL. SCI. TECHNOL. 21, 10 (1984).
14) GRUPPELAAR, H.: ECN-13 (1977).
15) LEDERER, C.M., ET AL.: "TABLE OF ISOTOPES, 7TH ED.", WILEY-
INTERSCIENCE PUBLICATION (1978).
16) BENZI, V. AND REFFO, G.: CCDN-NW/10 (1969).
17) KIKUCHI, K. AND KAWAI, M.: "NUCLEAR MATTER AND NUCLEAR
REACTIONS", NORTH HOLLAND (1968).
18) FORREST, R.A.: AERE-R 12419 (1986).
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