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6-C - 0 LANL,ORNL EVAL-JUN96 M.B.CHADWICK, P.G.YOUNG, C.Y. FU Ch96a,Ch96b,Fu90,Ch99DIST-JAN09 20090105 ----JEFF-311 MATERIAL 600 REVISION 2 -----INCIDENT NEUTRON DATA ------ENDF-6 FORMAT *************************** JEFF-3.1.1 ************************* ** ** ** Original data taken from: JEFF-3.1 ** ** ** ****************************************************************** ***************************** JEFF-3.1 ************************* ** ** ** Original data taken from: ENDF/B-VI.8 ** ** ** ****************************************************************** ****************************************************************** ENDF/B-VI MOD 3 Evaluation, June 1996, M.B. Chadwick and P.G. Young (LANL) Los Alamos LA150 Library, produced with FKK/GNASH/GSCAN code in cooperation with ECN Petten. This evaluation provides a complete representation of the nuclear data needed for transport, damage, heating, radioactivity and shielding applications over the incident neutron energy range from 1.0E-11 to 150 MeV. The discussion here is divided into the region below and above 20 MeV. INCIDENT NEUTRON ENERGIES < 20 MeV Below 20 MeV the evaluation is based completely on the ENDF/B- VI.1 (Release 1) evaluation by Fu [Fu90]. The following minor modifications were made to the ENDF/B-VI.1 evaluation: 1. The energy range from En = 20 MeV to 32 MeV was replaced by the LANL evaluation (described below); 2. The elastic, nonelastic, and total cross sections from 19 to 20 MeV were varied to join smoothly with the higher energy values at 20 MeV. 3. The new flag, LTT=3, is used in MF=4,MT=2 to indicate that Legendre polynomials are used below 20 MeV and probability tabulations at higher energies. A small discontinuity exists for MF=4,MT=2 at 20 MeV where the two different representations join. The higher energy evaluation utilizes a tabulation in order to overcome the inaccuracies caused by the ENDF-6 limitation of 20 for the maximum number of Legendre coefficients. INCIDENT NEUTRON ENERGIES > 20 MeV (12C analysis) The evaluation above 20 MeV utilizes MF=6, MT=5 to represent all reaction data. Production cross sections and emission spectra are given for neutrons, protons, deuterons, alpha particles, gamma rays, and all residual nuclides produced (A>5) in the reaction chains. To summarize, the ENDF sections with non-zero data above En = 20 MeV are: MF=3 MT= 1 Total Cross Section MT= 2 Elastic Scattering Cross Section MT= 3 Nonelastic Cross Section MT= 5 Sum of Binary (n,n') and (n,x) Reactions MT=102 Radiative Capture Cross Section (Estimate Only) MF=4 MT= 2 Elastic Angular Distributions MF=6 MT= 5 Production Cross Sections and Energy-Angle Distributions for Emission Neutrons, Protons, Deuterons, and Alphas; and Angle-Integrated Spectra for Gamma Rays and Residual Nuclei That Are Stable Against Particle Emission MF=33 MT= 1 Covariance file for total cross section MT= 2 Covariance file for elastic cross section MT= 3 Covariance file for nonelastic cross section MT= 5 Covariance file for composite reaction cross sect. MT=102 Covariance file for capture cross section The evaluation is based on nuclear model calculations that have been benchmarked to experimental data, especially for n + C12 and p + C12 reactions [Ch96a]. We use the GNASH code system [Yo92], which utilizes Hauser-Feshbach statistical, preequilibrium and direct-reaction theories. Coupled-channel and spherical optical model calculations are used to obtain particle transmission coefficients for the Hauser-Feshbach calculations, as well as for the elastic neutron angular distributions. Cross sections and spectra for producing individual residual nuclei are included for reactions that exceed a cross section of approximately 1 nb at any energy. The energy-angle-correlations for all outgoing particles are based on Kalbach systematics [Ka88]. A model was developed to calculate the energy distributions of all recoil nuclei in the GNASH calculations (Ch96b). The recoil energy distributions are represented in the laboratory system in MT=5, MF=6, and are given as isotropic in the lab system. Note that all other data in MT=5,MF=6 are given in the center-of-mass system. This method of representation requires a modification of the original ENDF-6 format. Preequilibrium corrections were performed in the course of the GNASH calculations using either Feshbach, Kerman, Koonin (FKK) theory [Ch93] or the exciton model of Kalbach [Ka77, Ka85]. Discrete level data from nuclear data sheets were matched to continuum level densities using the formulation of Ignatyuk [Ig75] and pairing and shell parameters from the Cook [Co67] analysis. Neutron and charged-particle transmission coefficients were obtained from the optical potentials, as discussed below. Gamma-ray transmission coefficients were calculated using the Kopecky-Uhl model [Ko90]. **************************************************************** ENDF/B-VI MOD 2 Revision, July 1991 The only changes for MOD 2 are completion of some references, and addition of total elastic scattering uncertainties as recommended by the Standards Subcommittee. "Following concerns expressed about the seemingly small standards uncertainties, the standards subcommitte has provided expanded uncertainties. These uncertainties are estimates such that if a modern day experiment were performed today on a given standard using the best techniques, those results should fall within these expanded uncertainties (2/3 of the time). They take into account data inconsistencies and concerns about R-Matrix parameters. Note that it is not assumed that the uncertainties are totally correlated within the energy ranges given. It is recommended that these expanded uncertainties be put in file 1 and in the documentation for the standards." Quote from Standards Subcommittee CSEWG minutes for the May 1990 meeting. C(n,n) Total elastic scattering cross section Energy (keV) Uncertainty (%) 1 - 500 0.46 500 - 1500 0.53 1500 - 1800 0.60 **************************************************************** ENDF/B-VI MOD 1 Evaluation, C.Y. Fu, E.J. Axton, and F.G. Perey ORNL NEW EVALUATION FOR VERSION VI: 1. Total and elastic scattering from 0.1 to 0.25 MeV and from 1.6 to 1.9 MeV due to inclusion of C13 resonances [Fu88]. 2. Elastic angular distribution: 0.1 to 2.0 MeV due to 13C effects [Fu88]. 3. New evaluation for all File 3 data 5-32 MeV by Axton [Ax88], including new data for (n,n'3a) [An86, Br84, Me84, Ol87], for (n,n') [Ba85, Gu81, Sa81], and for kerma factors [Be81, Br83, Bu85, De84, De85, De86, Di82, Ha84, Mc86, We79]. 4. Extention of energy and angular distributions to 32 MeV were mostly based on extrapolation. File 33 was extended to 32 MeV with the addition of the new LB=8 subsubsection. Retained from ENDF/B-V (with negligible changes such as Q-values): all data between 2.0 and 5.0 MeV [Fu78], all energy and angular data for neutron and gamma-ray productions, and uncertainty files (LB=8 subsubsection added). Data and evaluation techniques used in the new evaluation and ENDF/B-V evaluation, as adopted here, are summerized below. MF-MT 3-1 TOTAL 1.E-5 eV TO 4.81 MeV -- sum of 3-2 and 3-102. 4.81 MeV TO 20 MeV -- [Sc67, Ci69, Pe72]. 3-2 ELASTIC SCATTERING 1.E-5 eV to 4.81 MeV -- R-Matrix analysis with data [Sc67, Ci69, Pe72, Ah70, Bl75, Di68, Fr70, He75, La57, La61, La69, Me70, Ki76, Ho72, Ho75, St70, Me54, Wi58, Kn73, Pu64, El62, We65, Ke65, Go65, Ga72, Pk72]. Bayes theorem (or nonlinear least square) used for energies less then 2 MeV, resulting weights were then used in the R-Matrix analysis. A thermal total cross section of 4.746 +- 0.25 (evaluated by Lubitz [Lu76]) was also used in the R-Matrix fit. 4.81 MeV to 8 MeV -- [Ga72, Ve73, Pk72]. 8 MeV to 14 MeV -- [Ha75, Ve73, Pu76]. 14 MeV to 32 MeV -- [Bo68, Me84]. R-Matrix analysis for C13 below 2 MeV with data of [La81, He75, Co61, Au79]. 3-3 NONELASTIC 1.E-5 eV to 4.81 MeV -- same as 3-102. 4.81 MeV to 32 MeV -- 3-1 minus 3-2. 3-4 INELASTIC -- sum of 3-51 through 3-91 3-16 (N,2N) -- [An81, We81] 3-24 (N,2NA) -- empirical estimate 3-28 (N,NP) -- empirical estimate 3-32 (N,ND) -- empirical estimate 3-33 (N,NT) -- include (N,NPT) and (N,N2P) 3-41 (N,2NP) -- include (N,2NHE-3) 3-51 INELASTIC SCATTERING TO 4.439-MeV LEVEL 4.81 MeV to 6.32 MeV -- 3-3 minus 3-102. 6.32 MeV to 8.796 MeV -- 3-3 minus 3-102 minus 3-107. 8.796 MeV TO 32 MeV -- same refs. as in 3-2 and gamma-ray data of [Mo72]. New data considered for Version-VI: [Ba85, Gu81, Sa81]. 3-52 to 3-91 (N,N PRIME 3A) MT=52 to 57: real levels MT=58 to 73: pseudo levels with 1-MeV width MT=91: an evaporation component with T=0.3 to reproduce correct threshold effect and the decay of the 2.43-MeV level of 9Be. New data considered for ENDF/B-VI: [An86, Br84]. 3-102 CAPTURE 1.E-5 eV to 1 MeV -- 1/v with 3.36 mb at thermal. 1 MeV to 32 MeV -- derived from (G,N) cross section of [Co57]. 3-103 (N,P) -- [Ri68]. 3-104 (N,D) -- derived from (D,N) of [Am57]. 3-105 (N,T) -- estimated shape normalized to [Qa78] 3-107 (N,A) -- [Da63, Ve68, Re60, Gr55, Ob72, Va70]. 3-111 (N,2P) -- estimate 3-112 (N,PA) -- includes (N,LI-6), (N,DA), (N,TA), (N,DT), (N,HE6), (N,HE-3 A), (N,PTA) 3-115 (N,PD) -- estimate 3-116 (N,PT) -- estimate 3-203 PROTON PRODUCTION -- (3-28)+(3-41)+(3-103)+2*(3-111)+(3-112)+(3-115)+(3-116) 3-204 DEUTERON PRODUCTION -- (3-32)+(3-104)+(3-115) 3-205 TRITON PRODUCTION -- (3-33)+(3-105)+(3-116) 3-207 ALPHA PRODUCTION -- (3-24)+3*(3-52 to 3-91)+(3-107)+(3-112) 4-2 ANGULAR DISTRIBUTION OF ELASTICALLY SCATTERED NEUTRONS Same data and analysis as in 3-2. Legendre coefficients in center-of-mass. 4-51 INELASTIC SCATTERING TO 4.439-MeV LEVEL Same data sources as in 3-51. 4-52 INELASTIC SCATTERING TO 7.653-MeV LEVEL -- [Gr69]. 4-53 INELASTIC SCATTERING TO 9.638-MeV LEVEL -- [Gr69]. 4-54 to 4-91 -- isotropic in center-of-mass. 5-28 evaporation spectrum with T=0.3 to 0.5 MeV. 5-91 evaporation spectrum with T=0.3 MeV. This is a small component of (N,N PRIME 3A) and is used mainly for the decay of the 2.43-MeV level of 9Be [An75] and for reproducing the correct threshold effect [Fr55]. 12-51 MULTIMLICITY OF THE SINGLE GAMMA-RAY -- from 3-51 12-102 MULTIMLICITY OF (N,G) GAMMA-RAYS -- [Aj70]. 14-51 ANGULAR DISTRIBUTION OF 4.439-MeV GAMMA-RAYS -- [Mo72, Dr69, Ha59, Pr66, Ne64, An58, Ko65, En64]. 14-102 ANGULAR DISTRIBUTION OF CAPTURE GAMMA-RAYS -- isotropic in center-of-mass. 33-1 to 33-107 UNCERTAINTY FILES FOR FILE 3 DATA. ***************************************************************** REFERENCES [Aj70] F. Ajsenberg-Selove, Nucl.Phys. 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