Request ID3 Type of the request High Priority request
TargetReaction and processIncident EnergySecondary energy or angleTarget uncertaintyCovariance
 94-PU-239 (n,f) prompt g  Thermal-Fast Eg=0-10MeV 7.5 Y
FieldSubfieldDate Request createdDate Request acceptedOngoing action
 Fission LWR 28-APR-06 12-MAY-06 Y

Requester: Prof. Gerald RIMPAULT at CAD-DER, FR
Email: gerald.rimpault@outlook.fr

Project (context): JEFF, NEA WPEC Subgroup 27

Impact:
The four fast reactor systems of GenIV feature innovative core characteristics for which gamma-ray heating estimates for non-fuel zones require an uncertainty of 7.5% [1]. For the experimental Jules Horowitz Reactor (RJH) at Cadarache a similar requirement appears [2]. Recent studies show evidence of discrepancies on integral measurement in MASURCA, EOLE and MINERVE, from which it is clear that the expectations for GenIV systems and the RJH thermal reactor are not met [3]. Gamma-ray energy release is dominated by Pu-239 and U-235.

Accuracy:
7.5% on the total gamma energy. 7.5% on the multiplicity.
Best accuracy achievable for the gamma spectrum shape.

Justification document:
Reference 1: G. Rimpault, Proc. Workshop on Nuclear Data Needs for Generation IV, April 2005, Antwerp, Belgium
Reference 2: D. Blanchet, Proc. M&C 2005, Int. Topical Meeting on Mathematics and Computation, Supercomputing, Reactor Physics and Nuclear and Biological Applications, Sep. 2005, Avignon, France
Reference 3: 'Needs for accurate measurements of spectrum and multiplicity of prompt gammas emitted in fission', G. Rimpault, A. Courcelle and D. Blanchet, CEA/Cadarache - DEN/DER/SPRC.

Comment from requester:
Forty percent of the total gamma-ray energy release results from prompt decay of fission products. No comprehensive analytic expressions exist and Hauser-Feshbach model calculations are involved and presently lack sufficient knowledge to warrant a solution of the problem. New measurements would be needed to guide new evaluation efforts. Present evaluations are based on measurements from the seventies.

Review comment:
Discrepancies observed for C/E ratios in various benchmarks range from 10 to 28%. The request is well motivated and based on a considerable effort.

Entry Status:
Work in progress (as of SG-C review of May 2018)
Pending new evaluation or validation (as of SG-C review of June 2019)

Main references:
Please report any missing information to hprlinfo@oecd-nea.org

Experiments

Theory/Evaluation

Additional file attached:HPRLgammafission.pdf
Additional file attached:



Request ID99 Type of the request High Priority request
TargetReaction and processIncident EnergySecondary energy or angleTarget uncertaintyCovariance
 94-PU-239 (n,f) nubar  Thermal-5 eV  1 Y
FieldSubfieldDate Request createdDate Request acceptedOngoing action
 Fission  23-MAR-18 12-APR-18 Y

Requester: Dr Roberto CAPOTE NOY at IAEA, AUT
Email: roberto.capotenoy@iaea.org

Project (context):

Impact:

Cf. Ref. [1,2]. A similar, but stronger than in U-235, resonance nubar effect is expected for Pu-239 due to the 1/2 GS spin.

Accuracy:

Accuracy below 1% is required on the evaluated data. New measurements must strive to achieve a relative uncertainty below about 1% on the ratio to Cf-252(sf) nubar, as done in the best past experiments [3].

Statistical precision below about 1% at the resonances is required in order to unambiguously identify resonant fluctuations.

Justification document:

A new evaluation of the PFNS [4] in the thermal energy range has determined a lower value of the average neutron energy than that reported in the existing evaluated nuclear data libraries. This value is in agreement with Rising et al and Neudecker independent evaluations. However, a number of thermal-solution benchmarks has shown that the combined use of the new Thermal Neutron Constants and a softer prompt fission neutron spectrum at thermal energy yields k-eff values that are larger than measurements by a margin that increases as the above-thermal-leakage fraction (ATLF) increases (see Ref. [5]). Therefore a reduced criticality is needed for high-leakages solutions. Such reduced criticality may arises due to the (n,gf) process in Pu-239 resonance nubar.

Unfortunately, only measurements from the 70s and 80s are available, a critical region below 5 eV needs to be remeasured with higher incident-energy resolution and higher accuracy and precision to improve existing evaluated data files.

References

  1. M.T. Pigni, et al., n+235U resonance parameters and neutron multiplicities in the energy region below 100 eV, EPJ Web of Conferences 146, 02011 (2017)
  2. E. Fort et al., Evaluation of prompt nubar for 239Pu: Impact for applications of the fluctuations at low energy, Nuclear Science and Engineering 99, 375 (1988)
  3. Gwin et al., Measurements of the energy dependence of prompt neutron emission from 233U, 235U, 239Pu, and 241Pu for En = 0.005 to 10 eV relative to emission from spontaneous fission of 252Cf, Nuclear Science and Engineering 87, 381 (1984)
  4. R. Capote, et al., Prompt Fission Neutron Spectra of Actinides, Nuclear Data Sheets 131, 1-106 (2016)
  5. C. De Saint Jean (coordinator), Co-ordinated Evaluation of Plutonium-239 in the Resonance Region, Nuclear Energy Agency, International Evaluation Cooperation, NEA/WPEC-34, Report NEA/NSC/WPEC/DOC(2014)447 (2014)

Comment from requester:

Additionally to changes in nubar changes in resonance parameters may be required. We cannot split those effects on studied criticality benchmarks.

Review comment:

Entry Status:
Work in progress (as of SG-C review of May 2018)

Main references:
Please report any missing information to hprlinfo@oecd-nea.org

Experiments

  • F.J. Hambsch, et al., Prompt fission neutron emission in resonance fission of 239Pu, ND2004, Santa Fe (NM), USA, September 2004, AIP 769 (2005) 644

Theory/Evaluation

  • J.E. Lynn, P. Talou and O. Bouland, Reexamining the role of the (n,gf) process in the low-energy fission of 235U and 239Pu, PRC 97 (2018) 064601

Additional file attached:
Additional file attached: