Request ID4 Type of the request High Priority request
TargetReaction and processIncident EnergySecondary energy or angleTarget uncertaintyCovariance
 92-U-235 (n,f) prompt g  Thermal-Fast Eg=0-10MeV 7.5 Y
FieldSubfieldDate Request createdDate Request acceptedOngoing action
 Fission LWR, Gen-IV 10-MAY-06 12-MAY-06 Y

Requester: Prof. Gerald RIMPAULT at CAD-DER, FR
Email: gerald.rimpault@cea.fr

Project (context): JEFF, NEA WPEC Subgroup 27

Impact:
The four fast reactor systems of GenIV feature innovative core characteristics for which gamma-ray heating estimates for non-fuel zones require an uncertainty of 7.5% [1]. For the experimental Jules Horowitz Reactor (RJH) at Cadarache a similar requirement appears [2]. Recent studies show evidence of discrepancies on integral measurement in MASURCA, EOLE and MINERVE, from which it is clear that the expectations for GenIV systems and the RJH thermal reactor are not met [3]. Gamma-ray energy release is dominated by Pu-239 and U-235.

Accuracy:
7.5% on the total gamma energy
7.5% on multiplicity
Best accuracy achievable for the gamma spectrum shape

Justification document:
Reference 1: G. Rimpault, Proc. Workshop on Nuclear Data Needs for Generation IV, April 2005, Antwerp, Belgium
Reference 2: D. Blanchet, Proc. M&C 2005, Int. Topical Meeting on Mathematics and Computation, Supercomputing, Reactor Physics and Nuclear and Biological Applications, Sep. 2005, Avignon, France
Reference 3: 'Needs for accurate measurements of spectrum and multiplicity of prompt gammas emitted in fission', G. Rimpault, A. Courcelle and D. Blanchet, CEA/Cadarache – DEN/DER/SPRC.

Comment from requester:
Forty percent of the total gamma-ray energy release results from prompt decay of fission products. No comprehensive analytic expressions exist and Hauser-Feshbach model calculations are involved and presently lack sufficient knowledge to warrant a solution of the problem. New measurements would be needed to guide new evaluation efforts. Present evaluations are based on measurements from the seventies.

Review comment:
Discrepancies observed for C/E ratios in various benchmarks range from 10 to 28%. The request is well motivated and based on a considerable effort.

Entry Status:
Work in progress (as of SG-C review of May 2018)
Pending new evaluation or validation (as of SG-C review of June 2019)

Main references:
Please report any missing information to hprlinfo@oecd-nea.org

Experiments

Theory/Evaluation

Additional file attached:HPRLgammafission.pdf
Additional file attached:



Request ID12 Type of the request High Priority request
TargetReaction and processIncident EnergySecondary energy or angleTarget uncertaintyCovariance
 92-U-235 (n,g) SIG,RP  100 eV-1 MeV  3 Y
FieldSubfieldDate Request createdDate Request acceptedOngoing action
 Fission FBR, Thermal reactors 29-AUG-07 06-NOV-07 

Requester: Dr Yasunobu NAGAYA at JAEA, JPN
Email: nagaya.yasunobu@jaea.go.jp

Project (context): JENDL, NEA WPEC Subgroup 29

Impact:
U-235 cross sections are very important not only for major thermal reactors but for FBRs because lots of critical experiments for FBRs have been performed at critical assemblies where UO2 fuels are used as driver fuels. Experimental data obtained at such critical assemblies have a great impact on design work for FBRs. Recent studies show that calculated sodium void reactivity worths for BFS experiments underestimate the experimental results by 30-50% [1].
The significant discrepancies not only exceed the target accuracy of 20% for a FBR design but also deteriorate the design accuracy estimated with the cross-section adjustment and bias factor techniques. Thus such experimental data cannot be employed in these techniques.

Accuracy:
The requested accuracies (relative one standard deviation) are given for energy-averaged cross sections as follows:
Energy interval and accuracy
100eV - 500eV: 5%
500eV - 1keV: 5%
1keV -2.25keV: 5%
2.25keV- 5keV: 8%
5keV - 10keV: 8%
10keV - 20keV: 8%
20keV - 30keV: 8%
30keV - 40keV: 3%
40keV - 90keV: 3%
90keV -200keV: 3%
200keV-400keV: 3%
400keV-900keV: 3%
900keV - 1MeV: 3%
(It is assumed that the resolved resonance region is below 2.25 keV and the unresolved resonance region is between 2.25 keV and 30 keV. The boundaries for the resonance regions are the same as for JENDL-3.3.)

Justification document:
Reference 1: first attached document, O. Iwamoto, "WPEC Subgroup Proposal" JAEA, March 9 (2007).
Reference 2: second attached document, viewgraph for Dr. Iwamoto's proposal at the 19th WPEC meeting.

Comment from requester:
The re-evaluation of U-235 cross sections has been already proposed at the 19th WPEC meeting on 18 - 20 April 2007, at the NEA Headquarters, Issy-les-Moulineaux, France.

Review comment:
The proposal seems well motivated. Concerns were expressed in view of the recent changes to the evaluation that emerged from the activities of NEA/WPEC Subgroup 22 "Nuclear Data for Improved LEU-LWR Reactivity Predictions" and ENDF/B-VII benchmarking. The wider impact that new evaluations of U-235 will have, should be considered and duly accounted for by new efforts. Although, the sensitivity of the cross section for the target application is well argued, the documentation does not reveal if the problem must be uniquely attributed to the capture cross section of U-235 in the specified energy range.

Entry Status:
Work in progress (as of SG-C review of May 2018)
Completed (as of SG-C review of June 2019) - The request was related to an issue in the keV region identified by the JENDL project in the early 2000's. Some preliminary evaluation work was performed in the framework of WPEC/SG29 [Iwamoto:2011]. The new measurements performed at LANSCE [Jandel:2012], RPI [Danon:2017] and n_TOF [Balibrea:2017] have been used in the CIELO evaluation [Capote:2018]. The issue is now solved in all major libraries (JENDL-4.0, JEFF-3.3, ENDF/B-VIII.0).

Main references:
Please report any missing information to hprlinfo@oecd-nea.org

Experiments

  • M. Jandel et al., New Precision Measurements of the 235U(n,g) Cross Section, PRL 109 (2012) 202506, EXFOR 14149
  • A. Wallner et al., Novel Method to Study Neutron Capture of 235U and 238U Simultaneously at keV Energies, Phys. Rev. Lett. 112 (2014) 192501, EXFOR 23170
  • J. Balibrea et al., Measurement of the neutron capture cross section of the fissile isotope 235U with the CERN n_TOF Total Absorption Calorimeter and a fission tagging based on Micromegas detectors, NDS 119 (2014) 10
  • Y. Danon, et al., Simultaneous measurement of 235U fission and capture cross sections from 0.01 eV to 3 keV using a gamma multiplicity detector, Nucl. Sci. and Eng. 187 (2017) 191
  • J. Balibrea et al., Measurement of the neutron capture cross section of the fissile isotope 235U with the CERN n TOF total absorption calorimeter and a fission tagging based on micromegas detectors, EPJ Conferences 146 (2017) 11021

Theory/Evaluation

  • R. Capote et al., IAEA CIELO Evaluation of Neutron-induced Reactions on 235U and 238U Targets, NDS 148 (2018) 254

Validation

  • O. Iwamoto et al., Uranium-235 Capture Cross-section in the keV to MeV Energy Region, International evaluation cooperation, Report NEA/WPEC-29, OECD NEA (2011)
  • M. Salvatores, et al., Methods and Issues for the Combined Use of Integral Experiments and Covariance Data: Results of a NEA International Collaborative Study, Nuclear Data Sheets 118 (2014) 38
  • G. Palmiotti, et al., Combined Use of Integral Experiments and Covariance Data, Nuclear Data Sheets 118 (2014) 596

Additional file attached:U235proposal.pdf
Additional file attached:Viewgraph.U235proposal.pdf



Request ID100 Type of the request Special Purpose Quantity
TargetReaction and processIncident EnergySecondary energy or angleTarget uncertaintyCovariance
 92-U-235 (n,f),(p,f) SIG  100 MeV-500 MeV  5 Y
FieldSubfieldDate Request createdDate Request acceptedOngoing action
 Standard ADS 23-MAR-18 11-APR-18 Y

Requester: Dr Roberto CAPOTE NOY at IAEA, AUT
Email: roberto.capotenoy@iaea.org

Project (context):

Impact:

Improvements in the standard cause all measurements relative to that standard to be improved. See Ref. [1].

Accuracy:

5% of the cross-section

Justification document:

There are discrepancies (see Fig. 24 in section III.E, pp.161-162 of Ref. [1]) between different theoretical calculations, data estimated from the (p,f) reaction, and the only measured data set of U-238(n,f) cross section at those energies [2]. New measurements of absolute cross sections of U-235 or U-238 (n,f) and/or U-235 or U-238 (p,f) reactions in the energy range where pion channels begin to play an important role (100-500 MeV) are needed to solve the discrepancies and to reduce the uncertainties of the Neutron Standards in that energy range.

References

  1. A.D. Carlson, et al., Evaluation of the Neutron Data Standards, Nuclear Data Sheets 148, 143-188 (2018)
  2. Z.W. Miller, A Measurement of the Prompt Fission Neutron Energy Spectrum for 235U(n,f) and the Neutron-induced Fission Cross Section for 238U(n,f), PhD Thesis, University of Kentucky (2015); https://uknowledge.uky.edu/physastron_etds/29/

Comment from requester:

At high-energy the (n,f) cross-section can be inferred with rather low uncertainty from (p,f) cross-section measurements, and thanks to this can be used in the neutron standards evaluation.

Review comment:

Entry Status:
Work in progress (as of SG-C review of May 2018)

Main references:
Please report any missing information to hprlinfo@oecd-nea.org

Experiments

  • U-235 measurement performed at n_TOF in 2018

Theory/Evaluation

  • B. Marcinkevicius, S. Simakov, V. Pronyaev, 209Bi(n,f) and natPb(n,f) cross sections as a new reference and extension of the 235U, 238U and 239Pu(n,f) standards up to 1 GeV, IAEA Report INDC(NDS)-0681
  • A.D. Carlson et al., Evaluation of the Neutron Data Standards, NDS 148 (2018) 143

Additional file attached:
Additional file attached: