JEFF-3.1.1 General Purpose Neutron File, May 2005. 2310 0 0 0 4.309900+4 9.805661+1 1 0 2 14331 1451 1 0.000000+0 0.000000+0 0 0 0 64331 1451 2 1.000000+0 2.000000+8 1 0 10 314331 1451 3 0.000000+0 0.000000+0 0 0 616 1824331 1451 4 43-Tc- 99 CEA-NRG EVAL-FEB05 Gunsing, Serot, Koning 4331 1451 5 DIST-MAY05 REV1-MAY05 20050504 4331 1451 6 ----JEFF-31 Material 4331 REVISION 1 4331 1451 7 -----INCIDENT NEUTRON DATA 4331 1451 8 ------ENDF-6 FORMAT 4331 1451 9 ***************************** JEFF-3.1.1 ************************4331 1451 10 ** **4331 1451 11 ** Original data taken from: JEFF-3.1 **4331 1451 12 ** **4331 1451 13 ******************************************************************4331 1451 14 6334 1451 22 JEFF-3.1.1 Revision, March 2008, G.Noguere (CEA) 6334 1451 23 6334 1451 24 MF=2 RESONANCE PARAMETERS (Revised to acount integral trends) 6334 1451 25 6334 1451 21 ************** G E N E R A L I N F O R M A T I O N *************4331 1451 15 4331 1451 16 This evaluated data file is based primarily on new measurements in4331 1451 17 the resolved and unresolved resonance range and on a theoretical 4331 1451 18 analysis with the nuclear model code TALYS [kon04], version 0.65. 4331 1451 19 The nuclear model parameters of TALYS have been adjusted to 4331 1451 20 reproduce the existing experimental data. The resulting data file 4331 1451 21 provides a complete representation of nuclear data needed for 4331 1451 22 transport, damage, heating, radioactivity, and shielding 4331 1451 23 applications over the incident neutron energy range from 4331 1451 24 1.0E-11 to 200 MeV. 4331 1451 25 4331 1451 26 This file is part of a larger collection of isotopic evaluations, 4331 1451 27 all created by running TALYS with input parameters that do not or 4331 1451 28 slightly deviate from the default values. The mutual quality of 4331 1451 29 these isotopic evaluations is thus relatively consistent. 4331 1451 30 The same set of nuclear models is used and, equally important, 4331 1451 31 the same ENDF-6 formatting procedures for each isotope. We have 4331 1451 32 intended to make this evaluation complete in its description of 4331 1451 33 reaction channels, and use a compact method to store the data. 4331 1451 34 4331 1451 35 For certain reactions and energy ranges TALYS may not be used. 4331 1451 36 This is the case when TALYS is not appropriate, such as for the 4331 1451 37 description of resonances, or when the directly available 4331 1451 38 experimental data is of better quality, as for e.g. low-energy 4331 1451 39 total cross sections. In these cases, we have adopted the best 4331 1451 40 possible data from an existing library, or directly from unfiled 4331 1451 41 experimental data. All transport data for particles, photons and 4331 1451 42 residual nuclides are filed using a combination of MF1,2,3,4 and 4331 1451 43 MF6. This includes cross sections, angular distributions, 4331 1451 44 double-differential spectra, discrete and continuum photon 4331 1451 45 production cross sections, and residual production (activation) 4331 1451 46 cross sections. Moreover, isomeric production data are stored in 4331 1451 47 MF8 and MF10. This evaluation can thus be used as both transport 4331 1451 48 and activation library. The data file has been created 4331 1451 49 automatically using the ENDF-6 format generator TEFAL. 4331 1451 50 4331 1451 51 ##### ORIGIN 4331 1451 52 4331 1451 53 Data < 200 MeV : New evaluation CEA-NRG 4331 1451 54 4331 1451 55 Resonance parameters (MF2/MT151): CEA/IRMM data for E < 100 keV 4331 1451 56 Total and capture (MF3/MT1,102): CEA/IRMM data for E < 100 keV 4331 1451 57 All other data : Produced with TALYS code 4331 1451 58 4331 1451 59 ****************** R E S O N A N C E D A T A *******************4331 1451 60 MF = 2 Resonance parameters 4331 1451 61 4331 1451 62 Resolved resonance parameters of the Reich-Moore approximation 4331 1451 63 of the R-matrix (LRF=3) are taken from refs. [gun00,gun01]. 4331 1451 64 Resolved resonance parameters up to 11 keV are given but used 4331 1451 65 until 6 keV (EH=6000). One negative resonance has been adjusted 4331 1451 66 with the code SAMMY [lar03] to match a thermal cross section of 4331 1451 67 22.8b [fur04]. Processing with NJOY gives the following values: 4331 1451 68 4331 1451 69 4331 1451 70 thermal quantities at 293.6 K = 0.0253 eV 4331 1451 71 ----------------------------------------- 4331 1451 72 thermal capture xsec: 2.2820E+01 4331 1451 73 thermal capture integral: 2.0284E+01 4331 1451 74 thermal capture g-factor: 1.0030E+00 4331 1451 75 capture resonance integral: 3.2360E+02 4331 1451 76 ----------------------------------------- 4331 1451 77 4331 1451 78 From 6 keV to 100 keV unresolved resonances have been fitted 4331 1451 79 with SAMMY/FITACS code [lar03]. The average resonance 4331 1451 80 parameters were adjusted on capture and total cross sections 4331 1451 81 performed by Gunsing [gun00]. The following average parameters 4331 1451 82 were found: 4331 1451 83 4331 1451 84 | l=0 | l=1 | l=2 | 4331 1451 85 --------------------------------------------- 4331 1451 86 R' (fm) | 6.74 | 7.72 | 7.94 | 4331 1451 87
(eV) | 12.0 | 6.21 | 4.38 | 4331 1451 88 Sl * 10E-4 | 0.48 | 5.13 | 0.52 | 4331 1451 89 (meV) | 142.2 | 116.1 | 142.2 | 4331 1451 90 4331 1451 91 The SAMMY/FITACS Hauser Feshbach average parameters have been 4331 1451 92 transformed into single level Breit Wigner average parameters 4331 1451 93 to comply with ENDF-6 format. 4331 1451 94 4331 1451 95 *************************** T H E O R Y **************************4331 1451 96 4331 1451 97 TALYS is a computer code system for the prediction and analysis 4331 1451 98 of nuclear reactions. TALYS simulates reactions that involve 4331 1451 99 neutrons, gamma-rays, protons, deuterons, tritons, helions and 4331 1451 100 alpha-particles, in the 1 keV - 200 MeV energy range and for 4331 1451 101 target nuclides of mass 12 and heavier. This is achieved by 4331 1451 102 implementing a suite of nuclear reaction models into a single 4331 1451 103 code system. It enables to evaluate nuclear reactions from 4331 1451 104 the unresolved resonance region up to intermediate energies. This 4331 1451 105 evaluation is based on a theoretical analysis that utilizes the 4331 1451 106 optical model, compound nucleus statistical theory, direct 4331 1451 107 reactions and pre-equilibrium processes, in combination with 4331 1451 108 databases and models for nuclear structure. For Tc-99, the 4331 1451 109 following output of TALYS is stored in this data file: 4331 1451 110 4331 1451 111 - Total, elastic and non-elastic cross sections 4331 1451 112 - Elastic scattering angular distributions 4331 1451 113 - Inelastic cross sections to discrete states 4331 1451 114 - Inelastic scattering angular distributions to discrete states 4331 1451 115 - Exclusive channel cross sections, e.g. (n,g), (n,2n), (n,np),.. 4331 1451 116 - Exclusive channel energy spectra 4331 1451 117 - Exclusive channel double-differential spectra 4331 1451 118 - Exclusive gamma production for discrete states and continuum 4331 1451 119 - Isomeric and ground state cross sections 4331 1451 120 - Residual production cross sections 4331 1451 121 - Total particle cross sections, e.g. (n,xn), (n,xp),.. 4331 1451 122 - Total particle energy spectra 4331 1451 123 - Total particle double-differential spectra 4331 1451 124 4331 1451 125 Here follows a short description of the used nuclear models: 4331 1451 126 4331 1451 127 ##### OPTICAL MODEL 4331 1451 128 4331 1451 129 All optical model calculations are performed by ECIS-97 [ray94], 4331 1451 130 in TALYS used as a subroutine. The default optical model 4331 1451 131 potentials (OMP) used are the local and global parameterizations 4331 1451 132 of Koning and Delaroche [kon03]. These are phenomenological OMPs 4331 1451 133 for neutrons and protons which in principle are valid over the 4331 1451 134 1 keV - 200 MeV energy range, though the low energy boundary of 4331 1451 135 validity may differ from nucleus to nucleus (e.g. for the total 4331 1451 136 cross sections, experimental data are included directly in the 4331 1451 137 file for energies below that boundary). Solving the Schroedinger 4331 1451 138 equation with this OMP yields the total cross section, the 4331 1451 139 shape-elastic cross section, the shape-elastic angular 4331 1451 140 distribution, the wave functions for the direct reaction cross 4331 1451 141 sections (see below), the transmission coefficients for the 4331 1451 142 compound nucleus model (see below) and the reaction cross 4331 1451 143 sections for the pre-equilibrium model (see below). 4331 1451 144 For neutrons and protons, the used parameterization is given in 4331 1451 145 Eq. (7) of [kon03]. 4331 1451 146 To calculate the transmission coefficients and reaction cross 4331 1451 147 sections for deuterons, tritons, helions and alpha particles, we 4331 1451 148 use OMPs that are directly derived from our nucleon potentials 4331 1451 149 using Watanabe's folding approach [mad88]. 4331 1451 150 4331 1451 151 ##### DIRECT REACTIONS 4331 1451 152 4331 1451 153 The built-in ECIS-97 is used for coupled-channels or DWBA 4331 1451 154 calculations for rotational or vibrational (or a combination of 4331 1451 155 these) nuclides. For Tc-99, DWBA was used to compute the direct 4331 1451 156 cross sections to several low-lying discrete levels of the 4331 1451 157 even-even core Mo-98. The weak-coupling model was then used 4331 1451 158 to spread the collective strength over the odd levels of Tc-99. 4331 1451 159 4331 1451 160 In addition, a macroscopic, phenomenological model to describe 4331 1451 161 giant resonances in the inelastic channel is used. For each 4331 1451 162 multipolarity an energy weighted sum rule applies and a DWBA 4331 1451 163 calculation with ECIS-97 is performed for each giant resonance 4331 1451 164 state. The cross section is then spread over the continuum with a 4331 1451 165 Gaussian distribution. 4331 1451 166 4331 1451 167 ##### COMPOUND NUCLEUS 4331 1451 168 4331 1451 169 For binary compound nucleus reactions we use the model of 4331 1451 170 Moldauer [mol80], i.e. the Hauser-Feshbach model [hau52] 4331 1451 171 corrected for width fluctuations. The transmission coefficients 4331 1451 172 have been generated with the aforementioned OMPs and the full 4331 1451 173 j,l-dependence of the transmission coefficients in the 4331 1451 174 Hauser-Feshbach model is used. For each nucleus that can be 4331 1451 175 reached through a binary reaction, several discrete levels and a 4331 1451 176 continuum described by level densities are included 4331 1451 177 simultaneously as competing channels. 4331 1451 178 4331 1451 179 The compound nucleus angular distributions are calculated with 4331 1451 180 the Blatt-Biedenharn formalism [bla52], leading to compound 4331 1451 181 nucleus Legendre coefficients that are added to their direct 4331 1451 182 counterparts. For multiple compound emission, i.e. emitted 4331 1451 183 particles after the binary emission, we use the Hauser-Feshbach 4331 1451 184 model. Again, for each residual nucleus several discrete states 4331 1451 185 are included as well as a continuum described by level densities. 4331 1451 186 Multiple compound emission is continued until all reaction 4331 1451 187 channels are closed and the population distribution of all 4331 1451 188 residual nuclides is depleted, through gamma decay, until they 4331 1451 189 end up in the ground state or in an isomer. 4331 1451 190 4331 1451 191 For the level density, we take the composite formula proposed by 4331 1451 192 Gilbert and Cameron [gil65], consisting of a constant temperature 4331 1451 193 law at low energies and a Fermi gas expression at high energies. 4331 1451 194 For the level density parameter a we use the energy dependent 4331 1451 195 expression proposed by Ignatyuk [ign75] to take into account the 4331 1451 196 damping of shell effects at high excitation energy. We have 4331 1451 197 obtained the parameters for the Ignatyuk formula from a 4331 1451 198 simultaneous fit to all experimental D_0 values as present in the 4331 1451 199 RIPL library. If necessary, we adjust individual parameters to 4331 1451 200 obtain a better fit to experiment. 4331 1451 201 4331 1451 202 Gamma-ray transmission coefficients are generated with the 4331 1451 203 Kopecky-Uhl generalized Lorentzian for strength 4331 1451 204 functions [kop90], with giant dipole resonance parameters taken 4331 1451 205 from the RIPL library [rip98], and normalized with experimental 4331 1451 206 radiative widths [gar84]. 4331 1451 207 4331 1451 208 ##### PRE-EQUILIBRIUM REACTIONS 4331 1451 209 4331 1451 210 For pre-equilibrium reactions, which become important for 4331 1451 211 incident energies above about 10 MeV, we use the two-component 4331 1451 212 exciton model [kon04b], in which the neutron or proton types of 4331 1451 213 particles and holes are followed throughout the reaction. For 4331 1451 214 energies above 20 MeV, multiple pre-equilibrium emission up to 4331 1451 215 any order of particle emission was included in the calculations. 4331 1451 216 A parameterization for the squared matrix element is used that is 4331 1451 217 valid for the whole energy range of this evaluation. 4331 1451 218 4331 1451 219 For deuterons, tritons, helions and alpha-particles, an extra 4331 1451 220 contribution was added from the pick/up and knock-out reaction 4331 1451 221 model by Kalbach [kal01]. 4331 1451 222 4331 1451 223 For photons, the model of Akkermans and Gruppelaar [akk85] was 4331 1451 224 applied, to simulate the direct and semi-direct capture 4331 1451 225 processes. 4331 1451 226 4331 1451 227 The angular distribution systematics by Kalbach [kal88] were used 4331 1451 228 to describe the angular distributions for all continuum 4331 1451 229 particles. An isotopic distribution for photons was adopted. 4331 1451 230 4331 1451 231 ****** C O M P A R I S O N W I T H E X P E R I M E N T *****4331 1451 232 4331 1451 233 This evaluation was performed simultaneously with other adjacent 4331 1451 234 isotopes, both for incident neutrons and protons. This enables, 4331 1451 235 when compared with a single-isotope effort, to put stronger 4331 1451 236 constraints on the produced calculated data, i.e. a globally 4331 1451 237 good comparison between TALYS and experimental data is requested 4331 1451 238 for all isotopes at the same time, while nucleus-specific input 4331 1451 239 (default or adjusted) parameters are consistently used for all 4331 1451 240 isotopes. Also, experimental data that is not available for the 4331 1451 241 isotope under study may be present, and tested, for adjacent 4331 1451 242 nuclides or for other projectiles. If these can be successfully 4331 1451 243 described by the models, a similar performance can be expected 4331 1451 244 for the present data file. 4331 1451 245 A few level density parameters for residual nuclides have been 4331 1451 246 adjusted to enforce agreement with the experimental data. The 4331 1451 247 changes in the level density parameters, a, were all kept within 4331 1451 248 10% of their default values. 4331 1451 249 4331 1451 250 ##### TOTAL AND REACTION CROSS SECTIONS AND ELASTIC SCATTERING 4331 1451 251 4331 1451 252 The spherical OMP was tested against experimental data for total 4331 1451 253 cross sections. The new total cross section measurements gives 4331 1451 254 rise to parameters That are slightly different from those of 4331 1451 255 [kon03]: 4331 1451 256 4331 1451 257 rv: 1.221 fm 4331 1451 258 av: 0.655 fm 4331 1451 259 v1: 53.7 MeV 4331 1451 260 v2: 0.0073 /MeV 4331 1451 261 v3: 0.000018 /(MeV**2) 4331 1451 262 w1: 13.5 MeV 4331 1451 263 w2: 80. MeV 4331 1451 264 rd: 1.304 fm 4331 1451 265 ad: 0.554 fm 4331 1451 266 d1: 16.1 MeV 4331 1451 267 d2: 0.0243 /MeV 4331 1451 268 d3: 9.40 MeV 4331 1451 269 rvso: 1.050 fm 4331 1451 270 avso: 0.580 fm 4331 1451 271 vso1: 6.2 MeV 4331 1451 272 vso2: 0.0040 /MeV 4331 1451 273 wso1: -3.1 MeV 4331 1451 274 wso2: 160. MeV 4331 1451 275 4331 1451 276 ##### INELASTIC CROSS SECTIONS 4331 1451 277 4331 1451 278 Various experimental data sets exist for the (n,n') reaction to 4331 1451 279 the isomeric state of Tc-99. The first peak is not described by 4331 1451 280 this evaluation, while the rest of the excitation function is 4331 1451 281 described by adjusting the spin cutoff factor to 0.45 times 4331 1451 282 its original value. 4331 1451 283 4331 1451 284 ##### OTHER PARTIAL CROSS SECTIONS 4331 1451 285 4331 1451 286 - (n,gamma): 4331 1451 287 4331 1451 288 The calculated capture cross section is renormalized, by 4331 1451 289 adjusting the level density parameter of the compound nucleus, 4331 1451 290 to the both the new and the available experimental data, the 4331 1451 291 latter taken from the EXFOR database. The pre-equilibrium gamma 4331 1451 292 cross section was adjusted to the data by multiplying the 4331 1451 293 calculated result by a factor of 2.0. 4331 1451 294 4331 1451 295 - (n,2n): 4331 1451 296 4331 1451 297 Only one experimental (n,2n) data point is available, at 14 MeV. 4331 1451 298 The present evaluation is higher than this point. 4331 1451 299 4331 1451 300 - (n,p): 4331 1451 301 4331 1451 302 The available experimental (n,p) cross sections are well 4331 1451 303 described. This could only be accomplished by adjusting the 4331 1451 304 single-particle level density parameters of Tc-100 and Mo-99. 4331 1451 305 4331 1451 306 - (n,a): 4331 1451 307 4331 1451 308 The available experimental (n,a) cross sections are well 4331 1451 309 described. This could only be accomplished by adjusting the 4331 1451 310 pick-up strength parameter of the (n,a) pre-equilibrium model. 4331 1451 311 4331 1451 312 - (n,na): 4331 1451 313 4331 1451 314 Some near-threshold data points exist, whcih are well described 4331 1451 315 by the current evaluation. 4331 1451 316 4331 1451 317 ##### PARTICLE SPECTRA 4331 1451 318 4331 1451 319 Experiments for neutron induced reaction spectra do not exist 4331 1451 320 for Tc-99. The closest nuclides for which spectral 4331 1451 321 information exists are Mo and Nb. Our global exciton model 4331 1451 322 analysis, however, has enabled us to constrain the results, 4331 1451 323 through the aforementioned matrix element, for particle yields 4331 1451 324 and double-differential spectra for all ejectiles up to alpha 4331 1451 325 particles. For Tc-99, an adjustment of the default matrix element 4331 1451 326 parameterization of [kon04b] for pre-equilibrium reactions of a 4331 1451 327 factor of 0.85 was needed, to describe the aforementioned cross 4331 1451 328 sections and emission spectra for nuclides in this mass range. 4331 1451 329 4331 1451 330 ***************** F I L E I N F O R M A T I O N ****************4331 1451 331 4331 1451 332 ##### MF1: GENERAL INFORMATION 4331 1451 333 4331 1451 334 - MT451 : Descriptive data and directory 4331 1451 335 4331 1451 336 This text and the full directory of used MF/MT sections. 4331 1451 337 4331 1451 338 ##### MF2: RESONANCE PARAMETERS 4331 1451 339 4331 1451 340 - MT151 : Resonance parameters 4331 1451 341 4331 1451 342 New resolved parameters are included. 4331 1451 343 They are given in the energy region from 1.0e-5 eV to 100 keV. 4331 1451 344 4331 1451 345 ##### MF3: REACTION CROSS SECTIONS 4331 1451 346 4331 1451 347 Unless stated otherwise, all the data present in the following 4331 1451 348 MT-sections have been calculated with TALYS. If the maximal cross 4331 1451 349 section in an excitation function over the whole energy range 4331 1451 350 does not exceed 1.e-9 b, the MT-number is not included at all. 4331 1451 351 Cross sections lower than 1.e-20 b are assumed to have no 4331 1451 352 physical meaning and are set to zero. 4331 1451 353 4331 1451 354 - MT1 : Total cross section 4331 1451 355 4331 1451 356 Above 100 keV, calculations from the spherical OMP were used. 4331 1451 357 4331 1451 358 - MT2 : Elastic scattering cross section 4331 1451 359 4331 1451 360 Obtained by subtracting the non-elastic cross section from the 4331 1451 361 total cross section. Below 100 keV, resonance parameters are 4331 1451 362 used. 4331 1451 363 4331 1451 364 - MT3 : Non-elastic cross section 4331 1451 365 4331 1451 366 Calculated with the optical model over the whole energy range. 4331 1451 367 Below 100 keV, resonance parameters are used. 4331 1451 368 4331 1451 369 - MT4 : Total inelastic cross section 4331 1451 370 4331 1451 371 Sum of MT=51-91. 4331 1451 372 4331 1451 373 - MT5 : (n,anything) cross section 4331 1451 374 4331 1451 375 For energies below 20 MeV, MT5 contains the lumped (n,gamma x) 4331 1451 376 cross section, where x may represent neutron, proton, deuteron, 4331 1451 377 triton, Helium-3 or alpha. Using the relative yields of MF6/MT5, 4331 1451 378 the (n,gamma n), (n,gamma p), ..., (n,gamma alpha) can be 4331 1451 379 recovered. These cross sections are relatively small. However, 4331 1451 380 addition of these cross sections, which can not be stored in any 4331 1451 381 other MT-number, ensures that the partial cross sections add up 4331 1451 382 to the non-elastic cross section. Above 20 MeV, MT5 contains the 4331 1451 383 total non-elastic cross section, with which the information of 4331 1451 384 MF6/MT5 can be combined to obtain particle production cross 4331 1451 385 sections and (double-)differential cross sections. 4331 1451 386 4331 1451 387 - MT16 : (n,2n) cross section 4331 1451 388 - MT17 : (n,3n) cross section 4331 1451 389 - MT22 : (n,na) cross section 4331 1451 390 - MT24 : (n,2na) cross section 4331 1451 391 - MT28 : (n,np) cross section 4331 1451 392 - MT32 : (n,nd) cross section 4331 1451 393 - MT33 : (n,nt) cross section 4331 1451 394 - MT41 : (n,2np) cross section 4331 1451 395 - MT51-70 : (n,n') cross section for 1st-20th excited state 4331 1451 396 - MT91 : (n,n') continuum cross section 4331 1451 397 - MT102 : (n,gamma) cross section 4331 1451 398 Below 100 keV, resonance parameters are used. 4331 1451 399 4331 1451 400 - MT103 : (n,p) cross section 4331 1451 401 - MT104 : (n,d) cross section 4331 1451 402 - MT105 : (n,t) cross section 4331 1451 403 - MT106 : (n,h) cross section 4331 1451 404 - MT107 : (n,a) cross section 4331 1451 405 - MT108 : (n,2a) cross section 4331 1451 406 - MT111 : (n,2p) cross section 4331 1451 407 - MT112 : (n,pa) cross section 4331 1451 408 - MT600-610: (n,p) cross section for 0th-10th excited state 4331 1451 409 4331 1451 410 Obtained by mapping continuum (n,p) cross section from 4331 1451 411 pre-equilibrium and compound model on discrete states. 4331 1451 412 4331 1451 413 - MT649 : (n,p) continuum cross section 4331 1451 414 - MT650-655: (n,d) cross section for 0th-5th excited state 4331 1451 415 4331 1451 416 Obtained by mapping continuum (n,d) cross section from 4331 1451 417 pre-equilibrium and compound model on discrete states. 4331 1451 418 4331 1451 419 - MT699 : (n,d) continuum cross section 4331 1451 420 - MT700-705: (n,t) cross section for 0th-5th excited state 4331 1451 421 4331 1451 422 Obtained by mapping continuum (n,t) cross section from 4331 1451 423 pre-equilibrium and compound model on discrete states. 4331 1451 424 4331 1451 425 - MT749 : (n,t) continuum cross section 4331 1451 426 - MT750-755: (n,h) cross section for 0th-5th excited state 4331 1451 427 4331 1451 428 Obtained by mapping continuum (n,h) cross section from 4331 1451 429 pre-equilibrium and compound model on discrete states. 4331 1451 430 4331 1451 431 - MT799 : (n,t) continuum cross section 4331 1451 432 - MT800-810: (n,a) cross section for 0th-10th excited state 4331 1451 433 4331 1451 434 Obtained by mapping continuum (n,a) cross section from 4331 1451 435 pre-equilibrium and compound model on discrete states. 4331 1451 436 4331 1451 437 - MT849 : (n,a) continuum cross section 4331 1451 438 4331 1451 439 ##### MF4: ANGULAR DISTRIBUTIONS OF SECONDARY PARTICLES 4331 1451 440 4331 1451 441 The versatility of MF6 for the storage of almost any secondary 4331 1451 442 distribution entails that we only use MF4 for the neutron elastic 4331 1451 443 scattering distribution. All data are generated with TALYS. 4331 1451 444 4331 1451 445 - MT2 : Elastic angular distribution 4331 1451 446 4331 1451 447 The flag LTT=3 is used to indicate a switch at 20 MeV from a 4331 1451 448 Legendre representation to a tabulated representation. For 4331 1451 449 incident energies below 20 MeV, the Legendre coefficients are 4331 1451 450 given on a sufficiently precise energy grid. They are a sum of 4331 1451 451 calculated Legendre coefficients for compound nucleus and 4331 1451 452 shape-elastic scattering. For incident energies above 20 MeV, 4331 1451 453 relative angular distributions are tabulated on an angular grid. 4331 1451 454 4331 1451 455 ##### MF6: PRODUCT ENERGY-ANGLE DISTRIBUTIONS 4331 1451 456 4331 1451 457 In MF6 we store all secondary energy, angle, and energy-angle 4331 1451 458 distributions, as well as all residual and discrete + continuum 4331 1451 459 photon production cross sections. We thus do not use MF12-15 for 4331 1451 460 the photon production that accompanies each reaction. All data 4331 1451 461 are generated with TALYS. 4331 1451 462 4331 1451 463 - MT5 : (n,anything) yields and energy-angle distributions 4331 1451 464 4331 1451 465 For energies below 20 MeV, MT5 contains the relative yields of 4331 1451 466 the (n,gamma x) reaction, where x may represent neutron, proton, 4331 1451 467 deuteron, triton, Helium-3 or alpha. Using the (n,gamma x) cross 4331 1451 468 section of MF3/MT3, the (n,gamma p), ..., (n,gamma alpha) cross 4331 1451 469 section can be recovered. For energies above 20 MeV, MT5 contains 4331 1451 470 the production yields of particles and residual products. It also 4331 1451 471 contains the secondary energy-angle distributions for all 4331 1451 472 particles and photons. First, the yields for neutrons are given 4331 1451 473 for the whole energy range. Next, on a secondary energy grid the 4331 1451 474 relative emission spectra are given together with the parameters 4331 1451 475 for the Kalbach systematics for angular distributions. Inelastic 4331 1451 476 scattering cross sections for discrete states have been broadened 4331 1451 477 and added to the continuum spectra. This procedure is repeated 4331 1451 478 for protons, deuterons, tritons, Helium-3, alpha particles and 4331 1451 479 photons. Finally, the residual production yields are given per 4331 1451 480 final product. All these yields and relative distributions can 4331 1451 481 be multiplied with the cross sections given in MF3/MT5 to get 4331 1451 482 the production cross sections and (double-)differential cross 4331 1451 483 sections. 4331 1451 484 4331 1451 485 - MT16 : (n,2n) energy-angle distr. and photon production 4331 1451 486 4331 1451 487 First, for each type of outgoing particle, the (trivial) integer 4331 1451 488 particle yields are given. Next, on a sufficiently dense incident 4331 1451 489 energy grid the secondary energy-angle distributions are 4331 1451 490 specified by means of the relative emission spectra and the 4331 1451 491 parameters for the Kalbach systematics for angular distributions. 4331 1451 492 Next, the photon yield is tabulated as a function of incident 4331 1451 493 energy. For each incident energy, the photon production is given 4331 1451 494 for all discrete gamma lines present in the final nucleus. A 4331 1451 495 continuum photon distribution is added to this. We assume 4331 1451 496 isotropy for all produced gamma rays. 4331 1451 497 4331 1451 498 For the following MT-numbers, the same procedure as for MT16 is 4331 1451 499 followed: 4331 1451 500 ----- 4331 1451 501 - MT17 : (n,3n) energy-angle distr. and photon production 4331 1451 502 - MT22 : (n,na) energy-angle distr. and photon production 4331 1451 503 - MT24 : (n,2na) energy-angle distr. and photon production 4331 1451 504 - MT28 : (n,np) energy-angle distr. and photon production 4331 1451 505 - MT32 : (n,nd) energy-angle distr. and photon production 4331 1451 506 - MT33 : (n,nt) energy-angle distr. and photon production 4331 1451 507 - MT41 : (n,2np) energy-angle distr. and photon production 4331 1451 508 - MT91 : (n,n') continuum energy-angle distr. and phot. prod. 4331 1451 509 - MT102 : (n,gamma) photon production 4331 1451 510 - MT108 : (n,2a) energy-angle distr. and photon production 4331 1451 511 - MT111 : (n,2p) energy-angle distr. and photon production 4331 1451 512 - MT112 : (n,pa) energy-angle distr. and photon production 4331 1451 513 - MT649 : (n,p) continuum energy-angle distr. and photon prod. 4331 1451 514 - MT699 : (n,d) continuum energy-angle distr. and photon prod. 4331 1451 515 - MT749 : (n,t) continuum energy-angle distr. and photon prod. 4331 1451 516 - MT849 : (n,a) continuum energy-angle distr. and photon prod. 4331 1451 517 ----- 4331 1451 518 4331 1451 519 - MT51 : (n,n') angular distribution and photon production 4331 1451 520 for first excited state 4331 1451 521 4331 1451 522 The angular distribution for inelastic scattering to the first 4331 1451 523 inelastic state is given with Legendre coefficients up to 20 MeV. 4331 1451 524 Next, the exclusive yields for all the discrete gamma rays that 4331 1451 525 originate from this particular level are given. 4331 1451 526 4331 1451 527 For the following MT-numbers, the same procedure as for MT51 is 4331 1451 528 followed: 4331 1451 529 ----- 4331 1451 530 - MT52-70 : (n,n') angular distribution and photon production 4331 1451 531 for 2nd-20th excited state 4331 1451 532 - MT600-610: (n,p) angular distribution and photon production 4331 1451 533 for 0th-10th excited state 4331 1451 534 - MT650-655: (n,d) angular distribution and photon production 4331 1451 535 for 0th-5th excited state 4331 1451 536 - MT700-705: (n,t) angular distribution and photon production 4331 1451 537 for 0th-5th excited state 4331 1451 538 - MT750-755: (n,h) angular distribution and photon production 4331 1451 539 for 0th-5th excited state 4331 1451 540 - MT800-810: (n,a) angular distribution and photon production 4331 1451 541 for 0th-10th excited state 4331 1451 542 ----- 4331 1451 543 4331 1451 544 ##### MF8: RADIOACTIVE DECAY DATA 4331 1451 545 4331 1451 546 For reactions to isomers, MF8 designates where the information 4331 1451 547 for isomeric versus ground state production can be found, i.e. 4331 1451 548 for each MT number it points to either MF6, MF9 or MF10. 4331 1451 549 4331 1451 550 ##### MF10: CROSS SECTIONS FOR PRODUCTION OF RADIOACTIVE NUCLIDES 4331 1451 551 4331 1451 552 All data are generated with TALYS. Final states with a lifetime 4331 1451 553 that exceeds 1 second are treated as isomer. 4331 1451 554 4331 1451 555 - MT4 : (n,n') cross section to ground state and isomer 4331 1451 556 - MT17 : (n,3n) cross section to ground state and isomer 4331 1451 557 - MT22 : (n,a) cross section to ground state and isomer 4331 1451 558 - MT24 : (n,2na) cross section to ground state and isomer 4331 1451 559 - MT106 : (n,h) cross section to ground state and isomer 4331 1451 560 - MT111 : (n,2p) cross section to ground state and isomer 4331 1451 561 4331 1451 562 ***** F I L E C H E C K I N G A N D P R O C E S S I N G ****4331 1451 563 4331 1451 564 This file has been checked successfully by the BNL checking 4331 1451 565 codes CHECKR-6.12, FIZCON-6.12 and PSYCHE-6.12 [dun01] and has 4331 1451 566 been processed successfully into an MCNP library by the 4331 1451 567 processing code NJOY99.81 [mac00]. 4331 1451 568 4331 1451 569 *********************** R E F E R E N C E S **********************4331 1451 570 4331 1451 571 [akk85] J.M. Akkermans and H. Gruppelaar, Phys. Lett. 157B, 95 4331 1451 572 (1985). 4331 1451 573 [bla52] J.M. Blatt and L.C. Biedenharn, Rev. Mod. Phys. 52, 725 4331 1451 574 (1952). 4331 1451 575 [dun01] C. Dunford, ENDF Utility Codes Release 6.12, (2001). 4331 1451 576 [fur04] K. Furutaka, Nucl. Data. Sci. Tech., Santa Fe (2004) 4331 1451 577 [gar84] D.G. Gardner, in Neutron Radiative Capture, OECD/NEA 4331 1451 578 Series on Neutron Physics and Nuclear Data in Science and 4331 1451 579 Technology, eds. A. Michaudon et al., p. 62 (1984). 4331 1451 580 [gil65] A. Gilbert and A.G.W. Cameron, Can. J. Phys. 43, 1446 4331 1451 581 (1965). 4331 1451 582 [gun00] F. Gunsing et al. Phys. Rev. C61 (2000) 054608 4331 1451 583 [gun01] F. Gunsing et al. Nuclear Physics A688 (2001) 496c 4331 1451 584 [hau52] W. Hauser and H. Feshbach, Phys. Rev. 87, 366 (1952). 4331 1451 585 [ign75] A.V. Ignatyuk, G.N. Smirenkin, and A.S. Tishin, Sov. J. 4331 1451 586 Nucl. Phys. 21, no. 3, 255 (1975). 4331 1451 587 [kal88] C. Kalbach, Phys. Rev. C37, 2350 (1988). 4331 1451 588 [kal01] C. Kalbach, PRECO-2000: Exciton model pre-equilibrium 4331 1451 589 code with direct reactions, Duke University 2001, 4331 1451 590 www.nndc.bnl.gov/nndcscr/model-codes/preco-2000/. 4331 1451 591 [kon03] A.J. Koning and J.P. Delaroche, Nucl. Phys. A713, 231 4331 1451 592 (2003). 4331 1451 593 [kon04] A.J. Koning, S. Hilaire and M.C. Duijvestijn, ND2004 4331 1451 594 conference, Santa Fe (2004). 4331 1451 595 [kon04b] A.J. Koning and M.C. Duijvestijn, Nucl. Phys. A744, 15 4331 1451 596 (2004). 4331 1451 597 [kop90] J. Kopecky and M. Uhl, Phys. Rev. C42, 1941 (1990). 4331 1451 598 [lar03] N. M. L. Larson, SAMMY: Multilevel R-Matrix Fits To 4331 1451 599 Neutron Data Using Bayes Equation, ORNL/TM-9179/R6 (2003) 4331 1451 600 [mac00] R.E. Macfarlane, NJOY99 - Code system for producing 4331 1451 601 pointwise and multigroup neutron and photon cross 4331 1451 602 sections from ENDF/B Data, RSIC PSR-480 (2000). 4331 1451 603 [mad88] D.G. Madland, in Proceedings of a Specialists' Meeting on 4331 1451 604 Preequilibrium Reactions, Semmering, Austria, 4331 1451 605 February 10-12 1988, (OECD, Paris 1988), p. 103. 4331 1451 606 [mol80] P.A. Moldauer, Nucl. Phys. A344, 185 (1980). 4331 1451 607 [ray94] J. Raynal, Notes on ECIS94, CEA Saclay Report 4331 1451 608 No. CEA-N-2772, 1994. 4331 1451 609 [rip98] Handbook for calculations of nuclear reaction data: 4331 1451 610 Reference Input Parameter Library, IAEA-TECDOC-1034 4331 1451 611 (1998). 4331 1451 612 4331 1451 613 ************************* C O N T E N T S ************************4331 1451 614 4331 1451 615 1 451 797 14331 1451 616 2 151 836 14331 1451 617 3 1 108 14331 1451 618 3 2 108 14331 1451 619 3 3 108 14331 1451 620 3 4 32 14331 1451 621 3 5 69 14331 1451 622 3 16 10 14331 1451 623 3 17 6 14331 1451 624 3 22 15 14331 1451 625 3 24 7 14331 1451 626 3 28 13 14331 1451 627 3 32 7 14331 1451 628 3 33 7 14331 1451 629 3 41 6 14331 1451 630 3 51 32 14331 1451 631 3 52 31 14331 1451 632 3 53 31 14331 1451 633 3 54 29 14331 1451 634 3 55 29 14331 1451 635 3 56 29 14331 1451 636 3 57 28 14331 1451 637 3 58 28 14331 1451 638 3 59 27 14331 1451 639 3 60 27 14331 1451 640 3 61 26 14331 1451 641 3 62 26 14331 1451 642 3 63 26 14331 1451 643 3 64 25 14331 1451 644 3 65 24 14331 1451 645 3 66 24 14331 1451 646 3 67 23 14331 1451 647 3 68 23 14331 1451 648 3 69 23 14331 1451 649 3 70 22 14331 1451 650 3 91 22 14331 1451 651 3 102 27 14331 1451 652 3 103 23 14331 1451 653 3 104 16 14331 1451 654 3 105 11 14331 1451 655 3 106 9 14331 1451 656 3 107 29 14331 1451 657 3 108 29 14331 1451 658 3 111 8 14331 1451 659 3 112 11 14331 1451 660 3 600 23 14331 1451 661 3 601 23 14331 1451 662 3 602 22 14331 1451 663 3 603 22 14331 1451 664 3 604 22 14331 1451 665 3 605 22 14331 1451 666 3 606 22 14331 1451 667 3 607 22 14331 1451 668 3 608 22 14331 1451 669 3 609 22 14331 1451 670 3 610 21 14331 1451 671 3 649 21 14331 1451 672 3 650 16 14331 1451 673 3 651 15 14331 1451 674 3 652 15 14331 1451 675 3 653 14 14331 1451 676 3 654 13 14331 1451 677 3 655 13 14331 1451 678 3 699 12 14331 1451 679 3 700 11 14331 1451 680 3 701 11 14331 1451 681 3 702 11 14331 1451 682 3 703 11 14331 1451 683 3 704 11 14331 1451 684 3 705 11 14331 1451 685 3 749 11 14331 1451 686 3 750 9 14331 1451 687 3 751 8 14331 1451 688 3 752 8 14331 1451 689 3 753 8 14331 1451 690 3 754 8 14331 1451 691 3 755 8 14331 1451 692 3 799 7 14331 1451 693 3 800 29 14331 1451 694 3 801 29 14331 1451 695 3 802 29 14331 1451 696 3 803 29 14331 1451 697 3 804 29 14331 1451 698 3 805 29 14331 1451 699 3 806 29 14331 1451 700 3 807 29 14331 1451 701 3 808 29 14331 1451 702 3 809 29 14331 1451 703 3 810 29 14331 1451 704 3 849 29 14331 1451 705 4 2 1230 14331 1451 706 6 5 9453 14331 1451 707 6 16 439 14331 1451 708 6 17 134 14331 1451 709 6 22 896 14331 1451 710 6 24 252 14331 1451 711 6 28 770 14331 1451 712 6 32 274 14331 1451 713 6 33 261 14331 1451 714 6 41 199 14331 1451 715 6 51 157 14331 1451 716 6 52 142 14331 1451 717 6 53 154 14331 1451 718 6 54 147 14331 1451 719 6 55 148 14331 1451 720 6 56 151 14331 1451 721 6 57 147 14331 1451 722 6 58 151 14331 1451 723 6 59 146 14331 1451 724 6 60 147 14331 1451 725 6 61 147 14331 1451 726 6 62 147 14331 1451 727 6 63 147 14331 1451 728 6 64 150 14331 1451 729 6 65 142 14331 1451 730 6 66 148 14331 1451 731 6 67 148 14331 1451 732 6 68 137 14331 1451 733 6 69 144 14331 1451 734 6 70 145 14331 1451 735 6 91 1510 14331 1451 736 6 102 1072 14331 1451 737 6 108 409 14331 1451 738 6 111 227 14331 1451 739 6 112 630 14331 1451 740 6 600 74 14331 1451 741 6 601 87 14331 1451 742 6 602 87 14331 1451 743 6 603 80 14331 1451 744 6 604 82 14331 1451 745 6 605 82 14331 1451 746 6 606 88 14331 1451 747 6 607 82 14331 1451 748 6 608 84 14331 1451 749 6 609 86 14331 1451 750 6 610 84 14331 1451 751 6 649 1127 14331 1451 752 6 650 59 14331 1451 753 6 651 64 14331 1451 754 6 652 66 14331 1451 755 6 653 64 14331 1451 756 6 654 64 14331 1451 757 6 655 68 14331 1451 758 6 699 497 14331 1451 759 6 700 44 14331 1451 760 6 701 53 14331 1451 761 6 702 53 14331 1451 762 6 703 52 14331 1451 763 6 704 53 14331 1451 764 6 705 53 14331 1451 765 6 749 361 14331 1451 766 6 750 34 14331 1451 767 6 751 34 14331 1451 768 6 752 43 14331 1451 769 6 753 43 14331 1451 770 6 754 43 14331 1451 771 6 755 43 14331 1451 772 6 799 156 14331 1451 773 6 800 89 14331 1451 774 6 801 97 14331 1451 775 6 802 98 14331 1451 776 6 803 97 14331 1451 777 6 804 98 14331 1451 778 6 805 99 14331 1451 779 6 806 99 14331 1451 780 6 807 99 14331 1451 781 6 808 99 14331 1451 782 6 809 101 14331 1451 783 6 810 98 14331 1451 784 6 849 1255 14331 1451 785 8 4 3 14331 1451 786 8 17 3 14331 1451 787 8 22 3 14331 1451 788 8 24 3 14331 1451 789 8 106 3 14331 1451 790 8 111 3 14331 1451 791 10 4 49 14331 1451 792 10 17 11 14331 1451 793 10 22 28 14331 1451 794 10 24 13 14331 1451 795 10 106 15 14331 1451 796 10 111 13 14331 1451 797 4331 1 099999 4331 0 0 0 4.309900+4 9.805661+1 0 0 1 04331 2151 1 4.309900+4 1.000000+0 0 0 2 04331 2151 2 1.000000-5 6.000000+3 1 3 0 04331 2151 3 4.500000+0 7.300000-1 1 0 2 44331 2151 4 9.805660+1 0.000000+0 0 0 3234 5394331 2151 5 -1.661500+1 5.000000+0 1.337600-2 1.500000-1 0.000000+0 0.000000+04331 2151 6 5.584112+0 5.000000+0 3.310000-3 1.465000-1 0.000000+0 0.000000+04331 2151 7 2.027373+1 4.000000+0 8.365000-3 1.550000-1 0.000000+0 0.000000+04331 2151 8 3.984120+1 5.000000+0 1.082000-3 1.227000-1 0.000000+0 0.000000+04331 2151 9 5.667611+1 4.000000+0 3.902000-3 1.411000-1 0.000000+0 0.000000+04331 2151 10 1.112162+2 5.000000+0 9.938000-3 1.343000-1 0.000000+0 0.000000+04331 2151 11 1.237742+2 4.000000+0 4.105000-3 1.451000-1 0.000000+0 0.000000+04331 2151 12 1.630090+2 5.000000+0 5.782000-2 1.443000-1 0.000000+0 0.000000+04331 2151 13 1.820893+2 4.000000+0 6.733000-2 1.604000-1 0.000000+0 0.000000+04331 2151 14 1.917136+2 5.000000+0 3.640000-2 1.488000-1 0.000000+0 0.000000+04331 2151 15 2.064052+2 4.000000+0 6.903000-4 1.469000-1 0.000000+0 0.000000+04331 2151 16 2.148314+2 4.000000+0 1.192000-3 1.469000-1 0.000000+0 0.000000+04331 2151 17 2.412085+2 4.000000+0 3.794000-2 1.469000-1 0.000000+0 0.000000+04331 2151 18 2.799765+2 4.000000+0 1.502000-2 1.469000-1 0.000000+0 0.000000+04331 2151 19 2.999795+2 4.000000+0 3.694000-2 1.469000-1 0.000000+0 0.000000+04331 2151 20 3.068103+2 5.000000+0 1.432000-2 1.469000-1 0.000000+0 0.000000+04331 2151 21 3.432065+2 5.000000+0 1.619000-3 1.469000-1 0.000000+0 0.000000+04331 2151 22 3.586493+2 4.000000+0 1.961000-2 1.469000-1 0.000000+0 0.000000+04331 2151 23 3.626885+2 4.000000+0 1.967000-3 1.469000-1 0.000000+0 0.000000+04331 2151 24 3.649311+2 5.000000+0 1.424000-1 1.469000-1 0.000000+0 0.000000+04331 2151 25 3.798448+2 5.000000+0 2.094000-2 1.469000-1 0.000000+0 0.000000+04331 2151 26 4.168151+2 4.000000+0 6.438000-2 1.469000-1 0.000000+0 0.000000+04331 2151 27 4.265422+2 5.000000+0 6.085000-2 1.469000-1 0.000000+0 0.000000+04331 2151 28 4.476964+2 5.000000+0 2.219000-3 1.469000-1 0.000000+0 0.000000+04331 2151 29 4.599157+2 4.000000+0 4.182000-2 1.469000-1 0.000000+0 0.000000+04331 2151 30 4.787740+2 4.000000+0 1.272000-2 1.469000-1 0.000000+0 0.000000+04331 2151 31 4.865752+2 5.000000+0 5.354000-3 1.469000-1 0.000000+0 0.000000+04331 2151 32 5.164460+2 4.000000+0 1.315000-2 1.469000-1 0.000000+0 0.000000+04331 2151 33 5.205616+2 5.000000+0 2.953000-2 1.469000-1 0.000000+0 0.000000+04331 2151 34 5.366115+2 4.000000+0 3.045000-2 1.469000-1 0.000000+0 0.000000+04331 2151 35 5.632300+2 5.000000+0 7.969000-3 1.469000-1 0.000000+0 0.000000+04331 2151 36 5.937529+2 4.000000+0 6.196000-3 1.469000-1 0.000000+0 0.000000+04331 2151 37 5.981673+2 5.000000+0 2.611000-2 1.469000-1 0.000000+0 0.000000+04331 2151 38 5.995356+2 5.000000+0 3.262000-3 1.469000-1 0.000000+0 0.000000+04331 2151 39 6.067632+2 4.000000+0 3.760000-2 1.469000-1 0.000000+0 0.000000+04331 2151 40 6.234865+2 4.000000+0 5.491000-3 1.469000-1 0.000000+0 0.000000+04331 2151 41 6.325616+2 5.000000+0 2.394000-3 1.469000-1 0.000000+0 0.000000+04331 2151 42 6.547070+2 4.000000+0 4.647000-2 1.469000-1 0.000000+0 0.000000+04331 2151 43 6.722419+2 5.000000+0 2.150000-2 1.469000-1 0.000000+0 0.000000+04331 2151 44 6.862344+2 5.000000+0 5.214000-3 1.469000-1 0.000000+0 0.000000+04331 2151 45 7.240934+2 5.000000+0 8.266000-3 1.469000-1 0.000000+0 0.000000+04331 2151 46 7.453717+2 4.000000+0 1.147000-1 1.469000-1 0.000000+0 0.000000+04331 2151 47 7.536044+2 4.000000+0 6.296000-2 1.469000-1 0.000000+0 0.000000+04331 2151 48 7.660865+2 4.000000+0 1.087000-2 1.469000-1 0.000000+0 0.000000+04331 2151 49 7.745066+2 5.000000+0 2.893000-3 1.469000-1 0.000000+0 0.000000+04331 2151 50 7.986370+2 4.000000+0 4.823000-3 1.469000-1 0.000000+0 0.000000+04331 2151 51 8.055910+2 5.000000+0 2.743000-2 1.469000-1 0.000000+0 0.000000+04331 2151 52 8.159134+2 5.000000+0 2.464000-2 1.469000-1 0.000000+0 0.000000+04331 2151 53 8.280426+2 4.000000+0 3.959000-3 1.469000-1 0.000000+0 0.000000+04331 2151 54 8.387140+2 4.000000+0 1.191000-1 1.469000-1 0.000000+0 0.000000+04331 2151 55 8.472872+2 4.000000+0 6.067000-2 1.469000-1 0.000000+0 0.000000+04331 2151 56 8.735925+2 4.000000+0 5.899000-3 1.469000-1 0.000000+0 0.000000+04331 2151 57 8.759186+2 5.000000+0 1.293000-2 1.469000-1 0.000000+0 0.000000+04331 2151 58 8.927197+2 4.000000+0 1.393000-1 1.469000-1 0.000000+0 0.000000+04331 2151 59 9.269975+2 4.000000+0 4.717000-3 1.469000-1 0.000000+0 0.000000+04331 2151 60 9.717974+2 5.000000+0 1.075000-2 1.469000-1 0.000000+0 0.000000+04331 2151 61 9.946610+2 4.000000+0 5.225000-2 1.469000-1 0.000000+0 0.000000+04331 2151 62 1.020947+3 5.000000+0 2.184000-2 1.469000-1 0.000000+0 0.000000+04331 2151 63 1.045537+3 4.000000+0 3.883000-2 1.469000-1 0.000000+0 0.000000+04331 2151 64 1.047072+3 4.000000+0 1.484000-2 1.469000-1 0.000000+0 0.000000+04331 2151 65 1.072503+3 5.000000+0 1.439000-1 1.469000-1 0.000000+0 0.000000+04331 2151 66 1.083817+3 5.000000+0 3.113000-1 1.469000-1 0.000000+0 0.000000+04331 2151 67 1.089320+3 4.000000+0 6.442000-3 1.469000-1 0.000000+0 0.000000+04331 2151 68 1.105431+3 5.000000+0 4.505000-3 1.469000-1 0.000000+0 0.000000+04331 2151 69 1.111537+3 4.000000+0 5.320000-3 1.469000-1 0.000000+0 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1.534509+6 3.230421-9 0.000000+04331 6 5 1792 1.633509+6 6.749201-9 0.000000+0 1.732510+6 1.299861-8 0.000000+04331 6 5 1793 1.831510+6 2.358396-8 0.000000+0 1.930511+6 4.263064-8 0.000000+04331 6 5 1794 2.079012+6 9.770370-8 0.000000+0 2.277013+6 1.930098-7 0.000000+04331 6 5 1795 2.475014+6 3.157710-7 0.000000+0 2.673015+6 4.725410-7 0.000000+04331 6 5 1796 2.871017+6 6.079660-7 0.000000+0 3.069018+6 6.867647-7 0.000000+04331 6 5 1797 3.267019+6 7.147526-7 0.000000+0 3.465020+6 6.507834-7 0.000000+04331 6 5 1798 3.663021+6 5.142272-7 0.000000+0 3.861022+6 3.200129-7 0.000000+04331 6 5 1799 4.207524+6 7.121944-8 0.000000+0 4.702527+6 1.015798-9 0.000000+04331 6 5 1800 5.197530+6 1.00000-36 0.000000+0 4331 6 5 1801 0.000000+0 6.200000+6 0 1 96 324331 6 5 1802 2.475014+5 1.00000-36 0.000000+0 3.465020+5 1.58614-21 0.000000+04331 6 5 1803 4.455026+5 3.28742-19 0.000000+0 5.445031+5 2.92798-17 0.000000+04331 6 5 1804 6.435037+5 1.01003-15 0.000000+0 7.425043+5 1.74468-14 0.000000+04331 6 5 1805 8.415048+5 1.83598-13 0.000000+0 9.405054+5 1.31907-12 0.000000+04331 6 5 1806 1.039506+6 7.06591-12 0.000000+0 1.138507+6 3.03679-11 0.000000+04331 6 5 1807 1.237507+6 1.06237-10 0.000000+0 1.336508+6 3.17195-10 0.000000+04331 6 5 1808 1.435508+6 8.26802-10 0.000000+0 1.534509+6 1.922988-9 0.000000+04331 6 5 1809 1.633509+6 4.126811-9 0.000000+0 1.732510+6 8.065507-9 0.000000+04331 6 5 1810 1.831510+6 1.467635-8 0.000000+0 1.930511+6 2.721321-8 0.000000+04331 6 5 1811 2.079012+6 6.304315-8 0.000000+0 2.277013+6 1.272368-7 0.000000+04331 6 5 1812 2.475014+6 2.242966-7 0.000000+0 2.673015+6 3.376657-7 0.000000+04331 6 5 1813 2.871017+6 4.696068-7 0.000000+0 3.069018+6 5.722931-7 0.000000+04331 6 5 1814 3.267019+6 6.444584-7 0.000000+0 3.465020+6 6.573372-7 0.000000+04331 6 5 1815 3.663021+6 5.914005-7 0.000000+0 3.861022+6 4.604544-7 0.000000+04331 6 5 1816 4.207524+6 1.865753-7 0.000000+0 4.702527+6 2.211917-8 0.000000+04331 6 5 1817 5.197530+6 6.27373-11 0.000000+0 5.692533+6 1.00000-36 0.000000+04331 6 5 1818 0.000000+0 6.600000+6 0 1 96 324331 6 5 1819 2.475014+5 1.00000-36 0.000000+0 3.465020+5 1.16374-21 0.000000+04331 6 5 1820 4.455026+5 2.13238-19 0.000000+0 5.445031+5 1.77649-17 0.000000+04331 6 5 1821 6.435037+5 6.06622-16 0.000000+0 7.425043+5 1.05378-14 0.000000+04331 6 5 1822 8.415048+5 1.12748-13 0.000000+0 9.405054+5 8.17392-13 0.000000+04331 6 5 1823 1.039506+6 4.43523-12 0.000000+0 1.138507+6 1.90129-11 0.000000+04331 6 5 1824 1.237507+6 6.67802-11 0.000000+0 1.336508+6 2.01782-10 0.000000+04331 6 5 1825 1.435508+6 5.25981-10 0.000000+0 1.534509+6 1.250866-9 0.000000+04331 6 5 1826 1.633509+6 2.669208-9 0.000000+0 1.732510+6 5.250050-9 0.000000+04331 6 5 1827 1.831510+6 9.634821-9 0.000000+0 1.930511+6 1.831104-8 0.000000+04331 6 5 1828 2.079012+6 4.264390-8 0.000000+0 2.277013+6 8.932307-8 0.000000+04331 6 5 1829 2.475014+6 1.589170-7 0.000000+0 2.673015+6 2.539651-7 0.000000+04331 6 5 1830 2.871017+6 3.585329-7 0.000000+0 3.069018+6 4.675957-7 0.000000+04331 6 5 1831 3.267019+6 5.487237-7 0.000000+0 3.465020+6 6.021398-7 0.000000+04331 6 5 1832 3.663021+6 5.947524-7 0.000000+0 3.861022+6 5.344269-7 0.000000+04331 6 5 1833 4.207524+6 3.051486-7 0.000000+0 4.702527+6 7.961012-8 0.000000+04331 6 5 1834 5.197530+6 5.277417-9 0.000000+0 5.692533+6 1.00000-36 0.000000+04331 6 5 1835 0.000000+0 7.000000+6 0 1 99 334331 6 5 1836 2.475014+5 1.00000-36 0.000000+0 3.465020+5 8.31046-22 0.000000+04331 6 5 1837 4.455026+5 1.48800-19 0.000000+0 5.445031+5 1.19764-17 0.000000+04331 6 5 1838 6.435037+5 3.90772-16 0.000000+0 7.425043+5 6.87951-15 0.000000+04331 6 5 1839 8.415048+5 7.36412-14 0.000000+0 9.405054+5 5.45813-13 0.000000+04331 6 5 1840 1.039506+6 2.93348-12 0.000000+0 1.138507+6 1.26246-11 0.000000+04331 6 5 1841 1.237507+6 4.46138-11 0.000000+0 1.336508+6 1.35689-10 0.000000+04331 6 5 1842 1.435508+6 3.57857-10 0.000000+0 1.534509+6 8.50288-10 0.000000+04331 6 5 1843 1.633509+6 1.823885-9 0.000000+0 1.732510+6 3.619674-9 0.000000+04331 6 5 1844 1.831510+6 6.732511-9 0.000000+0 1.930511+6 1.266466-8 0.000000+04331 6 5 1845 2.079012+6 3.036027-8 0.000000+0 2.277013+6 6.438548-8 0.000000+04331 6 5 1846 2.475014+6 1.182729-7 0.000000+0 2.673015+6 1.916877-7 0.000000+04331 6 5 1847 2.871017+6 2.819435-7 0.000000+0 3.069018+6 3.755198-7 0.000000+04331 6 5 1848 3.267019+6 4.653111-7 0.000000+0 3.465020+6 5.278416-7 0.000000+04331 6 5 1849 3.663021+6 5.629481-7 0.000000+0 3.861022+6 5.462262-7 0.000000+04331 6 5 1850 4.207524+6 3.957230-7 0.000000+0 4.702527+6 1.589895-7 0.000000+04331 6 5 1851 5.197530+6 2.855041-8 0.000000+0 5.692533+6 7.45493-10 0.000000+04331 6 5 1852 6.187536+6 1.00000-36 0.000000+0 4331 6 5 1853 0.000000+0 7.400000+6 0 1 102 344331 6 5 1854 2.475014+5 1.00000-36 0.000000+0 3.465020+5 6.66516-22 0.000000+04331 6 5 1855 4.455026+5 1.12708-19 0.000000+0 5.445031+5 8.25707-18 0.000000+04331 6 5 1856 6.435037+5 2.79611-16 0.000000+0 7.425043+5 4.75920-15 0.000000+04331 6 5 1857 8.415048+5 5.11547-14 0.000000+0 9.405054+5 3.83491-13 0.000000+04331 6 5 1858 1.039506+6 2.09273-12 0.000000+0 1.138507+6 8.95708-12 0.000000+04331 6 5 1859 1.237507+6 3.15158-11 0.000000+0 1.336508+6 9.67324-11 0.000000+04331 6 5 1860 1.435508+6 2.56566-10 0.000000+0 1.534509+6 6.10379-10 0.000000+04331 6 5 1861 1.633509+6 1.317412-9 0.000000+0 1.732510+6 2.623865-9 0.000000+04331 6 5 1862 1.831510+6 4.923214-9 0.000000+0 1.930511+6 9.315626-9 0.000000+04331 6 5 1863 2.079012+6 2.247400-8 0.000000+0 2.277013+6 4.861561-8 0.000000+04331 6 5 1864 2.475014+6 9.026578-8 0.000000+0 2.673015+6 1.497052-7 0.000000+04331 6 5 1865 2.871017+6 2.220158-7 0.000000+0 3.069018+6 3.081293-7 0.000000+04331 6 5 1866 3.267019+6 3.874692-7 0.000000+0 3.465020+6 4.615447-7 0.000000+04331 6 5 1867 3.663021+6 5.044960-7 0.000000+0 3.861022+6 5.304830-7 0.000000+04331 6 5 1868 4.207524+6 4.450555-7 0.000000+0 4.702527+6 2.405758-7 0.000000+04331 6 5 1869 5.197530+6 7.254567-8 0.000000+0 5.692533+6 7.945511-9 0.000000+04331 6 5 1870 6.187536+6 7.47061-11 0.000000+0 6.682538+6 1.00000-36 0.000000+04331 6 5 1871 0.000000+0 7.800000+6 0 1 105 354331 6 5 1872 2.475014+5 1.00000-36 0.000000+0 3.465020+5 5.23802-22 0.000000+04331 6 5 1873 4.455026+5 9.27290-20 0.000000+0 5.445031+5 6.33329-18 0.000000+04331 6 5 1874 6.435037+5 2.02073-16 0.000000+0 7.425043+5 3.62668-15 0.000000+04331 6 5 1875 8.415048+5 3.82514-14 0.000000+0 9.405054+5 2.78219-13 0.000000+04331 6 5 1876 1.039506+6 1.56523-12 0.000000+0 1.138507+6 6.74331-12 0.000000+04331 6 5 1877 1.237507+6 2.38148-11 0.000000+0 1.336508+6 7.28315-11 0.000000+04331 6 5 1878 1.435508+6 1.94686-10 0.000000+0 1.534509+6 4.64681-10 0.000000+04331 6 5 1879 1.633509+6 9.99674-10 0.000000+0 1.732510+6 2.007113-9 0.000000+04331 6 5 1880 1.831510+6 3.792679-9 0.000000+0 1.930511+6 7.199830-9 0.000000+04331 6 5 1881 2.079012+6 1.748564-8 0.000000+0 2.277013+6 3.832868-8 0.000000+04331 6 5 1882 2.475014+6 7.119798-8 0.000000+0 2.673015+6 1.209544-7 0.000000+04331 6 5 1883 2.871017+6 1.826936-7 0.000000+0 3.069018+6 2.562696-7 0.000000+04331 6 5 1884 3.267019+6 3.314340-7 0.000000+0 3.465020+6 3.984423-7 0.000000+04331 6 5 1885 3.663021+6 4.581099-7 0.000000+0 3.861022+6 4.948731-7 0.000000+04331 6 5 1886 4.207524+6 4.653124-7 0.000000+0 4.702527+6 3.024005-7 0.000000+04331 6 5 1887 5.197530+6 1.236602-7 0.000000+0 5.692533+6 2.683708-8 0.000000+04331 6 5 1888 6.187536+6 1.925348-9 0.000000+0 6.682538+6 4.52241-12 0.000000+04331 6 5 1889 7.177542+6 1.00000-36 0.000000+0 4331 6 5 1890 0.000000+0 8.500000+6 0 1 108 364331 6 5 1891 2.475014+5 1.00000-36 0.000000+0 3.465020+5 4.38567-22 0.000000+04331 6 5 1892 4.455026+5 6.79127-20 0.000000+0 5.445031+5 4.34382-18 0.000000+04331 6 5 1893 6.435037+5 1.35926-16 0.000000+0 7.425043+5 2.38291-15 0.000000+04331 6 5 1894 8.415048+5 2.57087-14 0.000000+0 9.405054+5 1.89121-13 0.000000+04331 6 5 1895 1.039506+6 1.04959-12 0.000000+0 1.138507+6 4.55614-12 0.000000+04331 6 5 1896 1.237507+6 1.63097-11 0.000000+0 1.336508+6 4.97718-11 0.000000+04331 6 5 1897 1.435508+6 1.33443-10 0.000000+0 1.534509+6 3.20845-10 0.000000+04331 6 5 1898 1.633509+6 6.95002-10 0.000000+0 1.732510+6 1.394472-9 0.000000+04331 6 5 1899 1.831510+6 2.653443-9 0.000000+0 1.930511+6 5.084019-9 0.000000+04331 6 5 1900 2.079012+6 1.236612-8 0.000000+0 2.277013+6 2.746753-8 0.000000+04331 6 5 1901 2.475014+6 5.262710-8 0.000000+0 2.673015+6 8.864254-8 0.000000+04331 6 5 1902 2.871017+6 1.388038-7 0.000000+0 3.069018+6 1.975061-7 0.000000+04331 6 5 1903 3.267019+6 2.599060-7 0.000000+0 3.465020+6 3.275556-7 0.000000+04331 6 5 1904 3.663021+6 3.809388-7 0.000000+0 3.861022+6 4.355487-7 0.000000+04331 6 5 1905 4.207524+6 4.593823-7 0.000000+0 4.702527+6 3.591817-7 0.000000+04331 6 5 1906 5.197530+6 2.052985-7 0.000000+0 5.692533+6 7.476971-8 0.000000+04331 6 5 1907 6.187536+6 1.789799-8 0.000000+0 6.682538+6 1.807291-9 0.000000+04331 6 5 1908 7.177542+6 6.44004-11 0.000000+0 7.672544+6 1.00000-36 0.000000+04331 6 5 1909 0.000000+0 9.500000+6 0 1 114 384331 6 5 1910 2.475014+5 1.00000-36 0.000000+0 3.465020+5 2.82508-22 0.000000+04331 6 5 1911 4.455026+5 4.76578-20 0.000000+0 5.445031+5 3.23783-18 0.000000+04331 6 5 1912 6.435037+5 9.39364-17 0.000000+0 7.425043+5 1.52597-15 0.000000+04331 6 5 1913 8.415048+5 1.66387-14 0.000000+0 9.405054+5 1.27770-13 0.000000+04331 6 5 1914 1.039506+6 6.97373-13 0.000000+0 1.138507+6 3.04908-12 0.000000+04331 6 5 1915 1.237507+6 1.10725-11 0.000000+0 1.336508+6 3.38259-11 0.000000+04331 6 5 1916 1.435508+6 9.16564-11 0.000000+0 1.534509+6 2.20846-10 0.000000+04331 6 5 1917 1.633509+6 4.81893-10 0.000000+0 1.732510+6 9.72688-10 0.000000+04331 6 5 1918 1.831510+6 1.858585-9 0.000000+0 1.930511+6 3.568875-9 0.000000+04331 6 5 1919 2.079012+6 8.860990-9 0.000000+0 2.277013+6 1.966347-8 0.000000+04331 6 5 1920 2.475014+6 3.839213-8 0.000000+0 2.673015+6 6.611343-8 0.000000+04331 6 5 1921 2.871017+6 1.035043-7 0.000000+0 3.069018+6 1.502312-7 0.000000+04331 6 5 1922 3.267019+6 2.050796-7 0.000000+0 3.465020+6 2.592217-7 0.000000+04331 6 5 1923 3.663021+6 3.102307-7 0.000000+0 3.861022+6 3.705735-7 0.000000+04331 6 5 1924 4.207524+6 4.214664-7 0.000000+0 4.702527+6 3.832029-7 0.000000+04331 6 5 1925 5.197530+6 2.661783-7 0.000000+0 5.692533+6 1.418801-7 0.000000+04331 6 5 1926 6.187536+6 5.927537-8 0.000000+0 6.682538+6 1.834126-8 0.000000+04331 6 5 1927 7.177542+6 3.706895-9 0.000000+0 7.672544+6 3.98281-10 0.000000+04331 6 5 1928 8.167547+6 1.48917-11 0.000000+0 8.662550+6 1.00000-36 0.000000+04331 6 5 1929 0.000000+0 1.050000+7 0 1 120 404331 6 5 1930 2.475014+5 1.00000-36 0.000000+0 3.465020+5 2.06616-22 0.000000+04331 6 5 1931 4.455026+5 3.49441-20 0.000000+0 5.445031+5 2.27068-18 0.000000+04331 6 5 1932 6.435037+5 6.95459-17 0.000000+0 7.425043+5 1.15422-15 0.000000+04331 6 5 1933 8.415048+5 1.24634-14 0.000000+0 9.405054+5 9.39824-14 0.000000+04331 6 5 1934 1.039506+6 5.27024-13 0.000000+0 1.138507+6 2.32256-12 0.000000+04331 6 5 1935 1.237507+6 8.36816-12 0.000000+0 1.336508+6 2.59496-11 0.000000+04331 6 5 1936 1.435508+6 7.02366-11 0.000000+0 1.534509+6 1.69875-10 0.000000+04331 6 5 1937 1.633509+6 3.74529-10 0.000000+0 1.732510+6 7.57338-10 0.000000+04331 6 5 1938 1.831510+6 1.446777-9 0.000000+0 1.930511+6 2.787136-9 0.000000+04331 6 5 1939 2.079012+6 7.012256-9 0.000000+0 2.277013+6 1.579944-8 0.000000+04331 6 5 1940 2.475014+6 3.099425-8 0.000000+0 2.673015+6 5.396319-8 0.000000+04331 6 5 1941 2.871017+6 8.548588-8 0.000000+0 3.069018+6 1.252967-7 0.000000+04331 6 5 1942 3.267019+6 1.719596-7 0.000000+0 3.465020+6 2.227767-7 0.000000+04331 6 5 1943 3.663021+6 2.693776-7 0.000000+0 3.861022+6 3.284208-7 0.000000+04331 6 5 1944 4.207524+6 3.882461-7 0.000000+0 4.702527+6 3.745218-7 0.000000+04331 6 5 1945 5.197530+6 2.902728-7 0.000000+0 5.692533+6 1.813104-7 0.000000+04331 6 5 1946 6.187536+6 9.593128-8 0.000000+0 6.682538+6 4.337054-8 0.000000+04331 6 5 1947 7.177542+6 1.633661-8 0.000000+0 7.672544+6 4.792980-9 0.000000+04331 6 5 1948 8.167547+6 9.39740-10 0.000000+0 8.662550+6 9.83937-11 0.000000+04331 6 5 1949 9.157553+6 1.63692-12 0.000000+0 9.652555+6 1.00000-36 0.000000+04331 6 5 1950 0.000000+0 1.150000+7 0 1 126 424331 6 5 1951 2.475014+5 1.00000-36 0.000000+0 3.465020+5 1.27866-22 0.000000+04331 6 5 1952 4.455026+5 2.59537-20 0.000000+0 5.445031+5 1.69042-18 0.000000+04331 6 5 1953 6.435037+5 5.25670-17 0.000000+0 7.425043+5 8.97529-16 0.000000+04331 6 5 1954 8.415048+5 9.92753-15 0.000000+0 9.405054+5 7.43329-14 0.000000+04331 6 5 1955 1.039506+6 4.20242-13 0.000000+0 1.138507+6 1.85417-12 0.000000+04331 6 5 1956 1.237507+6 6.75452-12 0.000000+0 1.336508+6 2.09970-11 0.000000+04331 6 5 1957 1.435508+6 5.70955-11 0.000000+0 1.534509+6 1.38741-10 0.000000+04331 6 5 1958 1.633509+6 3.06471-10 0.000000+0 1.732510+6 6.26222-10 0.000000+04331 6 5 1959 1.831510+6 1.200424-9 0.000000+0 1.930511+6 2.331911-9 0.000000+04331 6 5 1960 2.079012+6 5.897010-9 0.000000+0 2.277013+6 1.333667-8 0.000000+04331 6 5 1961 2.475014+6 2.627865-8 0.000000+0 2.673015+6 4.625194-8 0.000000+04331 6 5 1962 2.871017+6 7.431770-8 0.000000+0 3.069018+6 1.104461-7 0.000000+04331 6 5 1963 3.267019+6 1.518249-7 0.000000+0 3.465020+6 1.975158-7 0.000000+04331 6 5 1964 3.663021+6 2.426529-7 0.000000+0 3.861022+6 2.997560-7 0.000000+04331 6 5 1965 4.207524+6 3.640493-7 0.000000+0 4.702527+6 3.645678-7 0.000000+04331 6 5 1966 5.197530+6 2.962519-7 0.000000+0 5.692533+6 2.029956-7 0.000000+04331 6 5 1967 6.187536+6 1.206976-7 0.000000+0 6.682538+6 6.403587-8 0.000000+04331 6 5 1968 7.177542+6 3.043170-8 0.000000+0 7.672544+6 1.259713-8 0.000000+04331 6 5 1969 8.167547+6 4.592358-9 0.000000+0 8.662550+6 1.295290-9 0.000000+04331 6 5 1970 9.157553+6 2.41672-10 0.000000+0 9.652555+6 2.44560-11 0.000000+04331 6 5 1971 1.014756+7 4.90033-13 0.000000+0 1.064256+7 1.00000-36 0.000000+04331 6 5 1972 0.000000+0 1.250000+7 0 1 132 444331 6 5 1973 2.475014+5 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