JEFF-3.1.3 General Purpose Neutron File, Nov. 2007. 2310 0 0 0 8.016000+3 1.585751+1 0 0 2 6 825 1451 1 0.000000+0 0.000000+0 0 0 0 6 825 1451 2 1.000000+0 1.500000+8 8 0 10 31 825 1451 3 0.000000+0 0.000000+0 0 0 828 144 825 1451 4 8-O - 16 LANL EVAL-APR01 HALE,YOUNG,CHADWICK,CARO,LUBITZ 825 1451 5 Ch96ab,Ca98,Ch99,Yo01 DIST-MAY05 REV1-MAY05 20050504 825 1451 6 ----JEFF-31 MATERIAL 825 825 1451 7 -----INCIDENT NEUTRON DATA 825 1451 8 ------ENDF-6 FORMAT 825 1451 9 *************************** JEFF-3.1.3 ************************* 825 1451 10 ** ** 825 1451 11 ** Original data taken from: JEFF-3.1 ** 825 1451 12 ** ** 825 1451 13 ****************************************************************** 825 1451 14 825 1451 15 HISTORY 825 1451 16 05-05 Evaluation for JEFF-3.1 is ENDF\B-VI.8 825 1451 17 11-07 (n,alpha0) cross section replaced by G. Noguere with 825 1451 18 cross section of ENDF\B-VII.0 in accordance with [Gi07] 825 1451 19 825 1451 20 ****************************************************************** 825 1451 21 825 1451 22 ENDF/B-VI MOD 3 Evaluation, April 2001, P.G. Young, G.M. Hale 825 1451 23 M.B. Chadwick (LANL), E.Caro, C.R. Lubitz (KAPL) 825 1451 24 825 1451 25 This evaluation is a combination of a new MOD 3 evaluation 825 1451 26 below 30 MeV and the previous MOD 2 evaluation from 20 to 150 MeV. 825 1451 27 Both these evaluations are described below. The only change to the 825 1451 28 data above 30 MeV is to add tritium-production data, based on 825 1451 29 experimental yield data and spectra calculated with the GNASH 825 1451 30 Hauser-Feshbach/preequilibrium code. 825 1451 31 This evaluation provides a complete representation of the 825 1451 32 nuclear data needed for transport, damage, heating, radioactivity, 825 1451 33 and shielding applications over the incident neutron energy range 825 1451 34 from 1.0E-11 to 150 MeV. The discussion here is divided into the 825 1451 35 region above and below 30 MeV. 825 1451 36 825 1451 37 ------------------------------------------------------------------ 825 1451 38 825 1451 39 INCIDENT NEUTRON ENERGIES > 30 MeV 825 1451 40 825 1451 41 The evaluation above 30 MeV utilizes MF=6, MT=5 to represent 825 1451 42 all reaction data. Production cross sections and emission 825 1451 43 spectra are given for neutrons, protons, deuterons, alpha 825 1451 44 particles, gamma rays, and all residual nuclides produced (A>5) 825 1451 45 in the reaction chains. To summarize, the ENDF sections with 825 1451 46 non-zero data above En = 30 MeV are: 825 1451 47 825 1451 48 MF=3 MT= 1 Total Cross Section 825 1451 49 MT= 2 Elastic Scattering Cross Section 825 1451 50 MT= 3 Nonelastic Cross Section 825 1451 51 MT= 5 Sum of Binary (n,n') and (n,x) Reactions 825 1451 52 MT=102 Radiative Capture Cross Section (Estimate Only) 825 1451 53 825 1451 54 MF=4 MT= 2 Elastic Angular Distributions 825 1451 55 825 1451 56 MF=6 MT= 5 Production Cross Sections and Energy-Angle 825 1451 57 Distributions for Emission Neutrons, Protons, 825 1451 58 Deuterons, and Alphas; and Angle-Integrated 825 1451 59 Spectra for Gamma Rays and Residual Nuclei That 825 1451 60 Are Stable Against Particle Emission 825 1451 61 825 1451 62 The evaluation is based on nuclear model calculations that 825 1451 63 have been benchmarked to experimental data, especially for n + 825 1451 64 O16 and p + O16 reactions [Ch96a]. We use the GNASH code system 825 1451 65 [Yo92], which utilizes Hauser-Feshbach statistical, preequi- 825 1451 66 librium and direct-reaction theories. Coupled-channel and 825 1451 67 spherical optical model calculations are used to obtain particle 825 1451 68 transmission coefficients for the Hauser-Feshbach calculations, 825 1451 69 as well as for the elastic neutron angular distributions. 825 1451 70 Cross sections and spectra for producing individual residual 825 1451 71 nuclei are included for reactions that exceed a cross section of 825 1451 72 approximately 1 nb at any energy. The energy-angle-correlations 825 1451 73 for all outgoing particles are based on Kalbach systematics 825 1451 74 [Ka88]. 825 1451 75 A model was developed to calculate the energy distributions of 825 1451 76 all recoil nuclei in the GNASH calculations [Ch96b]. The recoil 825 1451 77 energy distributions are represented in the laboratory system in 825 1451 78 MT=5, MF=6, and are given as isotropic in the lab system. Note 825 1451 79 that all other data in MT=5,MF=6 are given in the center-of-mass 825 1451 80 system. This method of representation requires a modification of 825 1451 81 the original ENDF-6 format. 825 1451 82 Preequilibrium corrections were performed in the course of the 825 1451 83 GNASH calculations using either Feshbach, Kerman, Koonin (FKK) 825 1451 84 theory [Ch93] or the exciton model of Kalbach [Ka77, Ka85]. 825 1451 85 Discrete level data from nuclear data sheets were matched to 825 1451 86 continuum level densities using the formulation of Ignatyuk 825 1451 87 [Ig75] and pairing and shell parameters from the Cook [Co67] 825 1451 88 analysis. Neutron and charged-particle transmission coefficients 825 1451 89 were obtained from the optical potentials, as discussed below. 825 1451 90 Gamma-ray transmission coefficients were calculated using the 825 1451 91 Kopecky-Uhl model [Ko90]. 825 1451 92 825 1451 93 ------------------------------------------------------------------ 825 1451 94 825 1451 95 INCIDENT NEUTRON ENERGIES < 30 MeV 825 1451 96 825 1451 97 The evaluation below 30 MeV includes complete data for all 825 1451 98 significant neutron-induced reactions. It is comprised of 825 1451 99 R-parameter [Ca98] and R-matrix analyses below 6.25 MeV, and a 825 1451 100 combination of experimental and theoretical data evaluation 825 1451 101 from 6.25 to 30 MeV. A summary of the evaluation by energy 825 1451 102 range is given below, followed by a detailed description of 825 1451 103 the evaluation, reaction by reaction. 825 1451 104 825 1451 105 NEUTRON ENERGY < 6.25 MeV 825 1451 106 825 1451 107 The evaluation below 3.4 MeV is an R-function fit [Ca98] to 825 1451 108 experimental data. At 3.4 MeV, it is spliced to the LANL R-matrix 825 1451 109 analysis with a transition region of about 60 keV centered at 825 1451 110 3.4 MeV. The LANL analysis is used for the region from 3.40 to 825 1451 111 6.25 MeV. 825 1451 112 825 1451 113 NEUTRON ENERGY > 6.25 MeV 825 1451 114 825 1451 115 The following major modifications were made above 6.25 MeV: 825 1451 116 1. The maximum energy of the evaluation was increased from 20 to 825 1451 117 30 MeV. 825 1451 118 2. New measurements of 16O(n,xgamma) angular distributions (7 825 1451 119 angles, En = 4 - 200 MeV) by Nelson et al. [Ne99] were incor- 825 1451 120 porated into the evaluation. The measurements use a high- 825 1451 121 resolution Ge detector and result in data for some 21 gamma rays. 825 1451 122 The distributions were fit with Legendre expansions to obtain 825 1451 123 angle-integrated cross sections for MF=13 and angular 825 1451 124 distributions for MF=14. Nuclear energy level schemes and gamma 825 1451 125 branching ratios [Aj86,Aj91] were utilized to extract level 825 1451 126 excitation cross sections in MF=3 for discrete states in 16O, 825 1451 127 14-16N, and 13C, corresponding to (n,n'), (n,p), (n,d), (n,t), 825 1451 128 and (n,alpha) reactions. 825 1451 129 3. New measurements of 16O(n,alpha) cross sections at 14 MeV by 825 1451 130 Sanami and Baba [Sa97] were used to adjust the (n,alpha) cross 825 1451 131 sections. 825 1451 132 4. The neutron total cross section measurements of Finlay [Fi93] 825 1451 133 were incorporated into the evaluation above 7.3 MeV. Adjustments 825 1451 134 of up to 2% were made in the existing evaluation. 825 1451 135 5. The new evaluation contains no pseudo level or excitation 825 1451 136 energy bin data. Calculations were made with the GNASH code to 825 1451 137 provide continuum emission data in MF=6 format, as well as any 825 1451 138 unmeasured data. Calculated cross sections were renormalized 825 1451 139 whenever possible using experimental data. The GNASH calculations 825 1451 140 utilized transmission coefficients calculated with a spherical 825 1451 141 optical potential and level densities from the Gilbert and 825 1451 142 Cameron model, plus preequilibrium corrections using systematic 825 1451 143 values of parameters. 825 1451 144 6. Comparisons of the evaluation with a large body of 825 1451 145 experimental data have been made to validate the new data. 825 1451 146 825 1451 147 ------------------------------------------------------------------ 825 1451 148 825 1451 149 DETAILED DESCRIPTION REACTION BY REACTION 825 1451 150 825 1451 151 MF=2 RESONANCE PARAMETERS ------------------------------------- 825 1451 152 825 1451 153 The evaluation below 3.4 MeV is an R-function fit [Ca98] to 825 1451 154 experimental data using an optical model to provide a background 825 1451 155 R-function. The procedure is coded in the KAPL code "OPTIC", 825 1451 156 with an extension of the original code to convert the optical- 825 1451 157 model phase shifts to background R-functions. 825 1451 158 The analysis is carried to 3.4 MeV, where it is spliced to the 825 1451 159 LANL R-matrix analysis, with a transition region of about 60 keV 825 1451 160 centered at 3.4 MeV. 825 1451 161 From 3.4 to 6.25 MeV, a test evaluation was obtained from a new 825 1451 162 multi-channel R-matrix analysis of a large part of the available 825 1451 163 experimental data base using the EDA code. The analysis of the 825 1451 164 17O system includes data for n+16O neutron total cross sections 825 1451 165 and elastic scattering angular distributions, as well as data 825 1451 166 for the 16O(n,alpha) reaction in both the (n,alpha) and 825 1451 167 (alpha,n) directions. Also included are excitation functions 825 1451 168 for alpha+13C elastic scattering. The total cross sections in 825 1451 169 the final version of this analysis may change, especially in the 825 1451 170 region above 4 MeV. 825 1451 171 825 1451 172 Effective scattering radius = 5.56256E-13 cm. 825 1451 173 825 1451 174 MF=3 NEUTRON CROSS SECTIONS ----------------------------------- 825 1451 175 825 1451 176 THERMAL (2200 m/s) CROSS SECTIONS 825 1451 177 825 1451 178 TOTAL = 3.89440 B RADIATIVE CAPTURE= 0.1900 MB 825 1451 179 ELASTIC= 3.89421 B 825 1451 180 825 1451 181 MT=1 TOTAL CROSS SECTION 825 1451 182 0.0 to 3.40 MeV, calculated from R-function fit to total cross 825 1451 183 section and elastic angular distributions - see above. 825 1451 184 3.4 to 6.25 MeV, calculated from R-Matrix parameters by 825 1451 185 simultaneously fitting most of the available 16O(n,n)16O and 825 1451 186 16O(n,alpha0)13C data, as well as 13C(alpha,alpha)13C data at 825 1451 187 energies below En = 6.2 MeV. The experimental total cross 825 1451 188 section data fitted in the analysis were the [Jo74] results below 825 1451 189 6.26 MeV, and the [La80] measurements at higher energies, with 825 1451 190 inserts of the high-resolution data of [Jo79] over the resonances 825 1451 191 and in the window at En = 2.3-2.4 MeV. 825 1451 192 6.25 to 30 MeV, based on an adjustment of the covariance 825 1451 193 analysis used for the ENDF/B-VI (Rel. 0) evaluation to 825 1451 194 accommodate the new measurements of Finlay et al. [Fi93]. The 825 1451 195 previous ENDF/B-VI (Rel. 0) evaluations is based on analysis 825 1451 196 with the GLUCS Bayes code [He80] of the remaining major total 825 1451 197 cross section measurements [Fo71], [Pe72], [Sc72], [La80], 825 1451 198 [Ci68], [Ci80], with structure inserted from the high-resolution 825 1451 199 [Ci80] measurement. 825 1451 200 825 1451 201 MT=2 ELASTIC SCATTERING CROSS SECTION 825 1451 202 0.0 to 3.40 MeV, calculated from R-function fit to total cross 825 1451 203 section and elastic angular distributions - see above. 825 1451 204 3.4 to 6.25 MeV, R-matrix analysis that includes all available 825 1451 205 experimental data, as described above. Elastic angular 825 1451 206 distribution data used in the analysis includes [La60], [Ok55], 825 1451 207 [Fo58], [Ma62], [Fo70], [Hu62], [Ph61], [Jo67], [Ki72], [Ch61], 825 1451 208 [Dr76], [Fo64]. 825 1451 209 6.25 to 20 MeV, obtained by subtracting the nonelastic cross 825 1451 210 section (MT=3) from the total cross section (MT=1), although 825 1451 211 small adjustments were made to several of the less well 825 1451 212 determined reaction cross sections in order to enhance agreement 825 1451 213 with the elastic measurements of Borker [Bo89], Glendinning 825 1451 214 [Gl82], and Petler [Pe85]. The magnitude of these adjustments 825 1451 215 was generally small and was greatest near structure and near 825 1451 216 18 MeV. 825 1451 217 825 1451 218 MT=4 INELASTIC CROSS SECTION 825 1451 219 Threshold to 30 MeV, sum of MT=51-57, 91. 825 1451 220 825 1451 221 MT=51-57 INELASTIC CROSS SECTION TO DISCRETE STATES 825 1451 222 Threshold to 30 MeV, the (n,n') cross sections corresponding 825 1451 223 to gamma-emitting excited levels of 16O are included in MT=51-57 825 1451 224 as follows: 825 1451 225 MT=51 Ex= 6.0494 MeV 825 1451 226 MT=52 Ex= 6.129893 MeV 825 1451 227 MT=53 Ex= 6.9171 MeV 825 1451 228 MT=54 Ex= 7.11685 MeV 825 1451 229 MT=55 Ex= 8.8719 MeV 825 1451 230 MT=56 Ex=10.957 MeV 825 1451 231 MT=57 Ex=11.080 MeV 825 1451 232 825 1451 233 Note that the 16O levels at 9.585, 9.8445, and 10.356 are 825 1451 234 omitted because they decay primarily by alpha particle emission 825 1451 235 and those data are included in MT=22. 825 1451 236 825 1451 237 MT=16 (N,2N) CROSS SECTION 825 1451 238 Threshold to 30 MeV, based on GNASH calculation, renormalized 825 1451 239 down by approximately 30% to improve agreement with measurement 825 1451 240 of Brill et al. [Br61]. 825 1451 241 825 1451 242 MT=22 (N,NALPHA) CROSS SECTION 825 1451 243 Threshold to 30 MeV, based on GNASH calculation, with 825 1451 244 adjustments made to improve agreement with experimental data, 825 1451 245 especially data of Bormann et al. [Bo63]. 825 1451 246 825 1451 247 MT=23 (N,N3ALPHA) CROSS SECTION 825 1451 248 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 249 from 28 to 30 MeV to agree with LA150 data. 825 1451 250 825 1451 251 MT=28 (N,NP) CROSS SECTION 825 1451 252 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 253 such that the production cross sections for the 5.2701 and 5.2988 825 1451 254 MeV gamma rays are consistent with Nelson et al.[Ne99] data, and 825 1451 255 normalization of proton spectra consistent with 27-MeV data of 825 1451 256 Subramanian et al. [Su94]. 825 1451 257 825 1451 258 MT=32 (N,ND) CROSS SECTION 825 1451 259 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 260 such that difference between total and nonelastic cross sections 825 1451 261 agrees with elastic cross section measurements. 825 1451 262 825 1451 263 MT=41 (N,2NP) CROSS SECTION 825 1451 264 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 265 such that difference between total and nonelastic cross sections 825 1451 266 agrees with elastic cross section measurements. 825 1451 267 825 1451 268 MT=44 (N,N2P) CROSS SECTION 825 1451 269 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 270 such that difference between total and nonelastic cross sections 825 1451 271 agrees with elastic cross section measurements. 825 1451 272 825 1451 273 MT=45 (N,NPALPHA) CROSS SECTION 825 1451 274 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 275 such that difference between total and nonelastic cross sections 825 1451 276 agrees with elastic cross section measurements. 825 1451 277 825 1451 278 MT=91 (N,N'CONTINUUM) CROSS SECTION 825 1451 279 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 280 such that difference between total and nonelastic cross sections 825 1451 281 agrees with elastic cross section measurements. 825 1451 282 825 1451 283 MT=102 (N,GAMMA) CROSS SECTION 825 1451 284 0 to 1 MeV,cross section based on experimental data obtained 825 1451 285 from E. Jurney [Ju64]; higher energy data is crude estimate. 825 1451 286 825 1451 287 MT=103 (N,P) CROSS SECTION 825 1451 288 Sum of MT=600-603. 825 1451 289 825 1451 290 MT=104 (N,D) CROSS SECTION 825 1451 291 Sum of MT=650-669. 825 1451 292 825 1451 293 MT=105 (N,T) CROSS SECTION 825 1451 294 Sum of MT=700-709,749. 825 1451 295 825 1451 296 MT=107 (N,ALPHA) CROSS SECTION 825 1451 297 Sum of MT=800-803. 825 1451 298 825 1451 299 MT=108 (N,2ALPHA) CROSS SECTION 825 1451 300 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 301 such that difference between total and nonelastic cross sections 825 1451 302 agrees with elastic cross section measurements. 825 1451 303 825 1451 304 MT=112 (N,PALPHA) CROSS SECTION 825 1451 305 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 306 such that difference between total and nonelastic cross sections 825 1451 307 agrees with elastic cross section measurements. 825 1451 308 825 1451 309 MT=600 (N,P) INTEGRATED CROSS SECTION TO 16N GROUND STATE 825 1451 310 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 311 renormalization (lowered approximately 30%) from comparison of 825 1451 312 excited state predictions with Nelson et al. [Ne99] 825 1451 313 measurements. 825 1451 314 825 1451 315 MT=601-603 (N,P) CROSS SECTION TO EXCITED LEVELS OF 16N 825 1451 316 Threshold to 30 MeV, the cross sections for the 0.0.297- and 825 1451 317 0.3975-MeV levels are inferred from the (n,p gamma) data of 825 1451 318 Nelson et al. [Ne99], using the level structure diagram of 16N 825 1451 319 by Ajzenberg-Selove [Aj86]. The cross section for the 0.1201- 825 1451 320 MeV level is based on GNASH calculations with some 825 1451 321 renormalization (lowered ~30%) from comparison of excited state 825 1451 322 predictions with Nelson et al. [Ne99] measurements. 825 1451 323 825 1451 324 MT=650 (N,D) INTEGRATED CROSS SECTION TO 15N GROUND STATE 825 1451 325 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 326 renormalization from comparison of excited state predictions 825 1451 327 with Nelson et al. [Ne99] measurements. 825 1451 328 825 1451 329 MT=651-669 (N,D) CROSS SECTION TO EXCITED LEVELS OF 15N 825 1451 330 Threshold to 30 MeV, the cross sections for the 5.2701- and 825 1451 331 5.2988-MeV levels are adjusted based on the (n,xgamma) data of 825 1451 332 Nelson et al. [Ne99], using the level structure diagram for 15N 825 1451 333 by Ajzenberg-Selove [Aj91]. Cross sections for remaining levels 825 1451 334 are based on GNASH calculations with some renormalization from 825 1451 335 comparison of excited state predictions with Nelson et al. 825 1451 336 [Ne99] measurements and 27-Mev data of Subramanian et al. [Su94]. 825 1451 337 825 1451 338 MT=700 (N,T) INTEGRATED CROSS SECTION TO 14N GROUND STATE 825 1451 339 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 340 renormalization from comparison of excited state predictions 825 1451 341 with Nelson et al. [Ne99] measurements. 825 1451 342 825 1451 343 MT=701-709 (N,T) CROSS SECTION TO EXCITED LEVELS OF 14N 825 1451 344 Threshold to 30 MeV, the cross section for the 2.3128-MeV 825 1451 345 levels is inferred from the (n,t gamma) data of Nelson et al. 825 1451 346 [Ne99], using the level structure diagram for 16N by Ajzenberg- 825 1451 347 Selove [Aj91]. Cross sections for the remaining levels are 825 1451 348 based on GNASH calculations with some renormalization from 825 1451 349 comparison of excited state predictions with Nelson et al. 825 1451 350 [Ne99] measurements. 825 1451 351 825 1451 352 MT=749 (N,T) CROSS SECTION TO 14N CONTINUUM 825 1451 353 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 354 renormalization from comparison of excited state predictions 825 1451 355 with Nelson et al. [Ne99] measurements and to enhance agreement 825 1451 356 of elastic cross section with measured data. 825 1451 357 825 1451 358 MT=800 (N,ALPHA0) CROSS SECTION TO 13C GROUND STATE 825 1451 359 0.0 to 6.2 MeV, based on R-matrix analysis described above 825 1451 360 under MT=1. Data of Ba72 were used in the original (alpha,n) 825 1451 361 direction, with no changes in energy scale or normalization. 825 1451 362 Also included were the low-energy (alpha,n) data of [Ke91] and 825 1451 363 [Dr93]. 825 1451 364 6.2 to 20 MeV, based on data of [Da63],[Da68],[Si68],[Ba73], 825 1451 365 and composite of [Mc66b],[Ma68],[Le68] at 14 MeV. Note that the 825 1451 366 [Da63] data were renormalized by factor of 1.5 to bring them 825 1451 367 into rough agreement with the R-matrix analysis of the [Ba73] 825 1451 368 (n,a0) data, together with the total and elastic data in the 825 1451 369 analysis. Because the [Da68] experimental data were normalized 825 1451 370 to [Da63], the former were also renormalized by the factor of 825 1451 371 1.5. 825 1451 372 825 1451 373 MT=801-803 (N,ALPHA) CROSS SECTION TO EXCITED LEVELS OF 13C 825 1451 374 Threshold to 30 MeV, the cross sections of the 3.0894-, 825 1451 375 3.6845-, and 3.8538-MeV levels are inferred from the (n,alpha 825 1451 376 gamma) data of Nelson et al. [Ne99], using the level structure 825 1451 377 diagram of 13C by Ajzenberg-Selove [Aj91]. 825 1451 378 825 1451 379 MF=4 ANGULAR DISTRIBUTIONS ------------------------------------ 825 1451 380 825 1451 381 MT=2 ELASTIC NEUTRON ANGULAR DISTRIBUTIONS 825 1451 382 0.0 to 3.4 MeV, calculated from R-function fit (see MF=3,MT=1). 825 1451 383 3.4 to 6.2 MeV, calculated from R-matrix fit (see MF=3,MT=1). 825 1451 384 Measured angular distributions input to the fit were those of 825 1451 385 [Ch61],[Fo58],[Fo70],[Hi58],[Hu62], [Jo67],[Ki72],[La60],[Li66], 825 1451 386 [Ma62],[Ph61],[Jo79]. Fits were attempted using new data of 825 1451 387 [Sc77], but those measurements were found to have significant 825 1451 388 uncertainties, and some discrepancies with other data were noted. 825 1451 389 6.2 to 20 MeV, smooth curve through coefficients derived from 825 1451 390 fits to elastic data of [Ph61],[Ne72],[Ch61],[Ba63],[Be67], 825 1451 391 [Mc66a],[Ki72],[Bu73],[Ne72],[Gl82],[Ba85],[Bo89],[Pe85]. 825 1451 392 825 1451 393 MT=51-57 DISCRETE (N,N') ANGULAR DISTRIBUTIONS 825 1451 394 Threshold to 10 MeV, assumed isotropic in center of mass. 825 1451 395 Above 10 MeV, based on fits of the 14-MeV data of [Ki72],[Ne72], 825 1451 396 [Ba63],[Mc66a],[Ba85],[Me69], and especially [Bo89]. 825 1451 397 825 1451 398 MT=600-603 DISCRETE (N,P) ANGULAR DISTRIBUTIONS 825 1451 399 Threshold to 30 MeV, assumed isotropic in center of mass. 825 1451 400 825 1451 401 MT=650-669 DISCRETE (N,D) ANGULAR DISTRIBUTIONS 825 1451 402 Threshold to 30 MeV, assumed isotropic in center of mass. 825 1451 403 825 1451 404 MT=700-709 DISCRETE (N,T) ANGULAR DISTRIBUTIONS 825 1451 405 Threshold to 30 MeV, assumed isotropic in center of mass. 825 1451 406 825 1451 407 MT=800 DISCRETE(N,ALPHA0) ANGULAR DISTRIBUTIONS 825 1451 408 0.0 to 6.2 MeV, calculated from R-Matrix fit (see MF=3,MT=1). 825 1451 409 Measured angular distributions input to the fit were 825 1451 410 reconstructed from the Legendre coefficients of [Wa57], and 825 1451 411 converted to (n,alpha) angular distributions using detailed 825 1451 412 balance. 825 1451 413 825 1451 414 MT=801-803 DISCRETE (N,T) ANGULAR DISTRIBUTIONS 825 1451 415 Threshold to 6 MeV, 825 1451 416 6 to 30 MeV, assumed isotropic in center of mass. 825 1451 417 825 1451 418 MF=6 PRODUCT ENERGY-ANGLE DISTRIBUTIONS ----------------------- 825 1451 419 825 1451 420 MT=16 (N,2N) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 421 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 422 are given for neutrons, and isotropic energy spectra are given 825 1451 423 for recoiling 15O nuclei. The neutron data were obtained from 825 1451 424 the GNASH calculations; the recoil 15O distributions were 825 1451 425 calculated with the RECOIL code [Ma83]. The discrete gamma rays 825 1451 426 from (n,2ngamma) reactions are given in MF=13 and 14. 825 1451 427 825 1451 428 MT=22 (N,NALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 429 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 430 are given for neutrons and alpha particles, and isotropic energy 825 1451 431 spectra are given for recoiling 12C nuclei. The neutron and 825 1451 432 alpha data were obtained from the GNASH calculations; the recoil 825 1451 433 12C distributions were calculated with the RECOIL code [Ma83]. 825 1451 434 The discrete gamma rays from (n,nalpha gamma) reactions are 825 1451 435 given in MF=13 and 14. 825 1451 436 825 1451 437 MT=28 (N,NP) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 438 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 439 are given for neutrons and protons; isotropic energy spectra are 825 1451 440 given for recoiling 15N nuclei; and isotropic energy spectra are 825 1451 441 given for emitted continuum gamma rays. The neutron, proton, 825 1451 442 and gamma-ray data were obtained from the GNASH calculations; 825 1451 443 the recoil 15N distributions were calculated with the RECOIL 825 1451 444 code [Ma83]. 825 1451 445 825 1451 446 MT=32 (N,ND) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 447 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 448 are given for neutrons and deuterons; isotropic energy spectra 825 1451 449 are given for recoiling 14N nuclei; and isotropic energy spectra 825 1451 450 are given for emitted continuum gamma rays. The neutron, 825 1451 451 deuteron, and gamma-ray data were obtained from the GNASH 825 1451 452 calculations; the recoil 14N distributions were calculated with 825 1451 453 the RECOIL code [Ma83]. 825 1451 454 825 1451 455 MT=41 (N,2NP) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 456 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 457 are given for neutrons and protons; isotropic energy spectra are 825 1451 458 given for recoiling 14N nuclei; and isotropic energy spectra are 825 1451 459 given for emitted continuum gamma rays. The neutron, proton, 825 1451 460 and gamma-ray data were obtained from the GNASH calculations; 825 1451 461 the recoil 14N distributions were calculated with the RECOIL 825 1451 462 code [Ma83]. 825 1451 463 825 1451 464 MT=44 (N,N2P) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 465 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 466 are given for neutrons and protons; isotropic energy spectra are 825 1451 467 given for recoiling 14C nuclei; and isotropic energy spectra are 825 1451 468 given for emitted continuum gamma rays. The neutron, proton, 825 1451 469 and gamma-ray data were obtained from the GNASH calculations; 825 1451 470 the recoil 14C distributions were calculated with the RECOIL 825 1451 471 code [Ma83]. 825 1451 472 825 1451 473 MT=45 (N,NPALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 474 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 475 are given for neutrons, protons, and alphas; isotropic energy 825 1451 476 spectra are given for recoiling 11B nuclei; and isotropic energy 825 1451 477 spectra are given for emitted continuum gamma rays. The 825 1451 478 neutron, proton, alpha, and gamma-ray data were obtained from 825 1451 479 the GNASH calculations; the recoil 11B distributions were 825 1451 480 calculated with the RECOIL code [Ma83]. 825 1451 481 825 1451 482 MT=91 (N,N'CONTINUUM) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 483 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 484 are given for neutrons; isotropic energy spectra are given for 825 1451 485 recoiling 16O nuclei; and isotropic energy spectra are given for 825 1451 486 emitted continuum gamma rays. The neutron and gamma-ray data 825 1451 487 were obtained from the GNASH calculations; the recoil 16O 825 1451 488 distributions were calculated with the RECOIL code [Ma83]. 825 1451 489 825 1451 490 MT=108 (N,2ALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 491 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 492 are given for alphas; isotropic energy spectra are given for 825 1451 493 recoiling 9Be nuclei; and isotropic energy spectra are given for 825 1451 494 emitted continuum gamma rays. The alpha, and gamma-ray data 825 1451 495 were obtained from the GNASH calculations; the recoil 9Be 825 1451 496 distributions were calculated with the RECOIL code [Ma83]. 825 1451 497 825 1451 498 MT=112 (N,PALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 499 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 500 are given for protons, and alphas; isotropic energy spectra are 825 1451 501 given for recoiling 12B nuclei; and isotropic energy spectra are 825 1451 502 given for emitted continuum gamma rays. The proton, alpha, and 825 1451 503 gamma-ray data were obtained from the GNASH calculations; the 825 1451 504 recoil 12B distributions were calculated with the RECOIL code 825 1451 505 [Ma83]. 825 1451 506 825 1451 507 MT=749 (N,ALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 508 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 509 are given for alpha particles; isotropic energy spectra are 825 1451 510 given for recoiling 13C nuclei; and isotropic energy spectra are 825 1451 511 given for emitted continuum gamma rays. The alpha and gamma-ray 825 1451 512 data were obtained from the GNASH calculations; the recoil 13C 825 1451 513 distributions were calculated with the RECOIL code [Ma83]. 825 1451 514 825 1451 515 MF=12 PHOTON PRODUCTION MULTIPLICITIES ------------------------ 825 1451 516 825 1451 517 MT=102 (N,GAMMA) PHOTON PRODUCTION MULTIPLICITIES 825 1451 518 Photon multiplicities for radiative capture are based on 825 1451 519 experimental data obtained from Jurney [Ju64]. 825 1451 520 825 1451 521 MF=13 PHOTON PRODUCTION CROSS SECTIONS ------------------------ 825 1451 522 825 1451 523 MT=4 (N,N'GAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 524 Threshold to 30 MeV: Based almost entirely on new angular 825 1451 525 distribution measurements by Nelson et al. [Ne99], which 825 1451 526 utilized a white neutron source and covered the energy range 825 1451 527 from threshold to 200 MeV. The measurements were made at 7 825 1451 528 angles using high-resolution Ge detectors and resulted in data 825 1451 529 for some 23 gamma rays from 7 different reactions. The angular 825 1451 530 distributions were fit with Legendre expansions to obtain angle- 825 1451 531 integrated cross sections. The fitted cross sections were 825 1451 532 smoothed somewhat for this evaluation, although much of the 825 1451 533 measured structure was preserved, particularly for the intense 825 1451 534 6.129-MeV gamma. The evaluated data for the following gamma 825 1451 535 rays are based directly on the measurements: 825 1451 536 825 1451 537 EG= 2.742 MeV (decay of 8.8719-MeV level of 16O) 825 1451 538 EG= 3.839 MeV (decay of 10.957-MeV level of 16O) 825 1451 539 EG= 4.950 MeV (decay of 11.080-MeV level of 16O) 825 1451 540 EG= 6.130 MeV (decay of 6.130-MeV level of 16O) 825 1451 541 EG= 6.917 MeV (decay of 6.917-MeV level of 16O) 825 1451 542 EG= 7.117 MeV (decay of 7.117-MeV level of 16O) 825 1451 543 825 1451 544 The evaluated cross sections for the remaining (n,n') gamma 825 1451 545 rays are inferred from these data using the energy level scheme 825 1451 546 of Ajzenberg-Selove [Aj86]. Data were also obtained for gamma 825 1451 547 rays of energy 1.755 and 1.955 from decay of the 8.8719-MeV 825 1451 548 level but the 2.742-MeV gamma was used to determine the level 825 1451 549 excitation cross section because it is the most intense. 825 1451 550 Similarly, data were obtained on a 4.179-MeV gamma from decay of 825 1451 551 the 11.080-MeV level, but the 4.950-MeV gamma is more intense 825 1451 552 and was used to determine the level excitation cross section. 825 1451 553 The evaluated data were compared to older gamma-ray 825 1451 554 measurements by [Be70], [Ne90], [No78], [Ha59], [Di70], [Or70], 825 1451 555 [Dr70], [Cl69], [Lu70], [Bu71], [Ny69]. Considering that very 825 1451 556 few (e.g., [Be70], [Dr70]) of these measurements are of full 825 1451 557 angular distributions, the agreement is reasonable. 825 1451 558 825 1451 559 MT=16 (N,2NGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 560 Threshold to 30 MeV: The cross section for the 5.2409-MeV 825 1451 561 gamma ray was obtained directly from the Nelson et al. [Ne99] 825 1451 562 data. The remaining discrete gammas are based on GNASH 825 1451 563 calculations, with some renomalization based on the experimental 825 1451 564 data. 825 1451 565 825 1451 566 MT=22 (N,NALPHA GAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 567 Threshold to 30 MeV: Only the 4.438-MeV discrete gamma ray 825 1451 568 is given and it is based on the Nelson et al. [Ne99] data. 825 1451 569 825 1451 570 MT=103 (N,PGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 571 Threshold to 30 MeV: The cross sections for the 0.2774- and 825 1451 572 0.297-MeV gamma rays are based on the Nelson et al. [Ne99] data. 825 1451 573 The 0.3975-MeV gamma is inferred from the 0.2774-MeV gamma data 825 1451 574 through the Ajzenberg-Selove level scheme [Aj86] for 16N. The 825 1451 575 0.1201-MeV gamma cross section is based partially on GNASH 825 1451 576 calculations and partially inferred from the [Ne99] data using 825 1451 577 the 16N level scheme. 825 1451 578 825 1451 579 MT=104 (N,DGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 580 Threshold to 30 MeV: The cross sections for the 5.2701- and 825 1451 581 5.2988-MeV gamma rays are based on the Nelson et al. [Ne99] 825 1451 582 data. The cross sections for the remaining 60 (n,dg) gamma rays 825 1451 583 are based on GNASH calculations and the Ajzenberg-Selove level 825 1451 584 scheme [Aj91] for 15N, after renomalization to agree with the 825 1451 585 measured 5.2701- and 5.2988-MeV gamma-ray data. 825 1451 586 825 1451 587 MT=105 (N,TGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 588 Threshold to 30 MeV: The cross section for the 2.313-MeV 825 1451 589 gamma ray is based on the Nelson et al. [Ne99] measurement. The 825 1451 590 cross sections for the remaining 20 (n,tg) gamma rays are based 825 1451 591 on GNASH calculations and the Ajzenberg-Selove level scheme 825 1451 592 [Aj91] for 14N, after renomalization to agree with the measured 825 1451 593 2.313-MeV gamma-ray data. 825 1451 594 825 1451 595 MT=107 (N,ALPHA GAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 596 Threshold to 30 MeV: The cross sections for the 3.0894-, 825 1451 597 3.6845- and 3.8538-MeV gamma rays are based on the Nelson et 825 1451 598 al. [Ne99] data. The 0.1693-, 0.5951- and 0.7644-MeV gamma-ray 825 1451 599 cross sections are inferred from the above data through the 825 1451 600 Ajzenberg-Selove level scheme [Aj91]. Note that the 0.1693-MeV 825 1451 601 gamma from decay of the 3.8538-MeV level also was measured, but 825 1451 602 the 3.8538-MeV gamma is more intense and was used to determine 825 1451 603 the level excitation cross section. 825 1451 604 825 1451 605 MF=14 PHOTON ANGULAR DISTRIBUTIONS ---------------------------- 825 1451 606 825 1451 607 MT=4 (N,N'GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 608 Anisotropic angular distributions in Legendre polynomial 825 1451 609 representation are given for the 1.755-, 2.742-, 6.130-, 6.917-, 825 1451 610 and 7.117-MeV gamma rays, obtained by fitting the measurements 825 1451 611 of Nelson et al. [Ne99]. Isotropic angular distributions are 825 1451 612 assumed for the remaining gamma rays. 825 1451 613 825 1451 614 MT=16 (N,2NGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 615 An anisotropic angular distribution in Legendre polynomial 825 1451 616 representation is given for the 5.2409-MeV gamma ray, obtained 825 1451 617 by fitting the measurements of Nelson et al. [Ne99]. Isotropic 825 1451 618 angular distributions are assumed for the remaining gamma rays. 825 1451 619 825 1451 620 MT=22 (N,NALPHA GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 621 An anisotropic angular distribution in Legendre polynomial 825 1451 622 representation is given for the 4.438-MeV gamma ray, obtained by 825 1451 623 fitting the measurements of Nelson et al. [Ne99]. 825 1451 624 825 1451 625 MT=102 (N,GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 626 All gamma rays from radiative capture are assumed to be 825 1451 627 isotropic. 825 1451 628 825 1451 629 MT=103 (N,PGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 630 Anisotropic angular distributions in Legendre polynomial 825 1451 631 representation are given for the 0.2774-, 0.297-, and 0.3975-MeV 825 1451 632 gamma rays, obtained by fitting the measurements of Nelson et 825 1451 633 al. [Ne99]. The angular distributions for all remaining gamma 825 1451 634 rays are assumed to be isotropic. 825 1451 635 825 1451 636 MT=104 (N,DGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 637 An anisotropic angular distribution in Legendre polynomial 825 1451 638 representation is given for the 5.2701-MeV gamma ray, obtained 825 1451 639 by fitting the measurements of Nelson et al. [Ne99]. The 825 1451 640 angular distributions for all remaining gamma rays are assumed 825 1451 641 to be isotropic. 825 1451 642 825 1451 643 MT=105 (N,TGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 644 All gamma rays from (n,tg) reactions are assumed to be 825 1451 645 isotropic. 825 1451 646 825 1451 647 MT=107 (N,ALPHA GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 648 Anisotropic angular distributions in Legendre polynomial 825 1451 649 representation are given for the 0.1693-, 3.6845- and 3.8538- 825 1451 650 MeV gamma rays, obtained by fitting the measurements of Nelson 825 1451 651 et al. [Ne99]. Isotropic angular distributions are assumed for 825 1451 652 all the remaining gamma rays. 825 1451 653 825 1451 654 **************************************************************** 825 1451 655 825 1451 656 SUMMARY OF DATA VALIDATION OF THIS FILE AGAINST INTEGRAL 825 1451 657 BENCHMARKS 825 1451 658 825 1451 659 KAPL (Weinman, Caro, Lubitz) performed a number of data 825 1451 660 validation benchmark calculations to test the performance of this 825 1451 661 file (June-August 2001). This O16 evaluation gives consistently 825 1451 662 good results for the 21 CSWEG solution critical calculations, the 825 1451 663 liquid-oxygen broomstick neutron-transmission experiment, and the 825 1451 664 neutron age in water experiment (see below for more details). 825 1451 665 825 1451 666 A) 21 CSWEG solution critical calculations. Weinman calculated a 825 1451 667 set of 21 ORNL and Rocky Flats benchmark solution criticals used 825 1451 668 for CSEWG analyses. These calculations were run with ENDF/B-VI 825 1451 669 release 5 U235 (Leal,Larson,wright,Derrien) and hydrogen (332.0 825 1451 670 mbarns 2200m/s). Four different oxygen 16 cross section 825 1451 671 evaluations were considered. 825 1451 672 825 1451 673 1. KAPL-Caro 825 1451 674 2. This evaluation (which contains the KAPL data below 3.4 MeV) 825 1451 675 3. ENDF/B-VI MOD 2 825 1451 676 4. JENDL 3.2 825 1451 677 825 1451 678 All four O16 cross section evaluations gave good reactivity 825 1451 679 responses versus our fitting parameter above-thermal-leakage ATL. 825 1451 680 The ATL parameter is a sensitive trending variable to high energy 825 1451 681 scattering cross sections. All four O16 evaluations produced 825 1451 682 eigenvalues whose mean values were all close to unity and only 825 1451 683 the older ENDF/B-VI.2 cross section evaluation gave a slight 825 1451 684 reactivity trend (about .0020 Delta Keff over the range). The 825 1451 685 average eigenvalues and slopes are listed below. 825 1451 686 825 1451 687 Library Av. Keff Slope 825 1451 688 825 1451 689 KAPL-Caro 0.9993 +.0001 825 1451 690 This file 0.9996 +.0004 825 1451 691 ENDF/B-VI.2 1.0003 +.0032 825 1451 692 JENDL 3.2 1.0004 -.0002 825 1451 693 825 1451 694 Thus the reactivity trend, labeled "slope" in the table above, is 825 1451 695 much smaller in the new file compared to the previous ENDF/B-VI.2 825 1451 696 evaluation. 825 1451 697 825 1451 698 B) The liquid-oxygen broomstick experiment. The oxygen window at 825 1451 699 2.3 MeV is the most important feature at which energy the 825 1451 700 greatest transmission takes place. The new evaluation produces 825 1451 701 close to exact agreement with the experiment in the energy range 825 1451 702 of the oxygen window. The previous ENDF/B-VI value is slightly 825 1451 703 below the experimental value. At energies higher than 5.5 MeV, 825 1451 704 the new evaluation produces slightly better results than does the 825 1451 705 previous ENDF/B-VI results. 825 1451 706 825 1451 707 C) Neutron age in water. KAPL obtained 26.4 to be compared 825 1451 708 against an experimental value of 26.6 +/- 0.6. The previous 825 1451 709 ENDF/B-VI file gave a result of 26.3. 825 1451 710 825 1451 711 Additionally, A.C. (Skip) Kahler at Bettis lab undertook 825 1451 712 benchmark testing of this file (memo, May 16, 2001) against 825 1451 713 thermal benchmarks documented in the Int. Handbook of Evaluated 825 1451 714 Criticality Safety Benchmark Experiments, as well as the L5 and 825 1451 715 L6 ORNL benchmarks. 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Conf. on Nuclear Data for Science and Technology (2007) 825 1451 830 825 1451 831 ************************ C O N T E N T S *********************** 825 1451 832 1 451 976 3 825 1451 833 2 151 4 3 825 1451 834 3 1 775 3 825 1451 835 3 2 775 3 825 1451 836 3 3 775 3 825 1451 837 3 4 97 3 825 1451 838 3 5 38 3 825 1451 839 3 16 32 3 825 1451 840 3 22 50 3 825 1451 841 3 23 33 3 825 1451 842 3 28 41 3 825 1451 843 3 32 20 3 825 1451 844 3 41 15 3 825 1451 845 3 44 16 3 825 1451 846 3 45 14 3 825 1451 847 3 51 97 3 825 1451 848 3 52 96 3 825 1451 849 3 53 90 3 825 1451 850 3 54 88 3 825 1451 851 3 55 74 3 825 1451 852 3 56 63 3 825 1451 853 3 57 62 3 825 1451 854 3 91 69 3 825 1451 855 3 102 5 3 825 1451 856 3 103 60 3 825 1451 857 3 104 64 3 825 1451 858 3 105 41 3 825 1451 859 3 107 406 3 825 1451 860 3 108 39 3 825 1451 861 3 112 22 3 825 1451 862 3 600 60 3 825 1451 863 3 601 59 3 825 1451 864 3 602 58 3 825 1451 865 3 603 57 3 825 1451 866 3 650 64 3 825 1451 867 3 651 41 3 825 1451 868 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